Enhanced supercapacitor performance of a 3D architecture tailored using atomically thin rGO-MoS2 2D sheets
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Data de Publicação: | 2016 |
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Tipo de documento: | Artigo |
Título da fonte: | Repositório da Produção Científica e Intelectual da Unicamp |
Texto Completo: | https://hdl.handle.net/20.500.12733/1667482 |
Resumo: | Agradecimentos: Sujin P. Jose and C. R. Gautam acknowledge the financial support from Indo-US Raman Post-Doctoral Research Fellowship, The University Grants Commission New Delhi, Government of India (06-01-04-SF1513) CST acknowledge the funding support from the U.S. Department of Defense: the U.S. Air Force Office of Scientific Research for the Project MURI: "Synthesis and Characterization of 3-D Carbon Nanotube Solid Networks" Award No. etFA9550-12-1-0035. LDM and DSG acknowledge computational and financial support from the Center for Computational Engineering and Sciences at Unicamp through the FAPESP/CEPID Grant No. 2013/08293-7. LDM acknowledges financial support from the Brazilian Federal Agency CAPES via its PNPD program |
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Enhanced supercapacitor performance of a 3D architecture tailored using atomically thin rGO-MoS2 2D sheetsÓxido de grafeno reduzidoDinâmica molecularDissulfeto de molibdênioReduced graphene oxideMolecular dynamicsMolybdenum disulfideArtigo originalAgradecimentos: Sujin P. Jose and C. R. Gautam acknowledge the financial support from Indo-US Raman Post-Doctoral Research Fellowship, The University Grants Commission New Delhi, Government of India (06-01-04-SF1513) CST acknowledge the funding support from the U.S. Department of Defense: the U.S. Air Force Office of Scientific Research for the Project MURI: "Synthesis and Characterization of 3-D Carbon Nanotube Solid Networks" Award No. etFA9550-12-1-0035. LDM and DSG acknowledge computational and financial support from the Center for Computational Engineering and Sciences at Unicamp through the FAPESP/CEPID Grant No. 2013/08293-7. LDM acknowledges financial support from the Brazilian Federal Agency CAPES via its PNPD programAbstract: A 3D architecture is fabricated using 2D nano-sheets of GO and MoS2 as the building blocks by a facile, one-pot chronoamperometry method to achieve a conductive additive free, binder free and scalable supercapacitor electrode. The superior electrochemical properties of the 3D PPy-rGO-MoS2 (PGMo) are due to its porous structure, thin wall, high surface area and high electrical conductivity that endow rapid transportation of electrolyte ions and electrons throughout the electrode matrix. The synergistic effect between the components in a proper ratio improves the supercapacitor performance and material stability of PGMo. The possible correlation of the structure and electrochemical performance of the 3D ternary composite is backed by a fully atomistic molecular dynamics (MD) simulation study. The high specific capacitance (387 F g(-1)) and impressive cycling stability (>1000 cycles) estimated for PGMo open up an opportunity to consider the 3D ternary nanostructures as cutting edge materials for energy storage solutionsFUNDAÇÃO DE AMPARO À PESQUISA DO ESTADO DE SÃO PAULO - FAPESPCOORDENAÇÃO DE APERFEIÇOAMENTO DE PESSOAL DE NÍVEL SUPERIOR - CAPESAbertoUNIVERSIDADE ESTADUAL DE CAMPINASMachado, Leonardo Dantas, 1982-Galvão, Douglas Soares, 1961-2016info:eu-repo/semantics/publishedVersioninfo:eu-repo/semantics/articleapplication/pdfhttps://hdl.handle.net/20.500.12733/1667482MACHADO, Leonardo Dantas; GALVÃO, Douglas Soares. Enhanced supercapacitor performance of a 3D architecture tailored using atomically thin rGO-MoS2 2D sheets. RSC advances. Cambridge : Royal Society of Chemistry, 2016. Vol. 6, n. 96 (Sept., 2016), p. 93384-93393. Disponível em: https://hdl.handle.net/20.500.12733/1667482. Acesso em: 24 mai. 2023.Inglêshttps://repositorio.unicamp.br/acervo/detalhe/1221228reponame:Repositório da Produção Científica e Intelectual da Unicampinstname:Universidade Estadual de Campinas (UNICAMP)instacron:UNICAMPinfo:eu-repo/semantics/openAccess2022-06-01T12:17:51Zoai:https://www.repositorio.unicamp.br/:1221228Repositório InstitucionalPUBhttp://repositorio.unicamp.br/oai/requestreposip@unicamp.bropendoar:2022-06-01T12:17:51Repositório da Produção Científica e Intelectual da Unicamp - Universidade Estadual de Campinas (UNICAMP)false |
dc.title.none.fl_str_mv |
Enhanced supercapacitor performance of a 3D architecture tailored using atomically thin rGO-MoS2 2D sheets |
title |
Enhanced supercapacitor performance of a 3D architecture tailored using atomically thin rGO-MoS2 2D sheets |
spellingShingle |
Enhanced supercapacitor performance of a 3D architecture tailored using atomically thin rGO-MoS2 2D sheets Machado, Leonardo Dantas, 1982- Óxido de grafeno reduzido Dinâmica molecular Dissulfeto de molibdênio Reduced graphene oxide Molecular dynamics Molybdenum disulfide Artigo original |
title_short |
Enhanced supercapacitor performance of a 3D architecture tailored using atomically thin rGO-MoS2 2D sheets |
title_full |
Enhanced supercapacitor performance of a 3D architecture tailored using atomically thin rGO-MoS2 2D sheets |
title_fullStr |
Enhanced supercapacitor performance of a 3D architecture tailored using atomically thin rGO-MoS2 2D sheets |
title_full_unstemmed |
Enhanced supercapacitor performance of a 3D architecture tailored using atomically thin rGO-MoS2 2D sheets |
title_sort |
Enhanced supercapacitor performance of a 3D architecture tailored using atomically thin rGO-MoS2 2D sheets |
author |
Machado, Leonardo Dantas, 1982- |
author_facet |
Machado, Leonardo Dantas, 1982- Galvão, Douglas Soares, 1961- |
author_role |
author |
author2 |
Galvão, Douglas Soares, 1961- |
author2_role |
author |
dc.contributor.none.fl_str_mv |
UNIVERSIDADE ESTADUAL DE CAMPINAS |
dc.contributor.author.fl_str_mv |
Machado, Leonardo Dantas, 1982- Galvão, Douglas Soares, 1961- |
dc.subject.por.fl_str_mv |
Óxido de grafeno reduzido Dinâmica molecular Dissulfeto de molibdênio Reduced graphene oxide Molecular dynamics Molybdenum disulfide Artigo original |
topic |
Óxido de grafeno reduzido Dinâmica molecular Dissulfeto de molibdênio Reduced graphene oxide Molecular dynamics Molybdenum disulfide Artigo original |
description |
Agradecimentos: Sujin P. Jose and C. R. Gautam acknowledge the financial support from Indo-US Raman Post-Doctoral Research Fellowship, The University Grants Commission New Delhi, Government of India (06-01-04-SF1513) CST acknowledge the funding support from the U.S. Department of Defense: the U.S. Air Force Office of Scientific Research for the Project MURI: "Synthesis and Characterization of 3-D Carbon Nanotube Solid Networks" Award No. etFA9550-12-1-0035. LDM and DSG acknowledge computational and financial support from the Center for Computational Engineering and Sciences at Unicamp through the FAPESP/CEPID Grant No. 2013/08293-7. LDM acknowledges financial support from the Brazilian Federal Agency CAPES via its PNPD program |
publishDate |
2016 |
dc.date.none.fl_str_mv |
2016 |
dc.type.status.fl_str_mv |
info:eu-repo/semantics/publishedVersion |
dc.type.driver.fl_str_mv |
info:eu-repo/semantics/article |
format |
article |
status_str |
publishedVersion |
dc.identifier.uri.fl_str_mv |
https://hdl.handle.net/20.500.12733/1667482 MACHADO, Leonardo Dantas; GALVÃO, Douglas Soares. Enhanced supercapacitor performance of a 3D architecture tailored using atomically thin rGO-MoS2 2D sheets. RSC advances. Cambridge : Royal Society of Chemistry, 2016. Vol. 6, n. 96 (Sept., 2016), p. 93384-93393. Disponível em: https://hdl.handle.net/20.500.12733/1667482. Acesso em: 24 mai. 2023. |
url |
https://hdl.handle.net/20.500.12733/1667482 |
identifier_str_mv |
MACHADO, Leonardo Dantas; GALVÃO, Douglas Soares. Enhanced supercapacitor performance of a 3D architecture tailored using atomically thin rGO-MoS2 2D sheets. RSC advances. Cambridge : Royal Society of Chemistry, 2016. Vol. 6, n. 96 (Sept., 2016), p. 93384-93393. Disponível em: https://hdl.handle.net/20.500.12733/1667482. Acesso em: 24 mai. 2023. |
dc.language.iso.fl_str_mv |
Inglês |
language_invalid_str_mv |
Inglês |
dc.relation.none.fl_str_mv |
https://repositorio.unicamp.br/acervo/detalhe/1221228 |
dc.rights.driver.fl_str_mv |
info:eu-repo/semantics/openAccess |
eu_rights_str_mv |
openAccess |
dc.format.none.fl_str_mv |
application/pdf |
dc.source.none.fl_str_mv |
reponame:Repositório da Produção Científica e Intelectual da Unicamp instname:Universidade Estadual de Campinas (UNICAMP) instacron:UNICAMP |
instname_str |
Universidade Estadual de Campinas (UNICAMP) |
instacron_str |
UNICAMP |
institution |
UNICAMP |
reponame_str |
Repositório da Produção Científica e Intelectual da Unicamp |
collection |
Repositório da Produção Científica e Intelectual da Unicamp |
repository.name.fl_str_mv |
Repositório da Produção Científica e Intelectual da Unicamp - Universidade Estadual de Campinas (UNICAMP) |
repository.mail.fl_str_mv |
reposip@unicamp.br |
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1766887317720530944 |