Light management with quantum nanostructured dots-in-host semiconductors

Detalhes bibliográficos
Autor(a) principal: Alexandre, Miguel
Data de Publicação: 2021
Outros Autores: Águas, Hugo, Fortunato, Elvira, Martins, Rodrigo, Mendes, Manuel João
Tipo de documento: Artigo
Idioma: eng
Título da fonte: Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos)
Texto Completo: http://hdl.handle.net/10362/128327
Resumo: PTCD/NAN-OPT/28837/2017
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spelling Light management with quantum nanostructured dots-in-host semiconductorsElectronic, Optical and Magnetic MaterialsAtomic and Molecular Physics, and OpticsPTCD/NAN-OPT/28837/2017Insightful knowledge on quantum nanostructured materials is paramount to engineer and exploit their vast gamut of applications. Here, a formalism based on the single-band effective mass equation was developed to determine the light absorption of colloidal quantum dots (CQDs) embedded in a wider bandgap semiconductor host, employing only three parameters (dots/host potential barrier, effective mass, and QD size). It was ascertained how to tune such parameters to design the energy level structure and consequent optical response. Our findings show that the CQD size has the biggest effect on the number and energy of the confined levels, while the potential barrier causes a linear shift of their values. While smaller QDs allow wider energetic separation between levels (as desired for most quantum-based technologies), the larger dots with higher number of levels are those that exhibit the strongest absorption. Nevertheless, it was unprecedently shown that such quantum-enabled absorption coefficients can reach the levels (104–105cm−1) of bulk semiconductors. [Figure not available: see fulltext.]CENIMAT-i3N - Centro de Investigação de Materiais (Lab. Associado I3N)DCM - Departamento de Ciência dos MateriaisUNINOVA-Instituto de Desenvolvimento de Novas TecnologiasRUNAlexandre, MiguelÁguas, HugoFortunato, ElviraMartins, RodrigoMendes, Manuel João2021-11-26T23:45:00Z2021-122021-12-01T00:00:00Zinfo:eu-repo/semantics/publishedVersioninfo:eu-repo/semantics/articleapplication/pdfhttp://hdl.handle.net/10362/128327eng2095-5545PURE: 35022797https://doi.org/10.1038/s41377-021-00671-xinfo:eu-repo/semantics/openAccessreponame:Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos)instname:Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informaçãoinstacron:RCAAP2024-03-11T05:07:59Zoai:run.unl.pt:10362/128327Portal AgregadorONGhttps://www.rcaap.pt/oai/openaireopendoar:71602024-03-20T03:46:17.683471Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) - Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informaçãofalse
dc.title.none.fl_str_mv Light management with quantum nanostructured dots-in-host semiconductors
title Light management with quantum nanostructured dots-in-host semiconductors
spellingShingle Light management with quantum nanostructured dots-in-host semiconductors
Alexandre, Miguel
Electronic, Optical and Magnetic Materials
Atomic and Molecular Physics, and Optics
title_short Light management with quantum nanostructured dots-in-host semiconductors
title_full Light management with quantum nanostructured dots-in-host semiconductors
title_fullStr Light management with quantum nanostructured dots-in-host semiconductors
title_full_unstemmed Light management with quantum nanostructured dots-in-host semiconductors
title_sort Light management with quantum nanostructured dots-in-host semiconductors
author Alexandre, Miguel
author_facet Alexandre, Miguel
Águas, Hugo
Fortunato, Elvira
Martins, Rodrigo
Mendes, Manuel João
author_role author
author2 Águas, Hugo
Fortunato, Elvira
Martins, Rodrigo
Mendes, Manuel João
author2_role author
author
author
author
dc.contributor.none.fl_str_mv CENIMAT-i3N - Centro de Investigação de Materiais (Lab. Associado I3N)
DCM - Departamento de Ciência dos Materiais
UNINOVA-Instituto de Desenvolvimento de Novas Tecnologias
RUN
dc.contributor.author.fl_str_mv Alexandre, Miguel
Águas, Hugo
Fortunato, Elvira
Martins, Rodrigo
Mendes, Manuel João
dc.subject.por.fl_str_mv Electronic, Optical and Magnetic Materials
Atomic and Molecular Physics, and Optics
topic Electronic, Optical and Magnetic Materials
Atomic and Molecular Physics, and Optics
description PTCD/NAN-OPT/28837/2017
publishDate 2021
dc.date.none.fl_str_mv 2021-11-26T23:45:00Z
2021-12
2021-12-01T00:00:00Z
dc.type.status.fl_str_mv info:eu-repo/semantics/publishedVersion
dc.type.driver.fl_str_mv info:eu-repo/semantics/article
format article
status_str publishedVersion
dc.identifier.uri.fl_str_mv http://hdl.handle.net/10362/128327
url http://hdl.handle.net/10362/128327
dc.language.iso.fl_str_mv eng
language eng
dc.relation.none.fl_str_mv 2095-5545
PURE: 35022797
https://doi.org/10.1038/s41377-021-00671-x
dc.rights.driver.fl_str_mv info:eu-repo/semantics/openAccess
eu_rights_str_mv openAccess
dc.format.none.fl_str_mv application/pdf
dc.source.none.fl_str_mv reponame:Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos)
instname:Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informação
instacron:RCAAP
instname_str Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informação
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reponame_str Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos)
collection Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos)
repository.name.fl_str_mv Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) - Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informação
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