Nanofiltration combined with ozone-based processes for the removal of antineoplastic drugs from wastewater effluents
| Autor(a) principal: | |
|---|---|
| Data de Publicação: | 2023 |
| Outros Autores: | , , , , , , , , |
| Tipo de documento: | Artigo |
| Idioma: | eng |
| Título da fonte: | Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) |
| Texto Completo: | http://hdl.handle.net/10362/164428 |
Resumo: | Funding Information: This research was financially supported by: (i) Project POCI-01-0145-FEDER-031297 (CytoStraTech)—funded by FEDER funds through COMPETE2020—Programa Operacional Competitividade e Internacionalização (POCI) and by national funds (PIDDAC) through FCT /MCTES; (ii) NORTE-01-0145-FEDER-000069 (Healthy Waters) co-funded by European Regional Development Fund (ERDF), through North Portugal Regional Operational Programme (NORTE2020), under the PORTUGAL 2020 Partnership Agreement; (iii) 2022.08738.PTDC (DRopH2O) funded by national funds through FCT/MCTES (PIDDAC); (iv) UIDB/04750/2020 (EPIUnit) and LA/P/0064/2020 (ITR), funded by national funds through the FCT - Foundation for Science and Technology, I.P.; (v) LA/P/0045/2020 (ALiCE), Base Fundings UIDB/00511/2020 and UIDP/00511/2020 (LEPABE) and UIDB/50020/2020 and UIDP/50020/2020 (LSRE-LCM), funded by national funds through FCT/MCTES (PIDDAC); and (vi) iNOVA4Health (UIDB/04462/2020 and UIDP/04462/2020) and LS4FUTURE Associated Laboratory (LA/P/0087/2020) financially supported by national funds through the FCT/MCTES. Associate Laboratory for Green Chemistry- LAQV which is financed by national funds from FCT/MCTES (UIDB/50006/2020 and UIDP/50006/2020) is gratefully acknowledged. Teresa I.A. Gouveia would like to thank the Portuguese Foundation for Science and Technology (FCT) for her Ph.D. grant (SFRH/BD/147301/2019). ARLR acknowledges FCT funding under the Scientific Employment Stimulus - Individual Call (2022.00184.CEECIND). Publisher Copyright: © 2023 |
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Nanofiltration combined with ozone-based processes for the removal of antineoplastic drugs from wastewater effluentsAnticancer drugsCytostaticsNanofiltrationOzonationPeroxoneRisk assessmentWastewater effluentEnvironmental EngineeringWaste Management and DisposalManagement, Monitoring, Policy and LawSDG 3 - Good Health and Well-beingSDG 6 - Clean Water and SanitationSDG 11 - Sustainable Cities and CommunitiesSDG 14 - Life Below WaterFunding Information: This research was financially supported by: (i) Project POCI-01-0145-FEDER-031297 (CytoStraTech)—funded by FEDER funds through COMPETE2020—Programa Operacional Competitividade e Internacionalização (POCI) and by national funds (PIDDAC) through FCT /MCTES; (ii) NORTE-01-0145-FEDER-000069 (Healthy Waters) co-funded by European Regional Development Fund (ERDF), through North Portugal Regional Operational Programme (NORTE2020), under the PORTUGAL 2020 Partnership Agreement; (iii) 2022.08738.PTDC (DRopH2O) funded by national funds through FCT/MCTES (PIDDAC); (iv) UIDB/04750/2020 (EPIUnit) and LA/P/0064/2020 (ITR), funded by national funds through the FCT - Foundation for Science and Technology, I.P.; (v) LA/P/0045/2020 (ALiCE), Base Fundings UIDB/00511/2020 and UIDP/00511/2020 (LEPABE) and UIDB/50020/2020 and UIDP/50020/2020 (LSRE-LCM), funded by national funds through FCT/MCTES (PIDDAC); and (vi) iNOVA4Health (UIDB/04462/2020 and UIDP/04462/2020) and LS4FUTURE Associated Laboratory (LA/P/0087/2020) financially supported by national funds through the FCT/MCTES. Associate Laboratory for Green Chemistry- LAQV which is financed by national funds from FCT/MCTES (UIDB/50006/2020 and UIDP/50006/2020) is gratefully acknowledged. Teresa I.A. Gouveia would like to thank the Portuguese Foundation for Science and Technology (FCT) for her Ph.D. grant (SFRH/BD/147301/2019). ARLR acknowledges FCT funding under the Scientific Employment Stimulus - Individual Call (2022.00184.CEECIND). Publisher Copyright: © 2023Over the past years, there has been an increasing concern about the occurrence of antineoplastic drugs in water bodies. The incomplete removal of these pharmaceuticals from wastewaters has been confirmed by several scientists, making it urgent to find a reliable technique or a combination of techniques capable to produce clean and safe water. In this work, the combination of nanofiltration and ozone (O3)-based processes (NF + O3, NF + O3/H2O2 and NF + O3/H2O2/UVA) was studied aiming to produce clean water from wastewater treatment plant (WWTP) secondary effluents to be safely discharged into water bodies, reused in daily practices such as aquaculture activities or for recharging aquifers used as abstraction sources for drinking water production. Nanofiltration was performed in a pilot-scale unit and O3-based processes in a continuous-flow column. The peroxone process (O3/H2O2) was considered the most promising technology to be coupled to nanofiltration, all the target pharmaceuticals being removed at an extent higher than 98% from WWTP secondary effluents, with a DOC reduction up to 92%. The applicability of the clean water stream for recharging aquifers used as abstraction sources for drinking water production was supported by a risk assessment approach, regarding the final concentrations of the target pharmaceuticals. Moreover, the toxicity of the nanofiltration retentate, a polluted stream generated from the nanofiltration system, was greatly decreased after the application of the peroxone process, which evidences the positive impact on the environment of implementing a NF + O3/H2O2 process.LAQV@REQUIMTEDQ - Departamento de QuímicaInstituto de Tecnologia Química e Biológica António Xavier (ITQB)RUNGouveia, Teresa I. A.Gorito, Ana M.Cristóvão, Maria B.Pereira, Vanessa J.Crespo, João G.Alves, ArmindaPereira, M. Fernando R.Ribeiro, Ana R. L.Silva, Adrián M. T.Santos, Mónica S. F.2024-03-05T00:13:01Z2023-12-152023-12-15T00:00:00Zinfo:eu-repo/semantics/publishedVersioninfo:eu-repo/semantics/article10application/pdfhttp://hdl.handle.net/10362/164428eng0301-4797PURE: 83896836https://doi.org/10.1016/j.jenvman.2023.119314info:eu-repo/semantics/openAccessreponame:Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos)instname:Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informaçãoinstacron:RCAAP2024-03-11T05:52:10Zoai:run.unl.pt:10362/164428Portal AgregadorONGhttps://www.rcaap.pt/oai/openaireopendoar:71602024-03-20T04:00:10.072146Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) - Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informaçãofalse |
| dc.title.none.fl_str_mv |
Nanofiltration combined with ozone-based processes for the removal of antineoplastic drugs from wastewater effluents |
| title |
Nanofiltration combined with ozone-based processes for the removal of antineoplastic drugs from wastewater effluents |
| spellingShingle |
Nanofiltration combined with ozone-based processes for the removal of antineoplastic drugs from wastewater effluents Gouveia, Teresa I. A. Anticancer drugs Cytostatics Nanofiltration Ozonation Peroxone Risk assessment Wastewater effluent Environmental Engineering Waste Management and Disposal Management, Monitoring, Policy and Law SDG 3 - Good Health and Well-being SDG 6 - Clean Water and Sanitation SDG 11 - Sustainable Cities and Communities SDG 14 - Life Below Water |
| title_short |
Nanofiltration combined with ozone-based processes for the removal of antineoplastic drugs from wastewater effluents |
| title_full |
Nanofiltration combined with ozone-based processes for the removal of antineoplastic drugs from wastewater effluents |
| title_fullStr |
Nanofiltration combined with ozone-based processes for the removal of antineoplastic drugs from wastewater effluents |
| title_full_unstemmed |
Nanofiltration combined with ozone-based processes for the removal of antineoplastic drugs from wastewater effluents |
| title_sort |
Nanofiltration combined with ozone-based processes for the removal of antineoplastic drugs from wastewater effluents |
| author |
Gouveia, Teresa I. A. |
| author_facet |
Gouveia, Teresa I. A. Gorito, Ana M. Cristóvão, Maria B. Pereira, Vanessa J. Crespo, João G. Alves, Arminda Pereira, M. Fernando R. Ribeiro, Ana R. L. Silva, Adrián M. T. Santos, Mónica S. F. |
| author_role |
author |
| author2 |
Gorito, Ana M. Cristóvão, Maria B. Pereira, Vanessa J. Crespo, João G. Alves, Arminda Pereira, M. Fernando R. Ribeiro, Ana R. L. Silva, Adrián M. T. Santos, Mónica S. F. |
| author2_role |
author author author author author author author author author |
| dc.contributor.none.fl_str_mv |
LAQV@REQUIMTE DQ - Departamento de Química Instituto de Tecnologia Química e Biológica António Xavier (ITQB) RUN |
| dc.contributor.author.fl_str_mv |
Gouveia, Teresa I. A. Gorito, Ana M. Cristóvão, Maria B. Pereira, Vanessa J. Crespo, João G. Alves, Arminda Pereira, M. Fernando R. Ribeiro, Ana R. L. Silva, Adrián M. T. Santos, Mónica S. F. |
| dc.subject.por.fl_str_mv |
Anticancer drugs Cytostatics Nanofiltration Ozonation Peroxone Risk assessment Wastewater effluent Environmental Engineering Waste Management and Disposal Management, Monitoring, Policy and Law SDG 3 - Good Health and Well-being SDG 6 - Clean Water and Sanitation SDG 11 - Sustainable Cities and Communities SDG 14 - Life Below Water |
| topic |
Anticancer drugs Cytostatics Nanofiltration Ozonation Peroxone Risk assessment Wastewater effluent Environmental Engineering Waste Management and Disposal Management, Monitoring, Policy and Law SDG 3 - Good Health and Well-being SDG 6 - Clean Water and Sanitation SDG 11 - Sustainable Cities and Communities SDG 14 - Life Below Water |
| description |
Funding Information: This research was financially supported by: (i) Project POCI-01-0145-FEDER-031297 (CytoStraTech)—funded by FEDER funds through COMPETE2020—Programa Operacional Competitividade e Internacionalização (POCI) and by national funds (PIDDAC) through FCT /MCTES; (ii) NORTE-01-0145-FEDER-000069 (Healthy Waters) co-funded by European Regional Development Fund (ERDF), through North Portugal Regional Operational Programme (NORTE2020), under the PORTUGAL 2020 Partnership Agreement; (iii) 2022.08738.PTDC (DRopH2O) funded by national funds through FCT/MCTES (PIDDAC); (iv) UIDB/04750/2020 (EPIUnit) and LA/P/0064/2020 (ITR), funded by national funds through the FCT - Foundation for Science and Technology, I.P.; (v) LA/P/0045/2020 (ALiCE), Base Fundings UIDB/00511/2020 and UIDP/00511/2020 (LEPABE) and UIDB/50020/2020 and UIDP/50020/2020 (LSRE-LCM), funded by national funds through FCT/MCTES (PIDDAC); and (vi) iNOVA4Health (UIDB/04462/2020 and UIDP/04462/2020) and LS4FUTURE Associated Laboratory (LA/P/0087/2020) financially supported by national funds through the FCT/MCTES. Associate Laboratory for Green Chemistry- LAQV which is financed by national funds from FCT/MCTES (UIDB/50006/2020 and UIDP/50006/2020) is gratefully acknowledged. Teresa I.A. Gouveia would like to thank the Portuguese Foundation for Science and Technology (FCT) for her Ph.D. grant (SFRH/BD/147301/2019). ARLR acknowledges FCT funding under the Scientific Employment Stimulus - Individual Call (2022.00184.CEECIND). Publisher Copyright: © 2023 |
| publishDate |
2023 |
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2023-12-15 2023-12-15T00:00:00Z 2024-03-05T00:13:01Z |
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info:eu-repo/semantics/publishedVersion |
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info:eu-repo/semantics/article |
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article |
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publishedVersion |
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http://hdl.handle.net/10362/164428 |
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http://hdl.handle.net/10362/164428 |
| dc.language.iso.fl_str_mv |
eng |
| language |
eng |
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0301-4797 PURE: 83896836 https://doi.org/10.1016/j.jenvman.2023.119314 |
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info:eu-repo/semantics/openAccess |
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openAccess |
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10 application/pdf |
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