Analytical quantitative semi-classical approach to the LoSurdo-Stark effect and ionization in 2D excitons
Autor(a) principal: | |
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Data de Publicação: | 2020 |
Outros Autores: | , , |
Tipo de documento: | Artigo |
Idioma: | eng |
Título da fonte: | Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) |
Texto Completo: | http://hdl.handle.net/1822/66036 |
Resumo: | Using a semiclassical approach, we derive a fully analytical expression for the ionization rate of excitons in two-dimensional materials due to an external static electric field, which eliminates the need for complicated numerical calculations. Our formula shows quantitative agreement with more sophisticated numerical methods based on the exterior complex scaling approach, which solves a non-Hermitian eigenvalue problem yielding complex energy eigenvalues, where the imaginary part describes the ionization rate. Results for excitons in hexagonal boron nitride and the A exciton in transition metal dichalcogenides are given as simple examples. The extension of the theory to include spin-orbit-split excitons in transition metal dichalcogenides is trivial. |
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Analytical quantitative semi-classical approach to the LoSurdo-Stark effect and ionization in 2D excitonsCiências Naturais::Ciências FísicasScience & TechnologyUsing a semiclassical approach, we derive a fully analytical expression for the ionization rate of excitons in two-dimensional materials due to an external static electric field, which eliminates the need for complicated numerical calculations. Our formula shows quantitative agreement with more sophisticated numerical methods based on the exterior complex scaling approach, which solves a non-Hermitian eigenvalue problem yielding complex energy eigenvalues, where the imaginary part describes the ionization rate. Results for excitons in hexagonal boron nitride and the A exciton in transition metal dichalcogenides are given as simple examples. The extension of the theory to include spin-orbit-split excitons in transition metal dichalcogenides is trivial.N.M.R.P. acknowledges support from the European Commission through the project “Graphene-Driven Revolutions in ICT and Beyond” (Ref. No. 881603 - core 3), and the Portuguese Foundation for Science and Technology (FCT) in the framework of the Strategic Financing UID/FIS/04650/2019. In addition, N. M. R. P. acknowledges COMPETE2020, PORTUGAL2020, FEDER and the Portuguese Foundation for Science and Technology (FCT) through projects POCI- 01-0145-FEDER-028114, POCI-01-0145-FEDER029265, PTDC/NAN-OPT/29265/2017, and POCI-01- 0145-FEDER-02888. H.C.K and T.G.P gratefully acknowledge financial support from the Center for Nanostructured Graphene (CNG), which is sponsored by the Danish National Research Foundation, Project No. DNRF103. Additionally, T.G.P. is supported by the QUSCOPE Center, sponsored by the Villum Foundation.American Physical SocietyUniversidade do MinhoHenriques, J. C. G.Kamban, Hogni C.Pedersen, Thomas G.Peres, N. M. R.20202020-01-01T00:00:00Zinfo:eu-repo/semantics/publishedVersioninfo:eu-repo/semantics/articleapplication/pdfhttp://hdl.handle.net/1822/66036eng2469-99502469-996910.1103/PhysRevB.102.035402https://journals.aps.org/prb/abstract/10.1103/PhysRevB.102.035402info:eu-repo/semantics/openAccessreponame:Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos)instname:Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informaçãoinstacron:RCAAP2023-07-21T12:44:11Zoai:repositorium.sdum.uminho.pt:1822/66036Portal AgregadorONGhttps://www.rcaap.pt/oai/openaireopendoar:71602024-03-19T19:41:49.596414Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) - Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informaçãofalse |
dc.title.none.fl_str_mv |
Analytical quantitative semi-classical approach to the LoSurdo-Stark effect and ionization in 2D excitons |
title |
Analytical quantitative semi-classical approach to the LoSurdo-Stark effect and ionization in 2D excitons |
spellingShingle |
Analytical quantitative semi-classical approach to the LoSurdo-Stark effect and ionization in 2D excitons Henriques, J. C. G. Ciências Naturais::Ciências Físicas Science & Technology |
title_short |
Analytical quantitative semi-classical approach to the LoSurdo-Stark effect and ionization in 2D excitons |
title_full |
Analytical quantitative semi-classical approach to the LoSurdo-Stark effect and ionization in 2D excitons |
title_fullStr |
Analytical quantitative semi-classical approach to the LoSurdo-Stark effect and ionization in 2D excitons |
title_full_unstemmed |
Analytical quantitative semi-classical approach to the LoSurdo-Stark effect and ionization in 2D excitons |
title_sort |
Analytical quantitative semi-classical approach to the LoSurdo-Stark effect and ionization in 2D excitons |
author |
Henriques, J. C. G. |
author_facet |
Henriques, J. C. G. Kamban, Hogni C. Pedersen, Thomas G. Peres, N. M. R. |
author_role |
author |
author2 |
Kamban, Hogni C. Pedersen, Thomas G. Peres, N. M. R. |
author2_role |
author author author |
dc.contributor.none.fl_str_mv |
Universidade do Minho |
dc.contributor.author.fl_str_mv |
Henriques, J. C. G. Kamban, Hogni C. Pedersen, Thomas G. Peres, N. M. R. |
dc.subject.por.fl_str_mv |
Ciências Naturais::Ciências Físicas Science & Technology |
topic |
Ciências Naturais::Ciências Físicas Science & Technology |
description |
Using a semiclassical approach, we derive a fully analytical expression for the ionization rate of excitons in two-dimensional materials due to an external static electric field, which eliminates the need for complicated numerical calculations. Our formula shows quantitative agreement with more sophisticated numerical methods based on the exterior complex scaling approach, which solves a non-Hermitian eigenvalue problem yielding complex energy eigenvalues, where the imaginary part describes the ionization rate. Results for excitons in hexagonal boron nitride and the A exciton in transition metal dichalcogenides are given as simple examples. The extension of the theory to include spin-orbit-split excitons in transition metal dichalcogenides is trivial. |
publishDate |
2020 |
dc.date.none.fl_str_mv |
2020 2020-01-01T00:00:00Z |
dc.type.status.fl_str_mv |
info:eu-repo/semantics/publishedVersion |
dc.type.driver.fl_str_mv |
info:eu-repo/semantics/article |
format |
article |
status_str |
publishedVersion |
dc.identifier.uri.fl_str_mv |
http://hdl.handle.net/1822/66036 |
url |
http://hdl.handle.net/1822/66036 |
dc.language.iso.fl_str_mv |
eng |
language |
eng |
dc.relation.none.fl_str_mv |
2469-9950 2469-9969 10.1103/PhysRevB.102.035402 https://journals.aps.org/prb/abstract/10.1103/PhysRevB.102.035402 |
dc.rights.driver.fl_str_mv |
info:eu-repo/semantics/openAccess |
eu_rights_str_mv |
openAccess |
dc.format.none.fl_str_mv |
application/pdf |
dc.publisher.none.fl_str_mv |
American Physical Society |
publisher.none.fl_str_mv |
American Physical Society |
dc.source.none.fl_str_mv |
reponame:Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) instname:Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informação instacron:RCAAP |
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Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informação |
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RCAAP |
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RCAAP |
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Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) |
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Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) |
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Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) - Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informação |
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1799132969233809408 |