Evaluation of the contamination of the subsurface and groundwater by monoaromatic hydrocarbons in an eastern Amazonian town in northern Brazil
Autor(a) principal: | |
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Data de Publicação: | 2023 |
Outros Autores: | , , , , , |
Tipo de documento: | Artigo |
Idioma: | eng |
Título da fonte: | Repositório Digital do Instituto Evandro Chagas (Patuá) |
Texto Completo: | https://patua.iec.gov.br/handle/iec/6726 |
Resumo: | The present study evaluated the contamination by monoaromatic hydrocarbons (BTEX: benzene, toluene, ethylbenzene, and xylene) of the subsurface of gas stations and adjacent residences in the Amazonian town of Bragança, in northern Brazil. We combined the ground penetrating radar (GPR) geophysical tool, to detect possible plumes of contamination by BTEX, with gas chromatography (GC) and mass spectrometry (MS), which were used to diagnose the presence of BTEX in water samples obtained from boreholes located within the study area. The GPR identifed low-amplitude refections in the vadose zone of two gas stations, whose attenuation near the surface was due to the low permittivity recorded in the radargrams, which may have been caused by the reduced permittivity of the hydrocarbons (gas vapor) in comparison with water. The GC–MS identifed benzene, toluene, ethylbenzene and/or xylene in 13 water samples (19.7% of the samples collected). Only three of the samples contained two contaminants, invariably toluene and xylene, whereas all the others contained only a single BTEX. Toluene and xylene were the BTEX compounds found most frequently in the samples. However, none of the samples collected in the study exceeded the threshold established by Brazilian legislation for BTEXs in drinking water. The integrated application of GPR and CG-MS produced satisfactory results for the diagnosis of the contamination of the subsurface of the gas stations surveyed in the present study |
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Gomes, Karen Jamile MoreiraOliva, Pedro Andrés ChiraRocha, Herson Oliveira daMendes, Rosivlado de AlcantaraCosta, Amilton César Gomes daMiranda, Camila dos SantosAlmeida, Nelise de Oliveira2023-03-09T12:05:50Z2023-03-09T12:05:50Z2023GOMES, Karen Jamile Moreira et al. Evaluation of the contamination of the subsurface and groundwater by monoaromatic hydrocarbons in an eastern Amazonian town in northern Brazil. Environmental Earth Sciences, v. 82, n. 23, p. 1-12, Jan. 2023. DOI: https://doi.org/10.1007/s12665-022-10680-71866-6299https://patua.iec.gov.br/handle/iec/672610.1007/s12665-022-10680-7The present study evaluated the contamination by monoaromatic hydrocarbons (BTEX: benzene, toluene, ethylbenzene, and xylene) of the subsurface of gas stations and adjacent residences in the Amazonian town of Bragança, in northern Brazil. We combined the ground penetrating radar (GPR) geophysical tool, to detect possible plumes of contamination by BTEX, with gas chromatography (GC) and mass spectrometry (MS), which were used to diagnose the presence of BTEX in water samples obtained from boreholes located within the study area. The GPR identifed low-amplitude refections in the vadose zone of two gas stations, whose attenuation near the surface was due to the low permittivity recorded in the radargrams, which may have been caused by the reduced permittivity of the hydrocarbons (gas vapor) in comparison with water. The GC–MS identifed benzene, toluene, ethylbenzene and/or xylene in 13 water samples (19.7% of the samples collected). Only three of the samples contained two contaminants, invariably toluene and xylene, whereas all the others contained only a single BTEX. Toluene and xylene were the BTEX compounds found most frequently in the samples. However, none of the samples collected in the study exceeded the threshold established by Brazilian legislation for BTEXs in drinking water. The integrated application of GPR and CG-MS produced satisfactory results for the diagnosis of the contamination of the subsurface of the gas stations surveyed in the present studyDean of Research and Graduate Studies - PROPESP/Federal University of Pará - UFPA (Brazil), Amazon Foundation for Studiesand Research - FAPESPA (Brazil).Federal University of Pará. Coastal Studies Institute. Laboratory of Cartography, Geoprocessing and Modeling. Bragança, PA, Brazil.Federal University of Pará. Coastal Studies Institute. Laboratory of Cartography, Geoprocessing and Modeling. Bragança, PA, Brazil.Federal Rural University of Amazonia - Parauapebas University Campus. Study Group in Geosciences, Engineering and Environment. Parauapebas, PA, Brazil.Ministério da Saúde. Secretaria de Ciência, Tecnologia, Inovação e Insumos Estratégicos. Instituto Evandro Chagas. Laboratório de Toxicologia. Ananindeua, PA, Brasil.Ministério da Saúde. Secretaria de Ciência, Tecnologia, Inovação e Insumos Estratégicos. Instituto Evandro Chagas. Laboratório de Toxicologia. Ananindeua, PA, Brasil.Federal Institute of Education, Science and Technology. Bragança, PA, Brazil.Federal University of Pará. Coastal Studies Institute. Laboratory of Cartography, Geoprocessing and Modeling. Bragança, PA, Brazil.engSpringerEvaluation of the contamination of the subsurface and groundwater by monoaromatic hydrocarbons in an eastern Amazonian town in northern Brazilinfo:eu-repo/semantics/publishedVersioninfo:eu-repo/semantics/articlePoluição Ambiental / análiseAnálise do SoloMonitoramento do SoloControle da Qualidade da ÁguaHidrocarbonetosPosto de CombustívelHabitaçãoBragança (PA)info:eu-repo/semantics/openAccessreponame:Repositório Digital do Instituto Evandro Chagas (Patuá)instname:Instituto Evandro Chagas (IEC)instacron:IECORIGINALEvaluation of the contamination of the subsurface and groundwater by monoaromatic hydrocarbons in an eastern Amazonian town in northern Brazil.pdfEvaluation of the contamination of the subsurface and groundwater by monoaromatic hydrocarbons in an eastern Amazonian town in northern Brazil.pdfapplication/pdf2082958https://patua.iec.gov.br/bitstreams/f4a09ad9-345d-483e-85b1-cf8f8651c261/download2899179f46f74137a26fb2b65104e819MD51LICENSElicense.txtlicense.txttext/plain; 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dc.title.pt_BR.fl_str_mv |
Evaluation of the contamination of the subsurface and groundwater by monoaromatic hydrocarbons in an eastern Amazonian town in northern Brazil |
title |
Evaluation of the contamination of the subsurface and groundwater by monoaromatic hydrocarbons in an eastern Amazonian town in northern Brazil |
spellingShingle |
Evaluation of the contamination of the subsurface and groundwater by monoaromatic hydrocarbons in an eastern Amazonian town in northern Brazil Gomes, Karen Jamile Moreira Poluição Ambiental / análise Análise do Solo Monitoramento do Solo Controle da Qualidade da Água Hidrocarbonetos Posto de Combustível Habitação Bragança (PA) |
title_short |
Evaluation of the contamination of the subsurface and groundwater by monoaromatic hydrocarbons in an eastern Amazonian town in northern Brazil |
title_full |
Evaluation of the contamination of the subsurface and groundwater by monoaromatic hydrocarbons in an eastern Amazonian town in northern Brazil |
title_fullStr |
Evaluation of the contamination of the subsurface and groundwater by monoaromatic hydrocarbons in an eastern Amazonian town in northern Brazil |
title_full_unstemmed |
Evaluation of the contamination of the subsurface and groundwater by monoaromatic hydrocarbons in an eastern Amazonian town in northern Brazil |
title_sort |
Evaluation of the contamination of the subsurface and groundwater by monoaromatic hydrocarbons in an eastern Amazonian town in northern Brazil |
author |
Gomes, Karen Jamile Moreira |
author_facet |
Gomes, Karen Jamile Moreira Oliva, Pedro Andrés Chira Rocha, Herson Oliveira da Mendes, Rosivlado de Alcantara Costa, Amilton César Gomes da Miranda, Camila dos Santos Almeida, Nelise de Oliveira |
author_role |
author |
author2 |
Oliva, Pedro Andrés Chira Rocha, Herson Oliveira da Mendes, Rosivlado de Alcantara Costa, Amilton César Gomes da Miranda, Camila dos Santos Almeida, Nelise de Oliveira |
author2_role |
author author author author author author |
dc.contributor.author.fl_str_mv |
Gomes, Karen Jamile Moreira Oliva, Pedro Andrés Chira Rocha, Herson Oliveira da Mendes, Rosivlado de Alcantara Costa, Amilton César Gomes da Miranda, Camila dos Santos Almeida, Nelise de Oliveira |
dc.subject.decsPrimary.pt_BR.fl_str_mv |
Poluição Ambiental / análise Análise do Solo Monitoramento do Solo Controle da Qualidade da Água Hidrocarbonetos Posto de Combustível Habitação Bragança (PA) |
topic |
Poluição Ambiental / análise Análise do Solo Monitoramento do Solo Controle da Qualidade da Água Hidrocarbonetos Posto de Combustível Habitação Bragança (PA) |
description |
The present study evaluated the contamination by monoaromatic hydrocarbons (BTEX: benzene, toluene, ethylbenzene, and xylene) of the subsurface of gas stations and adjacent residences in the Amazonian town of Bragança, in northern Brazil. We combined the ground penetrating radar (GPR) geophysical tool, to detect possible plumes of contamination by BTEX, with gas chromatography (GC) and mass spectrometry (MS), which were used to diagnose the presence of BTEX in water samples obtained from boreholes located within the study area. The GPR identifed low-amplitude refections in the vadose zone of two gas stations, whose attenuation near the surface was due to the low permittivity recorded in the radargrams, which may have been caused by the reduced permittivity of the hydrocarbons (gas vapor) in comparison with water. The GC–MS identifed benzene, toluene, ethylbenzene and/or xylene in 13 water samples (19.7% of the samples collected). Only three of the samples contained two contaminants, invariably toluene and xylene, whereas all the others contained only a single BTEX. Toluene and xylene were the BTEX compounds found most frequently in the samples. However, none of the samples collected in the study exceeded the threshold established by Brazilian legislation for BTEXs in drinking water. The integrated application of GPR and CG-MS produced satisfactory results for the diagnosis of the contamination of the subsurface of the gas stations surveyed in the present study |
publishDate |
2023 |
dc.date.accessioned.fl_str_mv |
2023-03-09T12:05:50Z |
dc.date.available.fl_str_mv |
2023-03-09T12:05:50Z |
dc.date.issued.fl_str_mv |
2023 |
dc.type.status.fl_str_mv |
info:eu-repo/semantics/publishedVersion |
dc.type.driver.fl_str_mv |
info:eu-repo/semantics/article |
format |
article |
status_str |
publishedVersion |
dc.identifier.citation.fl_str_mv |
GOMES, Karen Jamile Moreira et al. Evaluation of the contamination of the subsurface and groundwater by monoaromatic hydrocarbons in an eastern Amazonian town in northern Brazil. Environmental Earth Sciences, v. 82, n. 23, p. 1-12, Jan. 2023. DOI: https://doi.org/10.1007/s12665-022-10680-7 |
dc.identifier.uri.fl_str_mv |
https://patua.iec.gov.br/handle/iec/6726 |
dc.identifier.issn.-.fl_str_mv |
1866-6299 |
dc.identifier.doi.pt_BR.fl_str_mv |
10.1007/s12665-022-10680-7 |
identifier_str_mv |
GOMES, Karen Jamile Moreira et al. Evaluation of the contamination of the subsurface and groundwater by monoaromatic hydrocarbons in an eastern Amazonian town in northern Brazil. Environmental Earth Sciences, v. 82, n. 23, p. 1-12, Jan. 2023. DOI: https://doi.org/10.1007/s12665-022-10680-7 1866-6299 10.1007/s12665-022-10680-7 |
url |
https://patua.iec.gov.br/handle/iec/6726 |
dc.language.iso.fl_str_mv |
eng |
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eng |
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info:eu-repo/semantics/openAccess |
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openAccess |
dc.publisher.none.fl_str_mv |
Springer |
publisher.none.fl_str_mv |
Springer |
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reponame:Repositório Digital do Instituto Evandro Chagas (Patuá) instname:Instituto Evandro Chagas (IEC) instacron:IEC |
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Instituto Evandro Chagas (IEC) |
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IEC |
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IEC |
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Repositório Digital do Instituto Evandro Chagas (Patuá) |
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Repositório Digital do Instituto Evandro Chagas (Patuá) |
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