Manufacturing low enriched uranium metal by magnesiothermic reduction of UF4
Autor(a) principal: | |
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Data de Publicação: | 2018 |
Outros Autores: | , , , , |
Tipo de documento: | Artigo de conferência |
Título da fonte: | Repositório Institucional do IPEN |
Texto Completo: | http://repositorio.ipen.br/handle/123456789/29123 |
Resumo: | This work presents an experimental description of thermal and physical studies to attain a practical manufacturing process of uranium metal enriched to 20% U235 (LEU???Low Enriched Uranium) by metallothermic reduction of UF4, with nuclear purity, for reduced amounts (1000g of uranium). The magnesiothermic reduction is influenced by the thermal conditions for UF4 reduction. These variables are investigated. The physical arrangement of the crucible/reduction reactor/furnace system and the management of the furnace thermal input in the reduction reactor during the heating were studied. Thermal simulation experiments provided delineation for the reactants??? thermal progress before the ignition of the reaction. The heat input to the reduction system has proved to be the main variable that influenced the efficiency of the process. The levels of metallic yield and reproducibility have been improved. The typical yield in the production of uranium metal was above 80%. |
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2018-09-13T12:29:23Z2018-09-13T12:29:23ZMarch 11-15, 2018http://repositorio.ipen.br/handle/123456789/29123This work presents an experimental description of thermal and physical studies to attain a practical manufacturing process of uranium metal enriched to 20% U235 (LEU???Low Enriched Uranium) by metallothermic reduction of UF4, with nuclear purity, for reduced amounts (1000g of uranium). The magnesiothermic reduction is influenced by the thermal conditions for UF4 reduction. These variables are investigated. The physical arrangement of the crucible/reduction reactor/furnace system and the management of the furnace thermal input in the reduction reactor during the heating were studied. Thermal simulation experiments provided delineation for the reactants??? thermal progress before the ignition of the reaction. The heat input to the reduction system has proved to be the main variable that influenced the efficiency of the process. The levels of metallic yield and reproducibility have been improved. The typical yield in the production of uranium metal was above 80%.Submitted by Marco Antonio Oliveira da Silva (maosilva@ipen.br) on 2018-09-13T12:29:23Z No. of bitstreams: 1 24939.pdf: 944263 bytes, checksum: f4ad648f13ff89656d8daab2e343ebb3 (MD5)Made available in DSpace on 2018-09-13T12:29:23Z (GMT). No. of bitstreams: 1 24939.pdf: 944263 bytes, checksum: f4ad648f13ff89656d8daab2e343ebb3 (MD5)Conselho Nacional de Desenvolvimento Cient??fico e Tecnol??gico (CNPq)CNPq: 304034/2015-0; 310274/2012-5; 470363/2012-61-12European Nuclear Societyuraniummetalsnuclear fuelsmaterials recoveryenriched uraniumfuelsfabricationManufacturing low enriched uranium metal by magnesiothermic reduction of UF4info:eu-repo/semantics/publishedVersioninfo:eu-repo/semantics/conferenceObjectRRFMIBrussels, BelgiumMunich, GermanyDURAZZO, M.SALIBA-SILVA, A.M.MARTINS, I.C.CARVALHO, E.F.U. deRIELLA, H.G.EUROPEAN RESEARCH REACTOR CONFERENCEinfo:eu-repo/semantics/openAccessreponame:Repositório Institucional do IPENinstname:Instituto de Pesquisas Energéticas e Nucleares (IPEN)instacron:IPEN249392018DURAZZO, M.SALIBA-SILVA, A.M.MARTINS, I.C.CARVALHO, E.F.U. de18-09Proceedings90961720895DURAZZO, M.:90:410:SSALIBA-SILVA, A.M.:961:410:NMARTINS, I.C.:720:410:NCARVALHO, E.F.U. DE:895:410:NORIGINAL24939.pdf24939.pdfapplication/pdf944263http://repositorio.ipen.br/bitstream/123456789/29123/1/24939.pdff4ad648f13ff89656d8daab2e343ebb3MD51LICENSElicense.txtlicense.txttext/plain; charset=utf-81748http://repositorio.ipen.br/bitstream/123456789/29123/2/license.txt8a4605be74aa9ea9d79846c1fba20a33MD52123456789/291232021-06-29 14:17:11.962oai:repositorio.ipen.br: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Repositório InstitucionalPUBhttp://repositorio.ipen.br/oai/requestbibl@ipen.bropendoar:45102021-06-29T14:17:11Repositório Institucional do IPEN - Instituto de Pesquisas Energéticas e Nucleares (IPEN)false |
dc.title.pt_BR.fl_str_mv |
Manufacturing low enriched uranium metal by magnesiothermic reduction of UF4 |
title |
Manufacturing low enriched uranium metal by magnesiothermic reduction of UF4 |
spellingShingle |
Manufacturing low enriched uranium metal by magnesiothermic reduction of UF4 DURAZZO, M. uranium metals nuclear fuels materials recovery enriched uranium fuels fabrication |
title_short |
Manufacturing low enriched uranium metal by magnesiothermic reduction of UF4 |
title_full |
Manufacturing low enriched uranium metal by magnesiothermic reduction of UF4 |
title_fullStr |
Manufacturing low enriched uranium metal by magnesiothermic reduction of UF4 |
title_full_unstemmed |
Manufacturing low enriched uranium metal by magnesiothermic reduction of UF4 |
title_sort |
Manufacturing low enriched uranium metal by magnesiothermic reduction of UF4 |
author |
DURAZZO, M. |
author_facet |
DURAZZO, M. SALIBA-SILVA, A.M. MARTINS, I.C. CARVALHO, E.F.U. de RIELLA, H.G. EUROPEAN RESEARCH REACTOR CONFERENCE |
author_role |
author |
author2 |
SALIBA-SILVA, A.M. MARTINS, I.C. CARVALHO, E.F.U. de RIELLA, H.G. EUROPEAN RESEARCH REACTOR CONFERENCE |
author2_role |
author author author author author |
dc.contributor.author.fl_str_mv |
DURAZZO, M. SALIBA-SILVA, A.M. MARTINS, I.C. CARVALHO, E.F.U. de RIELLA, H.G. EUROPEAN RESEARCH REACTOR CONFERENCE |
dc.subject.por.fl_str_mv |
uranium metals nuclear fuels materials recovery enriched uranium fuels fabrication |
topic |
uranium metals nuclear fuels materials recovery enriched uranium fuels fabrication |
description |
This work presents an experimental description of thermal and physical studies to attain a practical manufacturing process of uranium metal enriched to 20% U235 (LEU???Low Enriched Uranium) by metallothermic reduction of UF4, with nuclear purity, for reduced amounts (1000g of uranium). The magnesiothermic reduction is influenced by the thermal conditions for UF4 reduction. These variables are investigated. The physical arrangement of the crucible/reduction reactor/furnace system and the management of the furnace thermal input in the reduction reactor during the heating were studied. Thermal simulation experiments provided delineation for the reactants??? thermal progress before the ignition of the reaction. The heat input to the reduction system has proved to be the main variable that influenced the efficiency of the process. The levels of metallic yield and reproducibility have been improved. The typical yield in the production of uranium metal was above 80%. |
publishDate |
2018 |
dc.date.evento.pt_BR.fl_str_mv |
March 11-15, 2018 |
dc.date.accessioned.fl_str_mv |
2018-09-13T12:29:23Z |
dc.date.available.fl_str_mv |
2018-09-13T12:29:23Z |
dc.type.status.fl_str_mv |
info:eu-repo/semantics/publishedVersion |
dc.type.driver.fl_str_mv |
info:eu-repo/semantics/conferenceObject |
format |
conferenceObject |
status_str |
publishedVersion |
dc.identifier.uri.fl_str_mv |
http://repositorio.ipen.br/handle/123456789/29123 |
url |
http://repositorio.ipen.br/handle/123456789/29123 |
dc.rights.driver.fl_str_mv |
info:eu-repo/semantics/openAccess |
eu_rights_str_mv |
openAccess |
dc.format.none.fl_str_mv |
1-12 |
dc.coverage.pt_BR.fl_str_mv |
I |
dc.publisher.none.fl_str_mv |
European Nuclear Society |
publisher.none.fl_str_mv |
European Nuclear Society |
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reponame:Repositório Institucional do IPEN instname:Instituto de Pesquisas Energéticas e Nucleares (IPEN) instacron:IPEN |
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IPEN |
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IPEN |
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Repositório Institucional do IPEN |
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Repositório Institucional do IPEN |
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