Gasification of carbon deposited on supported Ni-Cu catalysts
Autor(a) principal: | |
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Data de Publicação: | 1986 |
Outros Autores: | , |
Tipo de documento: | Artigo |
Idioma: | eng |
Título da fonte: | Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) |
Texto Completo: | http://hdl.handle.net/1822/5534 |
Resumo: | The activity of supported Ni-Cu alloy catalysts in the gasification of carbon was studied for a range of copper concentrations. Deposits formed from the decomposition of methane under constant and well-defined conditions were gasified by hydrogen and hydrogen-steam mixtures. The kinetics of hydrogasification were determined under such conditions that the reaction rates did not depend on the extent of carbon burn-off. Comparison of the different catalysts indicates that, similarly to previous results for the decomposition, an ensemble of surface nickel atoms plays a role in the gasification. |
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Gasification of carbon deposited on supported Ni-Cu catalystsGasification of carbonCatalystSurface depositionScience & TechnologyThe activity of supported Ni-Cu alloy catalysts in the gasification of carbon was studied for a range of copper concentrations. Deposits formed from the decomposition of methane under constant and well-defined conditions were gasified by hydrogen and hydrogen-steam mixtures. The kinetics of hydrogasification were determined under such conditions that the reaction rates did not depend on the extent of carbon burn-off. Comparison of the different catalysts indicates that, similarly to previous results for the decomposition, an ensemble of surface nickel atoms plays a role in the gasification.North Atlantic Treaty Organization (NATO) - Research Grant.ElsevierUniversidade do MinhoTavares, M. T.Bernardo, C. A.Figueiredo, J. L.1986-101986-10-01T00:00:00Zinfo:eu-repo/semantics/publishedVersioninfo:eu-repo/semantics/articleapplication/pdfhttp://hdl.handle.net/1822/5534eng"Fuel". ISSN 0016-2361. 65:10 (1986) 1392-1395.0016-236110.1016/0016-2361(86)90111-0http://www.elsevier.com/wps/find/journaldescription.cws_home/30420/description#descriptioninfo:eu-repo/semantics/openAccessreponame:Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos)instname:Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informaçãoinstacron:RCAAP2023-07-21T12:27:29Zoai:repositorium.sdum.uminho.pt:1822/5534Portal AgregadorONGhttps://www.rcaap.pt/oai/openaireopendoar:71602024-03-19T19:22:05.197728Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) - Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informaçãofalse |
dc.title.none.fl_str_mv |
Gasification of carbon deposited on supported Ni-Cu catalysts |
title |
Gasification of carbon deposited on supported Ni-Cu catalysts |
spellingShingle |
Gasification of carbon deposited on supported Ni-Cu catalysts Tavares, M. T. Gasification of carbon Catalyst Surface deposition Science & Technology |
title_short |
Gasification of carbon deposited on supported Ni-Cu catalysts |
title_full |
Gasification of carbon deposited on supported Ni-Cu catalysts |
title_fullStr |
Gasification of carbon deposited on supported Ni-Cu catalysts |
title_full_unstemmed |
Gasification of carbon deposited on supported Ni-Cu catalysts |
title_sort |
Gasification of carbon deposited on supported Ni-Cu catalysts |
author |
Tavares, M. T. |
author_facet |
Tavares, M. T. Bernardo, C. A. Figueiredo, J. L. |
author_role |
author |
author2 |
Bernardo, C. A. Figueiredo, J. L. |
author2_role |
author author |
dc.contributor.none.fl_str_mv |
Universidade do Minho |
dc.contributor.author.fl_str_mv |
Tavares, M. T. Bernardo, C. A. Figueiredo, J. L. |
dc.subject.por.fl_str_mv |
Gasification of carbon Catalyst Surface deposition Science & Technology |
topic |
Gasification of carbon Catalyst Surface deposition Science & Technology |
description |
The activity of supported Ni-Cu alloy catalysts in the gasification of carbon was studied for a range of copper concentrations. Deposits formed from the decomposition of methane under constant and well-defined conditions were gasified by hydrogen and hydrogen-steam mixtures. The kinetics of hydrogasification were determined under such conditions that the reaction rates did not depend on the extent of carbon burn-off. Comparison of the different catalysts indicates that, similarly to previous results for the decomposition, an ensemble of surface nickel atoms plays a role in the gasification. |
publishDate |
1986 |
dc.date.none.fl_str_mv |
1986-10 1986-10-01T00:00:00Z |
dc.type.status.fl_str_mv |
info:eu-repo/semantics/publishedVersion |
dc.type.driver.fl_str_mv |
info:eu-repo/semantics/article |
format |
article |
status_str |
publishedVersion |
dc.identifier.uri.fl_str_mv |
http://hdl.handle.net/1822/5534 |
url |
http://hdl.handle.net/1822/5534 |
dc.language.iso.fl_str_mv |
eng |
language |
eng |
dc.relation.none.fl_str_mv |
"Fuel". ISSN 0016-2361. 65:10 (1986) 1392-1395. 0016-2361 10.1016/0016-2361(86)90111-0 http://www.elsevier.com/wps/find/journaldescription.cws_home/30420/description#description |
dc.rights.driver.fl_str_mv |
info:eu-repo/semantics/openAccess |
eu_rights_str_mv |
openAccess |
dc.format.none.fl_str_mv |
application/pdf |
dc.publisher.none.fl_str_mv |
Elsevier |
publisher.none.fl_str_mv |
Elsevier |
dc.source.none.fl_str_mv |
reponame:Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) instname:Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informação instacron:RCAAP |
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Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informação |
instacron_str |
RCAAP |
institution |
RCAAP |
reponame_str |
Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) |
collection |
Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) |
repository.name.fl_str_mv |
Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) - Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informação |
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1799132689990680576 |