Four metal-organic frameworks for the sensing of oxytetracycline/nitrofurazone and Fe3+ ions
Autor(a) principal: | |
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Data de Publicação: | 2023 |
Outros Autores: | , , |
Tipo de documento: | Artigo |
Idioma: | eng |
Título da fonte: | Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) |
Texto Completo: | http://hdl.handle.net/10773/37902 |
Resumo: | Four new d10 metal-organic frameworks (MOFs), named {[Cd(L)(TPA)]}n (1), {[Zn3(L)(BTC)2]}n (2), {[Zn(L)(1,4-NDC)]·2H2O}n (3), and {[Cd(L)(1,4-NDC)]·1.5H2O}n (4) (L = 1,6-bis(1-(pyridine-4-ylmethyl)-1H-benzo[d]imidazole-2-yl)hexane, H2TPA = terephthalic acid, H3BTC = 1,3,5-benzenetricarboxylic acid, 1,4-H2NDC = 1,4-naphthalene dicarboxylic acid), are successfully synthesized by hydrothermal method and further characterized. 1 can be simplified into a dia framework, an unusual 4-nodal 3,4,4,6-topology of 2 was deposited into the TopCryst database as cgh8, 3–4 are simplified to 2D sql networks. 1–4 exhibit chemical stability, which are stable in a wide pH range from 3 to 12. The sensing of the oxytetracycline/nitrofurazone and Fe3+ ions display the selectivity, sensitivity, and reusability of 1‒4. Moreover, the mechanism of luminescence quenching is also investigated as photo-induced electron transfer and Förster resonance energy transfer. |
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Four metal-organic frameworks for the sensing of oxytetracycline/nitrofurazone and Fe3+ ionsBis(benzimidazole) derivativeDensity functional theoryLuminescence quenchingMetal-organic frameworkOxytetracyclineFour new d10 metal-organic frameworks (MOFs), named {[Cd(L)(TPA)]}n (1), {[Zn3(L)(BTC)2]}n (2), {[Zn(L)(1,4-NDC)]·2H2O}n (3), and {[Cd(L)(1,4-NDC)]·1.5H2O}n (4) (L = 1,6-bis(1-(pyridine-4-ylmethyl)-1H-benzo[d]imidazole-2-yl)hexane, H2TPA = terephthalic acid, H3BTC = 1,3,5-benzenetricarboxylic acid, 1,4-H2NDC = 1,4-naphthalene dicarboxylic acid), are successfully synthesized by hydrothermal method and further characterized. 1 can be simplified into a dia framework, an unusual 4-nodal 3,4,4,6-topology of 2 was deposited into the TopCryst database as cgh8, 3–4 are simplified to 2D sql networks. 1–4 exhibit chemical stability, which are stable in a wide pH range from 3 to 12. The sensing of the oxytetracycline/nitrofurazone and Fe3+ ions display the selectivity, sensitivity, and reusability of 1‒4. Moreover, the mechanism of luminescence quenching is also investigated as photo-induced electron transfer and Förster resonance energy transfer.Elsevier2023-082023-08-01T00:00:00Z2025-08-31T00:00:00Zinfo:eu-repo/semantics/publishedVersioninfo:eu-repo/semantics/articleapplication/pdfhttp://hdl.handle.net/10773/37902eng0022-459610.1016/j.jssc.2023.124124Zhang, Xu-PengFu, LiansheBlatova, Olga A.Cui, Guang-Huainfo:eu-repo/semantics/embargoedAccessreponame:Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos)instname:Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informaçãoinstacron:RCAAP2024-02-22T12:14:00Zoai:ria.ua.pt:10773/37902Portal AgregadorONGhttps://www.rcaap.pt/oai/openaireopendoar:71602024-03-20T03:08:27.172702Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) - Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informaçãofalse |
dc.title.none.fl_str_mv |
Four metal-organic frameworks for the sensing of oxytetracycline/nitrofurazone and Fe3+ ions |
title |
Four metal-organic frameworks for the sensing of oxytetracycline/nitrofurazone and Fe3+ ions |
spellingShingle |
Four metal-organic frameworks for the sensing of oxytetracycline/nitrofurazone and Fe3+ ions Zhang, Xu-Peng Bis(benzimidazole) derivative Density functional theory Luminescence quenching Metal-organic framework Oxytetracycline |
title_short |
Four metal-organic frameworks for the sensing of oxytetracycline/nitrofurazone and Fe3+ ions |
title_full |
Four metal-organic frameworks for the sensing of oxytetracycline/nitrofurazone and Fe3+ ions |
title_fullStr |
Four metal-organic frameworks for the sensing of oxytetracycline/nitrofurazone and Fe3+ ions |
title_full_unstemmed |
Four metal-organic frameworks for the sensing of oxytetracycline/nitrofurazone and Fe3+ ions |
title_sort |
Four metal-organic frameworks for the sensing of oxytetracycline/nitrofurazone and Fe3+ ions |
author |
Zhang, Xu-Peng |
author_facet |
Zhang, Xu-Peng Fu, Lianshe Blatova, Olga A. Cui, Guang-Hua |
author_role |
author |
author2 |
Fu, Lianshe Blatova, Olga A. Cui, Guang-Hua |
author2_role |
author author author |
dc.contributor.author.fl_str_mv |
Zhang, Xu-Peng Fu, Lianshe Blatova, Olga A. Cui, Guang-Hua |
dc.subject.por.fl_str_mv |
Bis(benzimidazole) derivative Density functional theory Luminescence quenching Metal-organic framework Oxytetracycline |
topic |
Bis(benzimidazole) derivative Density functional theory Luminescence quenching Metal-organic framework Oxytetracycline |
description |
Four new d10 metal-organic frameworks (MOFs), named {[Cd(L)(TPA)]}n (1), {[Zn3(L)(BTC)2]}n (2), {[Zn(L)(1,4-NDC)]·2H2O}n (3), and {[Cd(L)(1,4-NDC)]·1.5H2O}n (4) (L = 1,6-bis(1-(pyridine-4-ylmethyl)-1H-benzo[d]imidazole-2-yl)hexane, H2TPA = terephthalic acid, H3BTC = 1,3,5-benzenetricarboxylic acid, 1,4-H2NDC = 1,4-naphthalene dicarboxylic acid), are successfully synthesized by hydrothermal method and further characterized. 1 can be simplified into a dia framework, an unusual 4-nodal 3,4,4,6-topology of 2 was deposited into the TopCryst database as cgh8, 3–4 are simplified to 2D sql networks. 1–4 exhibit chemical stability, which are stable in a wide pH range from 3 to 12. The sensing of the oxytetracycline/nitrofurazone and Fe3+ ions display the selectivity, sensitivity, and reusability of 1‒4. Moreover, the mechanism of luminescence quenching is also investigated as photo-induced electron transfer and Förster resonance energy transfer. |
publishDate |
2023 |
dc.date.none.fl_str_mv |
2023-08 2023-08-01T00:00:00Z 2025-08-31T00:00:00Z |
dc.type.status.fl_str_mv |
info:eu-repo/semantics/publishedVersion |
dc.type.driver.fl_str_mv |
info:eu-repo/semantics/article |
format |
article |
status_str |
publishedVersion |
dc.identifier.uri.fl_str_mv |
http://hdl.handle.net/10773/37902 |
url |
http://hdl.handle.net/10773/37902 |
dc.language.iso.fl_str_mv |
eng |
language |
eng |
dc.relation.none.fl_str_mv |
0022-4596 10.1016/j.jssc.2023.124124 |
dc.rights.driver.fl_str_mv |
info:eu-repo/semantics/embargoedAccess |
eu_rights_str_mv |
embargoedAccess |
dc.format.none.fl_str_mv |
application/pdf |
dc.publisher.none.fl_str_mv |
Elsevier |
publisher.none.fl_str_mv |
Elsevier |
dc.source.none.fl_str_mv |
reponame:Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) instname:Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informação instacron:RCAAP |
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Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informação |
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RCAAP |
institution |
RCAAP |
reponame_str |
Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) |
collection |
Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) |
repository.name.fl_str_mv |
Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) - Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informação |
repository.mail.fl_str_mv |
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1799137737097347072 |