Photocatalytic performance of textiles coated with titanium dioxide-reduced graphene oxide system for degradation of crude petroleum under similar solar irradiation
Autor(a) principal: | |
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Data de Publicação: | 2022 |
Outros Autores: | , , , , , , , |
Tipo de documento: | Artigo |
Idioma: | eng |
Título da fonte: | Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) |
Texto Completo: | https://hdl.handle.net/1822/82649 |
Resumo: | The pollution caused by oil and its toxic derivatives presents a considerable risk to the public health and the environment. This work is devoted to the study of the influence of TiO2 nanoparticles immobilized on three types of textiles materials (Cotton, Entretela, and Polylactic Acid-PLA) coated with reduced graphene oxide (RGO) to be used for degradation of crude petroleum under simulated solar irradiation. The morphological studies of the functionalized textiles substrates were performed by using Scanning Electron Microscopy and Energy Dispersive X-ray Spectroscopy, which indicated an excellent dispersion and adhesion of nanoparticles of about 60% (atomic %Ti) on the textile fibers covered with RGO after washing. Ultraviolet-visible Diffuse Reflectance spectra suggest a reduction in the band gap energy of TiO2 up to 2.86 eV due to the presence of RGO. The functionalized textiles presented at least 60% of photocatalytic efficiency measured by Rhodamine B degradation, decreasing less than 12% after the rigorous washing. The excitation/emission Synchronous Fluorescence Spectroscopy and Fourier-transform Infrared spectroscopies demonstrated a great potential for photocatalytic degradation of the functionalized textiles substrates as the appearance of the hydroxyl, carboxyl, and the C-O bands confirm the photoinduced oxidation of the organic compounds implying with high prospects in petroleum and wastewater treatment areas. Moreover, this environmentally friendly, sustainable, and inclusive research work can be included in clean technologies, contributing to the novel socio-economic model recognized as "Green Recovery".[GRAPHICS]. |
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Photocatalytic performance of textiles coated with titanium dioxide-reduced graphene oxide system for degradation of crude petroleum under similar solar irradiationScience & TechnologyThe pollution caused by oil and its toxic derivatives presents a considerable risk to the public health and the environment. This work is devoted to the study of the influence of TiO2 nanoparticles immobilized on three types of textiles materials (Cotton, Entretela, and Polylactic Acid-PLA) coated with reduced graphene oxide (RGO) to be used for degradation of crude petroleum under simulated solar irradiation. The morphological studies of the functionalized textiles substrates were performed by using Scanning Electron Microscopy and Energy Dispersive X-ray Spectroscopy, which indicated an excellent dispersion and adhesion of nanoparticles of about 60% (atomic %Ti) on the textile fibers covered with RGO after washing. Ultraviolet-visible Diffuse Reflectance spectra suggest a reduction in the band gap energy of TiO2 up to 2.86 eV due to the presence of RGO. The functionalized textiles presented at least 60% of photocatalytic efficiency measured by Rhodamine B degradation, decreasing less than 12% after the rigorous washing. The excitation/emission Synchronous Fluorescence Spectroscopy and Fourier-transform Infrared spectroscopies demonstrated a great potential for photocatalytic degradation of the functionalized textiles substrates as the appearance of the hydroxyl, carboxyl, and the C-O bands confirm the photoinduced oxidation of the organic compounds implying with high prospects in petroleum and wastewater treatment areas. Moreover, this environmentally friendly, sustainable, and inclusive research work can be included in clean technologies, contributing to the novel socio-economic model recognized as "Green Recovery".[GRAPHICS].This work was supported by the Portuguese Foundation for Science and Technology (FCT) in the framework of the Strategic Funding UID/FIS/04650/2019 and the project PTDC/FIS-MAC/6606/2020. Also, the third author would like to acknowledge the FCT for the Ph.D. scholarship (SFRH/BD/137421/2018). Moreover, the authors would like to acknowledge Sociedade Nacional de Combusti ' veis de Angola (Sonangol), which partially provided the crude oil samples.SpringerUniversidade do MinhoSilva, DavideLandi Jr, SalmonSegundo, Iran RochaAfonso, CatiaFernandes, FilipaNunes, Eloiza da SilvaTeixeira, VascoMoreto, Jeferson AparecidoCarneiro, Joaquim A. O.2022-02-052022-02-05T00:00:00Zinfo:eu-repo/semantics/publishedVersioninfo:eu-repo/semantics/articleapplication/pdfhttps://hdl.handle.net/1822/82649engSilva, D., Landi, S., Rocha Segundo, I. et al. Photocatalytic performance of textiles coated with titanium dioxide-reduced graphene oxide system for degradation of crude petroleum under similar solar irradiation. J Mater Sci 57, 8464–8480 (2022). https://doi.org/10.1007/s10853-021-06849-30022-246110.1007/s10853-021-06849-3https://link.springer.com/article/10.1007/s10853-021-06849-3info:eu-repo/semantics/openAccessreponame:Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos)instname:Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informaçãoinstacron:RCAAP2023-07-21T12:26:07Zoai:repositorium.sdum.uminho.pt:1822/82649Portal AgregadorONGhttps://www.rcaap.pt/oai/openaireopendoar:71602024-03-19T19:20:27.604442Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) - Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informaçãofalse |
dc.title.none.fl_str_mv |
Photocatalytic performance of textiles coated with titanium dioxide-reduced graphene oxide system for degradation of crude petroleum under similar solar irradiation |
title |
Photocatalytic performance of textiles coated with titanium dioxide-reduced graphene oxide system for degradation of crude petroleum under similar solar irradiation |
spellingShingle |
Photocatalytic performance of textiles coated with titanium dioxide-reduced graphene oxide system for degradation of crude petroleum under similar solar irradiation Silva, Davide Science & Technology |
title_short |
Photocatalytic performance of textiles coated with titanium dioxide-reduced graphene oxide system for degradation of crude petroleum under similar solar irradiation |
title_full |
Photocatalytic performance of textiles coated with titanium dioxide-reduced graphene oxide system for degradation of crude petroleum under similar solar irradiation |
title_fullStr |
Photocatalytic performance of textiles coated with titanium dioxide-reduced graphene oxide system for degradation of crude petroleum under similar solar irradiation |
title_full_unstemmed |
Photocatalytic performance of textiles coated with titanium dioxide-reduced graphene oxide system for degradation of crude petroleum under similar solar irradiation |
title_sort |
Photocatalytic performance of textiles coated with titanium dioxide-reduced graphene oxide system for degradation of crude petroleum under similar solar irradiation |
author |
Silva, Davide |
author_facet |
Silva, Davide Landi Jr, Salmon Segundo, Iran Rocha Afonso, Catia Fernandes, Filipa Nunes, Eloiza da Silva Teixeira, Vasco Moreto, Jeferson Aparecido Carneiro, Joaquim A. O. |
author_role |
author |
author2 |
Landi Jr, Salmon Segundo, Iran Rocha Afonso, Catia Fernandes, Filipa Nunes, Eloiza da Silva Teixeira, Vasco Moreto, Jeferson Aparecido Carneiro, Joaquim A. O. |
author2_role |
author author author author author author author author |
dc.contributor.none.fl_str_mv |
Universidade do Minho |
dc.contributor.author.fl_str_mv |
Silva, Davide Landi Jr, Salmon Segundo, Iran Rocha Afonso, Catia Fernandes, Filipa Nunes, Eloiza da Silva Teixeira, Vasco Moreto, Jeferson Aparecido Carneiro, Joaquim A. O. |
dc.subject.por.fl_str_mv |
Science & Technology |
topic |
Science & Technology |
description |
The pollution caused by oil and its toxic derivatives presents a considerable risk to the public health and the environment. This work is devoted to the study of the influence of TiO2 nanoparticles immobilized on three types of textiles materials (Cotton, Entretela, and Polylactic Acid-PLA) coated with reduced graphene oxide (RGO) to be used for degradation of crude petroleum under simulated solar irradiation. The morphological studies of the functionalized textiles substrates were performed by using Scanning Electron Microscopy and Energy Dispersive X-ray Spectroscopy, which indicated an excellent dispersion and adhesion of nanoparticles of about 60% (atomic %Ti) on the textile fibers covered with RGO after washing. Ultraviolet-visible Diffuse Reflectance spectra suggest a reduction in the band gap energy of TiO2 up to 2.86 eV due to the presence of RGO. The functionalized textiles presented at least 60% of photocatalytic efficiency measured by Rhodamine B degradation, decreasing less than 12% after the rigorous washing. The excitation/emission Synchronous Fluorescence Spectroscopy and Fourier-transform Infrared spectroscopies demonstrated a great potential for photocatalytic degradation of the functionalized textiles substrates as the appearance of the hydroxyl, carboxyl, and the C-O bands confirm the photoinduced oxidation of the organic compounds implying with high prospects in petroleum and wastewater treatment areas. Moreover, this environmentally friendly, sustainable, and inclusive research work can be included in clean technologies, contributing to the novel socio-economic model recognized as "Green Recovery".[GRAPHICS]. |
publishDate |
2022 |
dc.date.none.fl_str_mv |
2022-02-05 2022-02-05T00:00:00Z |
dc.type.status.fl_str_mv |
info:eu-repo/semantics/publishedVersion |
dc.type.driver.fl_str_mv |
info:eu-repo/semantics/article |
format |
article |
status_str |
publishedVersion |
dc.identifier.uri.fl_str_mv |
https://hdl.handle.net/1822/82649 |
url |
https://hdl.handle.net/1822/82649 |
dc.language.iso.fl_str_mv |
eng |
language |
eng |
dc.relation.none.fl_str_mv |
Silva, D., Landi, S., Rocha Segundo, I. et al. Photocatalytic performance of textiles coated with titanium dioxide-reduced graphene oxide system for degradation of crude petroleum under similar solar irradiation. J Mater Sci 57, 8464–8480 (2022). https://doi.org/10.1007/s10853-021-06849-3 0022-2461 10.1007/s10853-021-06849-3 https://link.springer.com/article/10.1007/s10853-021-06849-3 |
dc.rights.driver.fl_str_mv |
info:eu-repo/semantics/openAccess |
eu_rights_str_mv |
openAccess |
dc.format.none.fl_str_mv |
application/pdf |
dc.publisher.none.fl_str_mv |
Springer |
publisher.none.fl_str_mv |
Springer |
dc.source.none.fl_str_mv |
reponame:Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) instname:Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informação instacron:RCAAP |
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Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informação |
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RCAAP |
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Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) |
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Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) |
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Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) - Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informação |
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