Operational properties of fine powder aerosol as radiation detection medium in gaseous proportional counters

Detalhes bibliográficos
Autor(a) principal: Duarte, N.F.V.
Data de Publicação: 2019
Outros Autores: Monteiro, C.M.B., Azevedo, C.D.R., Antognini, A., Amaro, F.D.
Tipo de documento: Artigo
Idioma: eng
Título da fonte: Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos)
Texto Completo: http://hdl.handle.net/10773/37447
Resumo: Due to its exceptional properties, 3He proportional counters are the golden standard for neutron detection, particularly in homeland security applications where large area detectors are deployed. However, in recent years 3He has become severely scarce, which led to a tremendous price increase and acquisition restrictions of this material. Motivated by this, the development of 3He-free solutions became a priority. In a previous work, we have established a novel concept for neutron detection: a proportional counter with boron carbide (B4C) fine powder suspended in the proportional gas, forming a neutron sensitive aerosol that relies on the 10B neutron capture reaction. Computer simulations and prototype exposure to a cold neutron beam yielded favorable results, validating the detection concept, which may also be applied to hard x-ray and gamma ray detection by using fine particles made of a heavy element, such as Bi or Au. In this work we study the effect of the presence of B4C microparticles in the charge gain and energy resolution of a proportional counter filled with Ar-CH4 (90%–10%), by irradiation with x-rays from a 55Fe source. For the same applied voltage, an average gain loss by a factor of 36% and energy resolution (FWHM) increase by 15% (absolute value) was observed with the inclusion of B4C microparticles. Intrinsic energy resolution was calculated, obtaining 15% for pure P10 operation and 32% in the presence of the microparticles. While the gain drop is recoverable by increasing anode voltage, energy resolution degradation may be a drawback in low energy applications, were energy resolution is favored over detection efficiency.
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spelling Operational properties of fine powder aerosol as radiation detection medium in gaseous proportional countersProportional counterNeutron detectionGamma ray detection10BHe alternativeDue to its exceptional properties, 3He proportional counters are the golden standard for neutron detection, particularly in homeland security applications where large area detectors are deployed. However, in recent years 3He has become severely scarce, which led to a tremendous price increase and acquisition restrictions of this material. Motivated by this, the development of 3He-free solutions became a priority. In a previous work, we have established a novel concept for neutron detection: a proportional counter with boron carbide (B4C) fine powder suspended in the proportional gas, forming a neutron sensitive aerosol that relies on the 10B neutron capture reaction. Computer simulations and prototype exposure to a cold neutron beam yielded favorable results, validating the detection concept, which may also be applied to hard x-ray and gamma ray detection by using fine particles made of a heavy element, such as Bi or Au. In this work we study the effect of the presence of B4C microparticles in the charge gain and energy resolution of a proportional counter filled with Ar-CH4 (90%–10%), by irradiation with x-rays from a 55Fe source. For the same applied voltage, an average gain loss by a factor of 36% and energy resolution (FWHM) increase by 15% (absolute value) was observed with the inclusion of B4C microparticles. Intrinsic energy resolution was calculated, obtaining 15% for pure P10 operation and 32% in the presence of the microparticles. While the gain drop is recoverable by increasing anode voltage, energy resolution degradation may be a drawback in low energy applications, were energy resolution is favored over detection efficiency.Elsevier2023-04-28T10:51:42Z2019-10-21T00:00:00Z2019-10-21info:eu-repo/semantics/publishedVersioninfo:eu-repo/semantics/articleapplication/pdfhttp://hdl.handle.net/10773/37447eng0168-900210.1016/j.nima.2019.162392Duarte, N.F.V.Monteiro, C.M.B.Azevedo, C.D.R.Antognini, A.Amaro, F.D.info:eu-repo/semantics/openAccessreponame:Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos)instname:Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informaçãoinstacron:RCAAP2024-02-22T12:12:19Zoai:ria.ua.pt:10773/37447Portal AgregadorONGhttps://www.rcaap.pt/oai/openaireopendoar:71602024-03-20T03:08:03.588423Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) - Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informaçãofalse
dc.title.none.fl_str_mv Operational properties of fine powder aerosol as radiation detection medium in gaseous proportional counters
title Operational properties of fine powder aerosol as radiation detection medium in gaseous proportional counters
spellingShingle Operational properties of fine powder aerosol as radiation detection medium in gaseous proportional counters
Duarte, N.F.V.
Proportional counter
Neutron detection
Gamma ray detection
10B
He alternative
title_short Operational properties of fine powder aerosol as radiation detection medium in gaseous proportional counters
title_full Operational properties of fine powder aerosol as radiation detection medium in gaseous proportional counters
title_fullStr Operational properties of fine powder aerosol as radiation detection medium in gaseous proportional counters
title_full_unstemmed Operational properties of fine powder aerosol as radiation detection medium in gaseous proportional counters
title_sort Operational properties of fine powder aerosol as radiation detection medium in gaseous proportional counters
author Duarte, N.F.V.
author_facet Duarte, N.F.V.
Monteiro, C.M.B.
Azevedo, C.D.R.
Antognini, A.
Amaro, F.D.
author_role author
author2 Monteiro, C.M.B.
Azevedo, C.D.R.
Antognini, A.
Amaro, F.D.
author2_role author
author
author
author
dc.contributor.author.fl_str_mv Duarte, N.F.V.
Monteiro, C.M.B.
Azevedo, C.D.R.
Antognini, A.
Amaro, F.D.
dc.subject.por.fl_str_mv Proportional counter
Neutron detection
Gamma ray detection
10B
He alternative
topic Proportional counter
Neutron detection
Gamma ray detection
10B
He alternative
description Due to its exceptional properties, 3He proportional counters are the golden standard for neutron detection, particularly in homeland security applications where large area detectors are deployed. However, in recent years 3He has become severely scarce, which led to a tremendous price increase and acquisition restrictions of this material. Motivated by this, the development of 3He-free solutions became a priority. In a previous work, we have established a novel concept for neutron detection: a proportional counter with boron carbide (B4C) fine powder suspended in the proportional gas, forming a neutron sensitive aerosol that relies on the 10B neutron capture reaction. Computer simulations and prototype exposure to a cold neutron beam yielded favorable results, validating the detection concept, which may also be applied to hard x-ray and gamma ray detection by using fine particles made of a heavy element, such as Bi or Au. In this work we study the effect of the presence of B4C microparticles in the charge gain and energy resolution of a proportional counter filled with Ar-CH4 (90%–10%), by irradiation with x-rays from a 55Fe source. For the same applied voltage, an average gain loss by a factor of 36% and energy resolution (FWHM) increase by 15% (absolute value) was observed with the inclusion of B4C microparticles. Intrinsic energy resolution was calculated, obtaining 15% for pure P10 operation and 32% in the presence of the microparticles. While the gain drop is recoverable by increasing anode voltage, energy resolution degradation may be a drawback in low energy applications, were energy resolution is favored over detection efficiency.
publishDate 2019
dc.date.none.fl_str_mv 2019-10-21T00:00:00Z
2019-10-21
2023-04-28T10:51:42Z
dc.type.status.fl_str_mv info:eu-repo/semantics/publishedVersion
dc.type.driver.fl_str_mv info:eu-repo/semantics/article
format article
status_str publishedVersion
dc.identifier.uri.fl_str_mv http://hdl.handle.net/10773/37447
url http://hdl.handle.net/10773/37447
dc.language.iso.fl_str_mv eng
language eng
dc.relation.none.fl_str_mv 0168-9002
10.1016/j.nima.2019.162392
dc.rights.driver.fl_str_mv info:eu-repo/semantics/openAccess
eu_rights_str_mv openAccess
dc.format.none.fl_str_mv application/pdf
dc.publisher.none.fl_str_mv Elsevier
publisher.none.fl_str_mv Elsevier
dc.source.none.fl_str_mv reponame:Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos)
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