Surface modification of ZnO quantum dots coated polylactic acid knitted fabric for photocatalytic application
Autor(a) principal: | |
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Data de Publicação: | 2022 |
Outros Autores: | , , , , , , , |
Tipo de documento: | Artigo |
Idioma: | eng |
Título da fonte: | Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) |
Texto Completo: | https://hdl.handle.net/1822/76686 |
Resumo: | In this work, ZnO quantum dots (ZnOQD) were synthesized by Sol–gel synthe- sis and impregnated on polylactic acid (PLA) knitted fabric through self- assembly of different cycles from layer-by-layer (LBL) using cationic agent Poly(diallydimethylammonium chloride) (PDDA). Then, morphological, chemi- cal and photocatalytic properties were studied. The results demonstrate that the synthesis provided 8 nm Wurtzite-type ZnO nanoparticles. In addition, X-ray photoelectron spectroscopy (XPS) spectra, X-ray diffraction (XRD) and scanning electron microscopy (SEM) proved the inclusion of ZnOQD on the surface of PLA matrix, which allowed the evaluation of its photocatalytic properties, there- fore, coated PLA with five cycles of ZnOQD obtained the best result for degrading 85% of the dye Rhodamine B (RhB) in 360 min under UV radiation, in addition to its reusability for another five cycles of photocatalytic activity. |
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Surface modification of ZnO quantum dots coated polylactic acid knitted fabric for photocatalytic applicationLayer-by-layerNanoparticlesPhotocatalytic,Polylactic acidQuantum dotsZnOTextileEngenharia e Tecnologia::Engenharia dos MateriaisScience & TechnologyIn this work, ZnO quantum dots (ZnOQD) were synthesized by Sol–gel synthe- sis and impregnated on polylactic acid (PLA) knitted fabric through self- assembly of different cycles from layer-by-layer (LBL) using cationic agent Poly(diallydimethylammonium chloride) (PDDA). Then, morphological, chemi- cal and photocatalytic properties were studied. The results demonstrate that the synthesis provided 8 nm Wurtzite-type ZnO nanoparticles. In addition, X-ray photoelectron spectroscopy (XPS) spectra, X-ray diffraction (XRD) and scanning electron microscopy (SEM) proved the inclusion of ZnOQD on the surface of PLA matrix, which allowed the evaluation of its photocatalytic properties, there- fore, coated PLA with five cycles of ZnOQD obtained the best result for degrading 85% of the dye Rhodamine B (RhB) in 360 min under UV radiation, in addition to its reusability for another five cycles of photocatalytic activity.Coordenacao de Aperfeicoamento de Pessoal de Nivel Superior (CAPES); Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq)WileyUniversidade do MinhoCabral, Rivaldo Leonn BezerraGalvão, Felipe Mendonça FontesSouto Silva, Kesia Karina OliveiraFelipe, Brenno Henrique SilvaAndrade Neto, Nivaldo FreireAlmeida Fechine, Pierre BasílioZille, AndreaKim, SuyeonNascimento, José Heriberto Oliveira20222022-01-01T00:00:00Zinfo:eu-repo/semantics/publishedVersioninfo:eu-repo/semantics/articleapplication/pdfhttps://hdl.handle.net/1822/76686eng0021-89951097-462810.1002/app.52381https://onlinelibrary.wiley.com/doi/10.1002/app.52381info:eu-repo/semantics/openAccessreponame:Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos)instname:Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informaçãoinstacron:RCAAP2023-07-21T12:21:32Zoai:repositorium.sdum.uminho.pt:1822/76686Portal AgregadorONGhttps://www.rcaap.pt/oai/openaireopendoar:71602024-03-19T19:14:49.246339Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) - Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informaçãofalse |
dc.title.none.fl_str_mv |
Surface modification of ZnO quantum dots coated polylactic acid knitted fabric for photocatalytic application |
title |
Surface modification of ZnO quantum dots coated polylactic acid knitted fabric for photocatalytic application |
spellingShingle |
Surface modification of ZnO quantum dots coated polylactic acid knitted fabric for photocatalytic application Cabral, Rivaldo Leonn Bezerra Layer-by-layer Nanoparticles Photocatalytic, Polylactic acid Quantum dots ZnO Textile Engenharia e Tecnologia::Engenharia dos Materiais Science & Technology |
title_short |
Surface modification of ZnO quantum dots coated polylactic acid knitted fabric for photocatalytic application |
title_full |
Surface modification of ZnO quantum dots coated polylactic acid knitted fabric for photocatalytic application |
title_fullStr |
Surface modification of ZnO quantum dots coated polylactic acid knitted fabric for photocatalytic application |
title_full_unstemmed |
Surface modification of ZnO quantum dots coated polylactic acid knitted fabric for photocatalytic application |
title_sort |
Surface modification of ZnO quantum dots coated polylactic acid knitted fabric for photocatalytic application |
author |
Cabral, Rivaldo Leonn Bezerra |
author_facet |
Cabral, Rivaldo Leonn Bezerra Galvão, Felipe Mendonça Fontes Souto Silva, Kesia Karina Oliveira Felipe, Brenno Henrique Silva Andrade Neto, Nivaldo Freire Almeida Fechine, Pierre Basílio Zille, Andrea Kim, Suyeon Nascimento, José Heriberto Oliveira |
author_role |
author |
author2 |
Galvão, Felipe Mendonça Fontes Souto Silva, Kesia Karina Oliveira Felipe, Brenno Henrique Silva Andrade Neto, Nivaldo Freire Almeida Fechine, Pierre Basílio Zille, Andrea Kim, Suyeon Nascimento, José Heriberto Oliveira |
author2_role |
author author author author author author author author |
dc.contributor.none.fl_str_mv |
Universidade do Minho |
dc.contributor.author.fl_str_mv |
Cabral, Rivaldo Leonn Bezerra Galvão, Felipe Mendonça Fontes Souto Silva, Kesia Karina Oliveira Felipe, Brenno Henrique Silva Andrade Neto, Nivaldo Freire Almeida Fechine, Pierre Basílio Zille, Andrea Kim, Suyeon Nascimento, José Heriberto Oliveira |
dc.subject.por.fl_str_mv |
Layer-by-layer Nanoparticles Photocatalytic, Polylactic acid Quantum dots ZnO Textile Engenharia e Tecnologia::Engenharia dos Materiais Science & Technology |
topic |
Layer-by-layer Nanoparticles Photocatalytic, Polylactic acid Quantum dots ZnO Textile Engenharia e Tecnologia::Engenharia dos Materiais Science & Technology |
description |
In this work, ZnO quantum dots (ZnOQD) were synthesized by Sol–gel synthe- sis and impregnated on polylactic acid (PLA) knitted fabric through self- assembly of different cycles from layer-by-layer (LBL) using cationic agent Poly(diallydimethylammonium chloride) (PDDA). Then, morphological, chemi- cal and photocatalytic properties were studied. The results demonstrate that the synthesis provided 8 nm Wurtzite-type ZnO nanoparticles. In addition, X-ray photoelectron spectroscopy (XPS) spectra, X-ray diffraction (XRD) and scanning electron microscopy (SEM) proved the inclusion of ZnOQD on the surface of PLA matrix, which allowed the evaluation of its photocatalytic properties, there- fore, coated PLA with five cycles of ZnOQD obtained the best result for degrading 85% of the dye Rhodamine B (RhB) in 360 min under UV radiation, in addition to its reusability for another five cycles of photocatalytic activity. |
publishDate |
2022 |
dc.date.none.fl_str_mv |
2022 2022-01-01T00:00:00Z |
dc.type.status.fl_str_mv |
info:eu-repo/semantics/publishedVersion |
dc.type.driver.fl_str_mv |
info:eu-repo/semantics/article |
format |
article |
status_str |
publishedVersion |
dc.identifier.uri.fl_str_mv |
https://hdl.handle.net/1822/76686 |
url |
https://hdl.handle.net/1822/76686 |
dc.language.iso.fl_str_mv |
eng |
language |
eng |
dc.relation.none.fl_str_mv |
0021-8995 1097-4628 10.1002/app.52381 https://onlinelibrary.wiley.com/doi/10.1002/app.52381 |
dc.rights.driver.fl_str_mv |
info:eu-repo/semantics/openAccess |
eu_rights_str_mv |
openAccess |
dc.format.none.fl_str_mv |
application/pdf |
dc.publisher.none.fl_str_mv |
Wiley |
publisher.none.fl_str_mv |
Wiley |
dc.source.none.fl_str_mv |
reponame:Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) instname:Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informação instacron:RCAAP |
instname_str |
Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informação |
instacron_str |
RCAAP |
institution |
RCAAP |
reponame_str |
Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) |
collection |
Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) |
repository.name.fl_str_mv |
Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) - Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informação |
repository.mail.fl_str_mv |
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1799132591656271872 |