Monolayer transition metal dichalcogenides in strong magnetic fields: validating the Wannier model using a microscopic calculation
Autor(a) principal: | |
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Data de Publicação: | 2019 |
Outros Autores: | , , |
Tipo de documento: | Artigo |
Idioma: | eng |
Título da fonte: | Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) |
Texto Completo: | http://hdl.handle.net/1822/60490 |
Resumo: | Using an equation of motion (EOM) approach, we calculate excitonic properties of monolayer transition metal dichalcogenides (TMDs) perturbed by an external magnetic field. We compare our findings to the widely used Wannier model for excitons in two-dimensional materials and to recent experimental results. We find good agreement between the calculated excitonic transition energies and the experimental results. In addition, we find that the exciton energies calculated using the EOM approach are slightly lower than the ones calculated using the Wannier model. Finally, we also show that the effect of the dielectric environment on the magnetoexciton transition energy is minimal due to counteracting changes in the exciton energy and the exchange self-energy correction. |
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Monolayer transition metal dichalcogenides in strong magnetic fields: validating the Wannier model using a microscopic calculationCiências Naturais::Ciências FísicasScience & TechnologyUsing an equation of motion (EOM) approach, we calculate excitonic properties of monolayer transition metal dichalcogenides (TMDs) perturbed by an external magnetic field. We compare our findings to the widely used Wannier model for excitons in two-dimensional materials and to recent experimental results. We find good agreement between the calculated excitonic transition energies and the experimental results. In addition, we find that the exciton energies calculated using the EOM approach are slightly lower than the ones calculated using the Wannier model. Finally, we also show that the effect of the dielectric environment on the magnetoexciton transition energy is minimal due to counteracting changes in the exciton energy and the exchange self-energy correction.J.H. and T.G.P. gratefully acknowledge financial support by the QUSCOPE Center, sponsored by the Villum Foundation. Additionally, T.G.P. is supported by the Center for Nanostructured Graphene (CNG), which is sponsored by the Danish National Research Foundation, Project No. DNRF103. G.C. acknowledges financial support from FCT for the P2020-PTDC/FIS-NAN/4662/2014 project. N.M.R.P. acknowledges support from the European Commission through the project "Graphene-Driven Revolutions in ICT and Beyond" (Ref. No. 785219), and the Portuguese Foundation for Science and Technology (FCT) in the framework of the Strategic Financing UID/FIS/04650/2013. Additionally, N.M.R.P. acknowledges COMPETE2020, PORTUGAL2020, FEDER, and the Portuguese Foundation for Science and Technology (FCT) through Project No. PTDC/FIS-NAN/3668/201.info:eu-repo/semantics/publishedVersionAmerican Physical Society (APS)Universidade do MinhoHave, J.Catarina, G.Pedersen, T. G.Peres, N. M. R.20192019-01-01T00:00:00Zinfo:eu-repo/semantics/publishedVersioninfo:eu-repo/semantics/articleapplication/pdfhttp://hdl.handle.net/1822/60490eng2469-995010.1103/PhysRevB.99.035416info:eu-repo/semantics/openAccessreponame:Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos)instname:Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informaçãoinstacron:RCAAP2023-07-21T12:29:05Zoai:repositorium.sdum.uminho.pt:1822/60490Portal AgregadorONGhttps://www.rcaap.pt/oai/openaireopendoar:71602024-03-19T19:24:00.504274Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) - Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informaçãofalse |
dc.title.none.fl_str_mv |
Monolayer transition metal dichalcogenides in strong magnetic fields: validating the Wannier model using a microscopic calculation |
title |
Monolayer transition metal dichalcogenides in strong magnetic fields: validating the Wannier model using a microscopic calculation |
spellingShingle |
Monolayer transition metal dichalcogenides in strong magnetic fields: validating the Wannier model using a microscopic calculation Have, J. Ciências Naturais::Ciências Físicas Science & Technology |
title_short |
Monolayer transition metal dichalcogenides in strong magnetic fields: validating the Wannier model using a microscopic calculation |
title_full |
Monolayer transition metal dichalcogenides in strong magnetic fields: validating the Wannier model using a microscopic calculation |
title_fullStr |
Monolayer transition metal dichalcogenides in strong magnetic fields: validating the Wannier model using a microscopic calculation |
title_full_unstemmed |
Monolayer transition metal dichalcogenides in strong magnetic fields: validating the Wannier model using a microscopic calculation |
title_sort |
Monolayer transition metal dichalcogenides in strong magnetic fields: validating the Wannier model using a microscopic calculation |
author |
Have, J. |
author_facet |
Have, J. Catarina, G. Pedersen, T. G. Peres, N. M. R. |
author_role |
author |
author2 |
Catarina, G. Pedersen, T. G. Peres, N. M. R. |
author2_role |
author author author |
dc.contributor.none.fl_str_mv |
Universidade do Minho |
dc.contributor.author.fl_str_mv |
Have, J. Catarina, G. Pedersen, T. G. Peres, N. M. R. |
dc.subject.por.fl_str_mv |
Ciências Naturais::Ciências Físicas Science & Technology |
topic |
Ciências Naturais::Ciências Físicas Science & Technology |
description |
Using an equation of motion (EOM) approach, we calculate excitonic properties of monolayer transition metal dichalcogenides (TMDs) perturbed by an external magnetic field. We compare our findings to the widely used Wannier model for excitons in two-dimensional materials and to recent experimental results. We find good agreement between the calculated excitonic transition energies and the experimental results. In addition, we find that the exciton energies calculated using the EOM approach are slightly lower than the ones calculated using the Wannier model. Finally, we also show that the effect of the dielectric environment on the magnetoexciton transition energy is minimal due to counteracting changes in the exciton energy and the exchange self-energy correction. |
publishDate |
2019 |
dc.date.none.fl_str_mv |
2019 2019-01-01T00:00:00Z |
dc.type.status.fl_str_mv |
info:eu-repo/semantics/publishedVersion |
dc.type.driver.fl_str_mv |
info:eu-repo/semantics/article |
format |
article |
status_str |
publishedVersion |
dc.identifier.uri.fl_str_mv |
http://hdl.handle.net/1822/60490 |
url |
http://hdl.handle.net/1822/60490 |
dc.language.iso.fl_str_mv |
eng |
language |
eng |
dc.relation.none.fl_str_mv |
2469-9950 10.1103/PhysRevB.99.035416 |
dc.rights.driver.fl_str_mv |
info:eu-repo/semantics/openAccess |
eu_rights_str_mv |
openAccess |
dc.format.none.fl_str_mv |
application/pdf |
dc.publisher.none.fl_str_mv |
American Physical Society (APS) |
publisher.none.fl_str_mv |
American Physical Society (APS) |
dc.source.none.fl_str_mv |
reponame:Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) instname:Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informação instacron:RCAAP |
instname_str |
Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informação |
instacron_str |
RCAAP |
institution |
RCAAP |
reponame_str |
Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) |
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Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) |
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Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) - Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informação |
repository.mail.fl_str_mv |
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1799132717561937920 |