Late summer changes in burning conditions in the boreal regions and their implications for NO x and CO emissions from boreal fires
Autor(a) principal: | |
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Data de Publicação: | 2008 |
Outros Autores: | , , , , |
Tipo de documento: | Artigo |
Idioma: | eng |
Título da fonte: | Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) |
Texto Completo: | http://hdl.handle.net/10400.3/1471 |
Resumo: | Copyright © 2008 American Geophysical Union. All Rights Reserved. |
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Late summer changes in burning conditions in the boreal regions and their implications for NO x and CO emissions from boreal firesBoreal FiresNitrogen OxidesCarbon MonoxideNorth AtlanticCopyright © 2008 American Geophysical Union. All Rights Reserved.Building emission inventories for the fires in boreal regions remains a challenging task with significant uncertainties in the methods used. In this work, we assess the impact of seasonal trends in fuel consumption and flaming/smoldering ratios on emissions of species dominated by flaming combustion (e.g., NO x ) and species dominated by smoldering combustion (e.g., CO). This is accomplished using measurements of CO and NO y at the free tropospheric Pico Mountain observatory in the central North Atlantic during the active boreal fire seasons of 2004 and 2005. ΔNO y /ΔCO enhancement ratios in aged fire plumes had higher values in June-July (7.3 × 10−3 mol mol−1) relative to the values in August-September (2.8 × 10−3 mol mol−1), indicating that NO x /CO emission ratios declined significantly as the fire season progressed. This is consistent with our understanding that an increased amount of fuel is consumed via smoldering combustion during late summer, as deeper burning of the drying organic soil layer occurs. A major growth in fuel consumption per unit area is also expected, due to deeper burning. Emissions of CO and NO x from North American boreal fires were estimated using the Boreal Wildland Fire Emissions Model, and their long-range transport to the sampling site was modeled using FLEXPART. These simulations were generally consistent with the observations, but the modeled seasonal decline in the ΔNO y /ΔCO enhancement ratio was less than observed. Comparisons using alternative fire emission injection height scenarios suggest that plumes with the highest CO levels at the observatory were lofted well above the boundary layer, likely as a result of intense crown fires.American Geophysical Union (AGU)Repositório da Universidade dos AçoresLapina, K.Honrath, RichardOwen, R. ChrisVal Martin, MariaHyer, E. J.Fialho, Paulo2012-09-27T11:50:36Z2008-06-102012-09-26T16:40:09Z2008-06-10T00:00:00Zinfo:eu-repo/semantics/publishedVersioninfo:eu-repo/semantics/articleapplication/pdfhttp://hdl.handle.net/10400.3/1471engLapina, K.; Honrath, R. E.; Owen, R. C.; Val Martín, M.; Hyer, E. J.; Fialho, P. Late summer changes in burning conditions in the boreal regions and their implications for NO x and CO emissions from boreal fires, "Journal of Geophysical Research", 113, D11, D11304-1-D11304-13, 2008.0148-0227 (Print)info:eu-repo/semantics/openAccessreponame:Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos)instname:Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informaçãoinstacron:RCAAP2022-12-20T14:29:13Zoai:repositorio.uac.pt:10400.3/1471Portal AgregadorONGhttps://www.rcaap.pt/oai/openaireopendoar:71602024-03-19T16:24:19.921536Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) - Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informaçãofalse |
dc.title.none.fl_str_mv |
Late summer changes in burning conditions in the boreal regions and their implications for NO x and CO emissions from boreal fires |
title |
Late summer changes in burning conditions in the boreal regions and their implications for NO x and CO emissions from boreal fires |
spellingShingle |
Late summer changes in burning conditions in the boreal regions and their implications for NO x and CO emissions from boreal fires Lapina, K. Boreal Fires Nitrogen Oxides Carbon Monoxide North Atlantic |
title_short |
Late summer changes in burning conditions in the boreal regions and their implications for NO x and CO emissions from boreal fires |
title_full |
Late summer changes in burning conditions in the boreal regions and their implications for NO x and CO emissions from boreal fires |
title_fullStr |
Late summer changes in burning conditions in the boreal regions and their implications for NO x and CO emissions from boreal fires |
title_full_unstemmed |
Late summer changes in burning conditions in the boreal regions and their implications for NO x and CO emissions from boreal fires |
title_sort |
Late summer changes in burning conditions in the boreal regions and their implications for NO x and CO emissions from boreal fires |
author |
Lapina, K. |
author_facet |
Lapina, K. Honrath, Richard Owen, R. Chris Val Martin, Maria Hyer, E. J. Fialho, Paulo |
author_role |
author |
author2 |
Honrath, Richard Owen, R. Chris Val Martin, Maria Hyer, E. J. Fialho, Paulo |
author2_role |
author author author author author |
dc.contributor.none.fl_str_mv |
Repositório da Universidade dos Açores |
dc.contributor.author.fl_str_mv |
Lapina, K. Honrath, Richard Owen, R. Chris Val Martin, Maria Hyer, E. J. Fialho, Paulo |
dc.subject.por.fl_str_mv |
Boreal Fires Nitrogen Oxides Carbon Monoxide North Atlantic |
topic |
Boreal Fires Nitrogen Oxides Carbon Monoxide North Atlantic |
description |
Copyright © 2008 American Geophysical Union. All Rights Reserved. |
publishDate |
2008 |
dc.date.none.fl_str_mv |
2008-06-10 2008-06-10T00:00:00Z 2012-09-27T11:50:36Z 2012-09-26T16:40:09Z |
dc.type.status.fl_str_mv |
info:eu-repo/semantics/publishedVersion |
dc.type.driver.fl_str_mv |
info:eu-repo/semantics/article |
format |
article |
status_str |
publishedVersion |
dc.identifier.uri.fl_str_mv |
http://hdl.handle.net/10400.3/1471 |
url |
http://hdl.handle.net/10400.3/1471 |
dc.language.iso.fl_str_mv |
eng |
language |
eng |
dc.relation.none.fl_str_mv |
Lapina, K.; Honrath, R. E.; Owen, R. C.; Val Martín, M.; Hyer, E. J.; Fialho, P. Late summer changes in burning conditions in the boreal regions and their implications for NO x and CO emissions from boreal fires, "Journal of Geophysical Research", 113, D11, D11304-1-D11304-13, 2008. 0148-0227 (Print) |
dc.rights.driver.fl_str_mv |
info:eu-repo/semantics/openAccess |
eu_rights_str_mv |
openAccess |
dc.format.none.fl_str_mv |
application/pdf |
dc.publisher.none.fl_str_mv |
American Geophysical Union (AGU) |
publisher.none.fl_str_mv |
American Geophysical Union (AGU) |
dc.source.none.fl_str_mv |
reponame:Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) instname:Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informação instacron:RCAAP |
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Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informação |
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RCAAP |
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RCAAP |
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Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) |
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Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) |
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Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) - Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informação |
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