Tackling Humidity with Designer Ionic Liquid-Based Gas Sensing Soft Materials
Autor(a) principal: | |
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Data de Publicação: | 2022 |
Outros Autores: | , , , , , , , |
Tipo de documento: | Artigo |
Idioma: | eng |
Título da fonte: | Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) |
Texto Completo: | http://hdl.handle.net/10400.5/23391 |
Resumo: | Research Article |
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Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) |
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7160 |
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Tackling Humidity with Designer Ionic Liquid-Based Gas Sensing Soft Materialshumiditysensing mechanismsResearch ArticleRelative humidity is simultaneously a sensing target and a contaminant in gas and volatile organic compound (VOC) sensing systems, where strategies to control humidity interference are required. An unmet challenge is the creation of gas-sensitive materials where the response to humidity is controlled by the material itself. Here, humidity effects are controlled through the design of gelatin formulations in ionic liquids without and with liquid crystals as electrical and optical sensors, respectively. In this design, the anions [DCA]− and [Cl]− of room temperature ionic liquids from the 1-butyl-3-methylimidazolium family tailor the response to humidity and, subsequently, sensing of VOCs in dry and humid conditions. Due to the combined effect of the materials formulations and sensing mechanisms, changing the anion from [DCA]− to the much more hygroscopic [Cl]−, leads to stronger electrical responses and much weaker optical responses to humidity. Thus, either humidity sensors or humidity-tolerant VOC sensors that do not require sample preconditioning or signal processing to correct humidity impact are obtained. With the wide spread of 3D- and 4D-printing and intelligent devices, the monitoring and tuning of humidity in sustainable biobased materials offers excellent opportunities in e-nose sensing arrays and wearable devices compatible with operation at room conditionsWiley-VCHRepositório da Universidade de LisboaEsteves, C.Palma, S.I.C.J.Costa, H.M.A.Alves, C.Santos, G.M.C.Ramou, E.Carvalho, A.L.Delgado Alves, VitorRoque, A.C.A.2022-02-04T16:17:59Z20222022-01-01T00:00:00Zinfo:eu-repo/semantics/publishedVersioninfo:eu-repo/semantics/articleapplication/pdfhttp://hdl.handle.net/10400.5/23391engAdv. Mater. 2022, 210720510.1002/adma.202107205info:eu-repo/semantics/openAccessreponame:Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos)instname:Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informaçãoinstacron:RCAAP2023-03-06T14:52:56Zoai:www.repository.utl.pt:10400.5/23391Portal AgregadorONGhttps://www.rcaap.pt/oai/openaireopendoar:71602024-03-19T17:07:38.327544Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) - Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informaçãofalse |
dc.title.none.fl_str_mv |
Tackling Humidity with Designer Ionic Liquid-Based Gas Sensing Soft Materials |
title |
Tackling Humidity with Designer Ionic Liquid-Based Gas Sensing Soft Materials |
spellingShingle |
Tackling Humidity with Designer Ionic Liquid-Based Gas Sensing Soft Materials Esteves, C. humidity sensing mechanisms |
title_short |
Tackling Humidity with Designer Ionic Liquid-Based Gas Sensing Soft Materials |
title_full |
Tackling Humidity with Designer Ionic Liquid-Based Gas Sensing Soft Materials |
title_fullStr |
Tackling Humidity with Designer Ionic Liquid-Based Gas Sensing Soft Materials |
title_full_unstemmed |
Tackling Humidity with Designer Ionic Liquid-Based Gas Sensing Soft Materials |
title_sort |
Tackling Humidity with Designer Ionic Liquid-Based Gas Sensing Soft Materials |
author |
Esteves, C. |
author_facet |
Esteves, C. Palma, S.I.C.J. Costa, H.M.A. Alves, C. Santos, G.M.C. Ramou, E. Carvalho, A.L. Delgado Alves, Vitor Roque, A.C.A. |
author_role |
author |
author2 |
Palma, S.I.C.J. Costa, H.M.A. Alves, C. Santos, G.M.C. Ramou, E. Carvalho, A.L. Delgado Alves, Vitor Roque, A.C.A. |
author2_role |
author author author author author author author author |
dc.contributor.none.fl_str_mv |
Repositório da Universidade de Lisboa |
dc.contributor.author.fl_str_mv |
Esteves, C. Palma, S.I.C.J. Costa, H.M.A. Alves, C. Santos, G.M.C. Ramou, E. Carvalho, A.L. Delgado Alves, Vitor Roque, A.C.A. |
dc.subject.por.fl_str_mv |
humidity sensing mechanisms |
topic |
humidity sensing mechanisms |
description |
Research Article |
publishDate |
2022 |
dc.date.none.fl_str_mv |
2022-02-04T16:17:59Z 2022 2022-01-01T00:00:00Z |
dc.type.status.fl_str_mv |
info:eu-repo/semantics/publishedVersion |
dc.type.driver.fl_str_mv |
info:eu-repo/semantics/article |
format |
article |
status_str |
publishedVersion |
dc.identifier.uri.fl_str_mv |
http://hdl.handle.net/10400.5/23391 |
url |
http://hdl.handle.net/10400.5/23391 |
dc.language.iso.fl_str_mv |
eng |
language |
eng |
dc.relation.none.fl_str_mv |
Adv. Mater. 2022, 2107205 10.1002/adma.202107205 |
dc.rights.driver.fl_str_mv |
info:eu-repo/semantics/openAccess |
eu_rights_str_mv |
openAccess |
dc.format.none.fl_str_mv |
application/pdf |
dc.publisher.none.fl_str_mv |
Wiley-VCH |
publisher.none.fl_str_mv |
Wiley-VCH |
dc.source.none.fl_str_mv |
reponame:Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) instname:Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informação instacron:RCAAP |
instname_str |
Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informação |
instacron_str |
RCAAP |
institution |
RCAAP |
reponame_str |
Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) |
collection |
Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) |
repository.name.fl_str_mv |
Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) - Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informação |
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1799131170066137088 |