PREPARATION AND VISIBLE LIGHT RESPONSIVE PHOTOCATALYTIC ACTIVITY OF Fe3O4/Ni-Al-Ce LDH/Bi2WO6 COMPOSITES

Detalhes bibliográficos
Autor(a) principal: Hao,Jiaqi
Data de Publicação: 2017
Outros Autores: Qu,Ting, Wang,Qiufeng, Zhao,Zhenbo
Tipo de documento: Artigo
Idioma: eng
Título da fonte: Química Nova (Online)
Texto Completo: http://old.scielo.br/scielo.php?script=sci_arttext&pid=S0100-40422017000800849
Resumo: Novel Fe3O4/Ni-Al-Ce LDH/Bi2WO6 composites were prepared through a hydrothermal method and co-precipitation method. The morphologies and structures of the photocatalysts were characterized by XRD, Raman, TEM, UV-vis-DRS, BET surface area and VSM techniques. The photocatalytic performances of the photocatalysts were investigated by the decolorization of methyl orange (MO) under visible-light irradiation. The results showed that the Fe3O4/Ni-Al-Ce LDH/Bi2WO6 composites exhibited greater photocatalytic activities compared to pure Bi2WO6 and the Ni-Al-Ce LDH; the decolorization rate of MO was 87% within 60 min under visible-light irradiation. The decolorization efficiency of the composite material remained at 71% after 4 recycling runs, showing improved stability. Furthermore, the experimental results also showed that the photocatalytic reactions for the composites followed first-order reaction kinetics. Therefore, the Fe3O4/Ni-Al-Ce LDH/Bi2WO6 composites were photocatalysts with high efficiencies and stabilities for a photocatalytic reaction of an organic pollutant, and this study provides a new, effective method for the development of wastewater treatment.
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spelling PREPARATION AND VISIBLE LIGHT RESPONSIVE PHOTOCATALYTIC ACTIVITY OF Fe3O4/Ni-Al-Ce LDH/Bi2WO6 COMPOSITEShydrothermal methodco-precipitationFe3O4/Ni-Al-Ce LDH/Bi2WO6 compositesphotocatalyticNovel Fe3O4/Ni-Al-Ce LDH/Bi2WO6 composites were prepared through a hydrothermal method and co-precipitation method. The morphologies and structures of the photocatalysts were characterized by XRD, Raman, TEM, UV-vis-DRS, BET surface area and VSM techniques. The photocatalytic performances of the photocatalysts were investigated by the decolorization of methyl orange (MO) under visible-light irradiation. The results showed that the Fe3O4/Ni-Al-Ce LDH/Bi2WO6 composites exhibited greater photocatalytic activities compared to pure Bi2WO6 and the Ni-Al-Ce LDH; the decolorization rate of MO was 87% within 60 min under visible-light irradiation. The decolorization efficiency of the composite material remained at 71% after 4 recycling runs, showing improved stability. Furthermore, the experimental results also showed that the photocatalytic reactions for the composites followed first-order reaction kinetics. Therefore, the Fe3O4/Ni-Al-Ce LDH/Bi2WO6 composites were photocatalysts with high efficiencies and stabilities for a photocatalytic reaction of an organic pollutant, and this study provides a new, effective method for the development of wastewater treatment.Sociedade Brasileira de Química2017-09-01info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersiontext/htmlhttp://old.scielo.br/scielo.php?script=sci_arttext&pid=S0100-40422017000800849Química Nova v.40 n.8 2017reponame:Química Nova (Online)instname:Sociedade Brasileira de Química (SBQ)instacron:SBQ10.21577/0100-4042.20170062info:eu-repo/semantics/openAccessHao,JiaqiQu,TingWang,QiufengZhao,Zhenboeng2017-10-04T00:00:00Zoai:scielo:S0100-40422017000800849Revistahttps://www.scielo.br/j/qn/ONGhttps://old.scielo.br/oai/scielo-oai.phpquimicanova@sbq.org.br1678-70640100-4042opendoar:2017-10-04T00:00Química Nova (Online) - Sociedade Brasileira de Química (SBQ)false
dc.title.none.fl_str_mv PREPARATION AND VISIBLE LIGHT RESPONSIVE PHOTOCATALYTIC ACTIVITY OF Fe3O4/Ni-Al-Ce LDH/Bi2WO6 COMPOSITES
title PREPARATION AND VISIBLE LIGHT RESPONSIVE PHOTOCATALYTIC ACTIVITY OF Fe3O4/Ni-Al-Ce LDH/Bi2WO6 COMPOSITES
spellingShingle PREPARATION AND VISIBLE LIGHT RESPONSIVE PHOTOCATALYTIC ACTIVITY OF Fe3O4/Ni-Al-Ce LDH/Bi2WO6 COMPOSITES
Hao,Jiaqi
hydrothermal method
co-precipitation
Fe3O4/Ni-Al-Ce LDH/Bi2WO6 composites
photocatalytic
title_short PREPARATION AND VISIBLE LIGHT RESPONSIVE PHOTOCATALYTIC ACTIVITY OF Fe3O4/Ni-Al-Ce LDH/Bi2WO6 COMPOSITES
title_full PREPARATION AND VISIBLE LIGHT RESPONSIVE PHOTOCATALYTIC ACTIVITY OF Fe3O4/Ni-Al-Ce LDH/Bi2WO6 COMPOSITES
title_fullStr PREPARATION AND VISIBLE LIGHT RESPONSIVE PHOTOCATALYTIC ACTIVITY OF Fe3O4/Ni-Al-Ce LDH/Bi2WO6 COMPOSITES
title_full_unstemmed PREPARATION AND VISIBLE LIGHT RESPONSIVE PHOTOCATALYTIC ACTIVITY OF Fe3O4/Ni-Al-Ce LDH/Bi2WO6 COMPOSITES
title_sort PREPARATION AND VISIBLE LIGHT RESPONSIVE PHOTOCATALYTIC ACTIVITY OF Fe3O4/Ni-Al-Ce LDH/Bi2WO6 COMPOSITES
author Hao,Jiaqi
author_facet Hao,Jiaqi
Qu,Ting
Wang,Qiufeng
Zhao,Zhenbo
author_role author
author2 Qu,Ting
Wang,Qiufeng
Zhao,Zhenbo
author2_role author
author
author
dc.contributor.author.fl_str_mv Hao,Jiaqi
Qu,Ting
Wang,Qiufeng
Zhao,Zhenbo
dc.subject.por.fl_str_mv hydrothermal method
co-precipitation
Fe3O4/Ni-Al-Ce LDH/Bi2WO6 composites
photocatalytic
topic hydrothermal method
co-precipitation
Fe3O4/Ni-Al-Ce LDH/Bi2WO6 composites
photocatalytic
description Novel Fe3O4/Ni-Al-Ce LDH/Bi2WO6 composites were prepared through a hydrothermal method and co-precipitation method. The morphologies and structures of the photocatalysts were characterized by XRD, Raman, TEM, UV-vis-DRS, BET surface area and VSM techniques. The photocatalytic performances of the photocatalysts were investigated by the decolorization of methyl orange (MO) under visible-light irradiation. The results showed that the Fe3O4/Ni-Al-Ce LDH/Bi2WO6 composites exhibited greater photocatalytic activities compared to pure Bi2WO6 and the Ni-Al-Ce LDH; the decolorization rate of MO was 87% within 60 min under visible-light irradiation. The decolorization efficiency of the composite material remained at 71% after 4 recycling runs, showing improved stability. Furthermore, the experimental results also showed that the photocatalytic reactions for the composites followed first-order reaction kinetics. Therefore, the Fe3O4/Ni-Al-Ce LDH/Bi2WO6 composites were photocatalysts with high efficiencies and stabilities for a photocatalytic reaction of an organic pollutant, and this study provides a new, effective method for the development of wastewater treatment.
publishDate 2017
dc.date.none.fl_str_mv 2017-09-01
dc.type.driver.fl_str_mv info:eu-repo/semantics/article
dc.type.status.fl_str_mv info:eu-repo/semantics/publishedVersion
format article
status_str publishedVersion
dc.identifier.uri.fl_str_mv http://old.scielo.br/scielo.php?script=sci_arttext&pid=S0100-40422017000800849
url http://old.scielo.br/scielo.php?script=sci_arttext&pid=S0100-40422017000800849
dc.language.iso.fl_str_mv eng
language eng
dc.relation.none.fl_str_mv 10.21577/0100-4042.20170062
dc.rights.driver.fl_str_mv info:eu-repo/semantics/openAccess
eu_rights_str_mv openAccess
dc.format.none.fl_str_mv text/html
dc.publisher.none.fl_str_mv Sociedade Brasileira de Química
publisher.none.fl_str_mv Sociedade Brasileira de Química
dc.source.none.fl_str_mv Química Nova v.40 n.8 2017
reponame:Química Nova (Online)
instname:Sociedade Brasileira de Química (SBQ)
instacron:SBQ
instname_str Sociedade Brasileira de Química (SBQ)
instacron_str SBQ
institution SBQ
reponame_str Química Nova (Online)
collection Química Nova (Online)
repository.name.fl_str_mv Química Nova (Online) - Sociedade Brasileira de Química (SBQ)
repository.mail.fl_str_mv quimicanova@sbq.org.br
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