Optical properties of in situ doped and undoped titania nanocatalysts and doped titania sol–gel nanofilms
Autor(a) principal: | |
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Data de Publicação: | 2006 |
Outros Autores: | , , , , , , , |
Tipo de documento: | Artigo |
Idioma: | eng |
Título da fonte: | Repositório Institucional da UFBA |
Texto Completo: | http://www.repositorio.ufba.br/ri/handle/ri/6521 |
Resumo: | RESTRITO |
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Silva, A. Ferreira daPepe, Iuri MunizGole, James L.Tomás, S. A.Palomino, R.Azevedo, W. M. deSilva Junior, E. F. daAhuja, RajeevPersson, C.Silva, A. Ferreira daPepe, Iuri MunizGole, James L.Tomás, S. A.Palomino, R.Azevedo, W. M. deSilva Junior, E. F. daAhuja, RajeevPersson, C.2012-07-31T19:29:25Z2012-07-31T19:29:25Z20060169-4332http://www.repositorio.ufba.br/ri/handle/ri/6521v.252, n.15RESTRITOIn this paper we present spectroscopic properties of doped and undoped titanium dioxide (TiO2) as nanofilms prepared by the sol–gel process with rhodamine 6G doping and studied by photoacoustic absorption, excitation and emission spectroscopy. The absorption spectra of TiO2 thin films doped with rhodamine 6G at very low concentration during their preparation show two absorption bands, one at 2.3 eV attributed to molecular dimmer formation, which is responsible for the fluorescence quenching of the sample and the other at 3.0 eV attributed to TiO2 absorption, which subsequently yields a strong emission band at 600 nm. The electronic band structure and optical properties of the rutile phase of TiO2 are calculated employing a fully relativistic, full-potential, linearized, augmented plane-wave (FPLAPW) method within the local density approximation (LDA). Comparison of this calculation with experimental data for TiO2 films prepared for undoped sol–gels and by sputtering is performed. PACS 71.15.Mb; 71.20.Nr; 78.20.ci; 81.40.TvSubmitted by Santiago Fabio (fabio.ssantiago@hotmail.com) on 2012-07-31T19:29:24Z No. of bitstreams: 1 FF.pdf: 163108 bytes, checksum: fa9f02e3dd442b3a6d01fd65b93d8d91 (MD5)Made available in DSpace on 2012-07-31T19:29:25Z (GMT). No. of bitstreams: 1 FF.pdf: 163108 bytes, checksum: fa9f02e3dd442b3a6d01fd65b93d8d91 (MD5) Previous issue date: 2006Applied Surface Sciencehttp://dx.doi.org/10.1016/j.apsusc.2005.12.041reponame:Repositório Institucional da UFBAinstname:Universidade Federal da Bahia (UFBA)instacron:UFBAPolymerTiO2 nanofilmsElectronic band structureRhodamine 6G dopingOptical properties of in situ doped and undoped titania nanocatalysts and doped titania sol–gel nanofilmsApplied Surface Scienceinfo:eu-repo/semantics/publishedVersioninfo:eu-repo/semantics/articleenginfo:eu-repo/semantics/openAccessORIGINALFF.pdfFF.pdfapplication/pdf163108https://repositorio.ufba.br/bitstream/ri/6521/1/FF.pdffa9f02e3dd442b3a6d01fd65b93d8d91MD51LICENSElicense.txtlicense.txttext/plain1762https://repositorio.ufba.br/bitstream/ri/6521/2/license.txt1b89a9a0548218172d7c829f87a0eab9MD52TEXTFF.pdf.txtFF.pdf.txtExtracted texttext/plain12624https://repositorio.ufba.br/bitstream/ri/6521/3/FF.pdf.txt54c4ae14efdb83c0076a381cc767b7a1MD53ri/65212022-07-05 14:03:45.668oai:repositorio.ufba.br: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Repositório InstitucionalPUBhttp://192.188.11.11:8080/oai/requestopendoar:19322022-07-05T17:03:45Repositório Institucional da UFBA - Universidade Federal da Bahia (UFBA)false |
dc.title.pt_BR.fl_str_mv |
Optical properties of in situ doped and undoped titania nanocatalysts and doped titania sol–gel nanofilms |
dc.title.alternative.pt_BR.fl_str_mv |
Applied Surface Science |
title |
Optical properties of in situ doped and undoped titania nanocatalysts and doped titania sol–gel nanofilms |
spellingShingle |
Optical properties of in situ doped and undoped titania nanocatalysts and doped titania sol–gel nanofilms Silva, A. Ferreira da Polymer TiO2 nanofilms Electronic band structure Rhodamine 6G doping |
title_short |
Optical properties of in situ doped and undoped titania nanocatalysts and doped titania sol–gel nanofilms |
title_full |
Optical properties of in situ doped and undoped titania nanocatalysts and doped titania sol–gel nanofilms |
title_fullStr |
Optical properties of in situ doped and undoped titania nanocatalysts and doped titania sol–gel nanofilms |
title_full_unstemmed |
Optical properties of in situ doped and undoped titania nanocatalysts and doped titania sol–gel nanofilms |
title_sort |
Optical properties of in situ doped and undoped titania nanocatalysts and doped titania sol–gel nanofilms |
author |
Silva, A. Ferreira da |
author_facet |
Silva, A. Ferreira da Pepe, Iuri Muniz Gole, James L. Tomás, S. A. Palomino, R. Azevedo, W. M. de Silva Junior, E. F. da Ahuja, Rajeev Persson, C. |
author_role |
author |
author2 |
Pepe, Iuri Muniz Gole, James L. Tomás, S. A. Palomino, R. Azevedo, W. M. de Silva Junior, E. F. da Ahuja, Rajeev Persson, C. |
author2_role |
author author author author author author author author |
dc.contributor.author.fl_str_mv |
Silva, A. Ferreira da Pepe, Iuri Muniz Gole, James L. Tomás, S. A. Palomino, R. Azevedo, W. M. de Silva Junior, E. F. da Ahuja, Rajeev Persson, C. Silva, A. Ferreira da Pepe, Iuri Muniz Gole, James L. Tomás, S. A. Palomino, R. Azevedo, W. M. de Silva Junior, E. F. da Ahuja, Rajeev Persson, C. |
dc.subject.por.fl_str_mv |
Polymer TiO2 nanofilms Electronic band structure Rhodamine 6G doping |
topic |
Polymer TiO2 nanofilms Electronic band structure Rhodamine 6G doping |
description |
RESTRITO |
publishDate |
2006 |
dc.date.issued.fl_str_mv |
2006 |
dc.date.accessioned.fl_str_mv |
2012-07-31T19:29:25Z |
dc.date.available.fl_str_mv |
2012-07-31T19:29:25Z |
dc.type.status.fl_str_mv |
info:eu-repo/semantics/publishedVersion |
dc.type.driver.fl_str_mv |
info:eu-repo/semantics/article |
format |
article |
status_str |
publishedVersion |
dc.identifier.uri.fl_str_mv |
http://www.repositorio.ufba.br/ri/handle/ri/6521 |
dc.identifier.issn.none.fl_str_mv |
0169-4332 |
dc.identifier.number.pt_BR.fl_str_mv |
v.252, n.15 |
identifier_str_mv |
0169-4332 v.252, n.15 |
url |
http://www.repositorio.ufba.br/ri/handle/ri/6521 |
dc.language.iso.fl_str_mv |
eng |
language |
eng |
dc.rights.driver.fl_str_mv |
info:eu-repo/semantics/openAccess |
eu_rights_str_mv |
openAccess |
dc.publisher.none.fl_str_mv |
Applied Surface Science |
publisher.none.fl_str_mv |
Applied Surface Science |
dc.source.pt_BR.fl_str_mv |
http://dx.doi.org/10.1016/j.apsusc.2005.12.041 |
dc.source.none.fl_str_mv |
reponame:Repositório Institucional da UFBA instname:Universidade Federal da Bahia (UFBA) instacron:UFBA |
instname_str |
Universidade Federal da Bahia (UFBA) |
instacron_str |
UFBA |
institution |
UFBA |
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Repositório Institucional da UFBA |
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Repositório Institucional da UFBA |
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