The influence of dopants on the catalytic activity of hematite in the ethylbenzene dehydrogenation
Autor(a) principal: | |
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Data de Publicação: | 2008 |
Outros Autores: | , , , |
Tipo de documento: | Artigo |
Idioma: | eng |
Título da fonte: | Repositório Institucional da UFBA |
Texto Completo: | http://www.repositorio.ufba.br/ri/handle/ri/6128 |
Resumo: | Acesso restrito: Texto completo. p. 12-17 |
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Ramos, Márcia de SouzaSantos, Manuela de SantanaGomes, Lucimar PachecoAlbornoz, AlbertoVarela, Maria do Carmo Rangel SantosRamos, Márcia de SouzaSantos, Manuela de SantanaGomes, Lucimar PachecoAlbornoz, AlbertoVarela, Maria do Carmo Rangel Santos2012-06-14T11:08:14Z20080926-860Xhttp://www.repositorio.ufba.br/ri/handle/ri/6128v. 341, n. 1-2Acesso restrito: Texto completo. p. 12-17The effect of neodymium, lanthanum, aluminum and zirconium on the textural and catalytic properties of hematite was studied in this work, which aimed to develop catalysts to ethylbenzene dehydrogenation, in the presence of steam, the main commercial route to obtain styrene. Hematite and magnetite were found in fresh and spent catalysts, respectively. All dopants increased the specific surface area of the fresh and spent catalysts and made them more resistant against reduction, but only aluminum avoided sintering during reaction. The dopants increased the catalytic activity per area of hematite, except aluminumwhich acted only as a textural promoter. The selectivity was decreased due to zirconium and lanthanum while the other dopants did not change this parameter. The neodymiumcontaining catalyst showed high levels of activity and selectivity and was able to work up to 530 8C, without deactivation, being the most promising with regard to styrene production.Submitted by JURANDI DE SOUZA SILVA (jssufba@hotmail.com) on 2012-06-14T11:08:14Z No. of bitstreams: 1 __ac.els-cdn.com_S003592...94ad7d084f834772b5bc760c76585.pdf: 235873 bytes, checksum: e1c84fdd7522fe1db5c5031dbef7f109 (MD5)Made available in DSpace on 2012-06-14T11:08:14Z (GMT). No. of bitstreams: 1 __ac.els-cdn.com_S003592...94ad7d084f834772b5bc760c76585.pdf: 235873 bytes, checksum: e1c84fdd7522fe1db5c5031dbef7f109 (MD5) Previous issue date: 2008http://dx.doi.org/10.1016/j.apcata.2007.12.035reponame:Repositório Institucional da UFBAinstname:Universidade Federal da Bahia (UFBA)instacron:UFBAStyreneEthylbenzeneHematiteThe influence of dopants on the catalytic activity of hematite in the ethylbenzene dehydrogenationApplied Catalysis A-Generalinfo:eu-repo/semantics/publishedVersioninfo:eu-repo/semantics/article10000-01-01enginfo:eu-repo/semantics/openAccessORIGINAL__ac.els-cdn.com_S003592...94ad7d084f834772b5bc760c76585.pdf__ac.els-cdn.com_S003592...94ad7d084f834772b5bc760c76585.pdfapplication/pdf235873https://repositorio.ufba.br/bitstream/ri/6128/1/__ac.els-cdn.com_S003592...94ad7d084f834772b5bc760c76585.pdfe1c84fdd7522fe1db5c5031dbef7f109MD51LICENSElicense.txtlicense.txttext/plain1762https://repositorio.ufba.br/bitstream/ri/6128/2/license.txt1b89a9a0548218172d7c829f87a0eab9MD52TEXT__ac.els-cdn.com_S003592...94ad7d084f834772b5bc760c76585.pdf.txt__ac.els-cdn.com_S003592...94ad7d084f834772b5bc760c76585.pdf.txtExtracted texttext/plain30285https://repositorio.ufba.br/bitstream/ri/6128/3/__ac.els-cdn.com_S003592...94ad7d084f834772b5bc760c76585.pdf.txtfb227dca27cdf8912874e046887f2560MD53ri/61282022-07-05 14:03:12.299oai:repositorio.ufba.br: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Repositório InstitucionalPUBhttp://192.188.11.11:8080/oai/requestopendoar:19322022-07-05T17:03:12Repositório Institucional da UFBA - Universidade Federal da Bahia (UFBA)false |
dc.title.pt_BR.fl_str_mv |
The influence of dopants on the catalytic activity of hematite in the ethylbenzene dehydrogenation |
dc.title.alternative.pt_BR.fl_str_mv |
Applied Catalysis A-General |
title |
The influence of dopants on the catalytic activity of hematite in the ethylbenzene dehydrogenation |
spellingShingle |
The influence of dopants on the catalytic activity of hematite in the ethylbenzene dehydrogenation Ramos, Márcia de Souza Styrene Ethylbenzene Hematite |
title_short |
The influence of dopants on the catalytic activity of hematite in the ethylbenzene dehydrogenation |
title_full |
The influence of dopants on the catalytic activity of hematite in the ethylbenzene dehydrogenation |
title_fullStr |
The influence of dopants on the catalytic activity of hematite in the ethylbenzene dehydrogenation |
title_full_unstemmed |
The influence of dopants on the catalytic activity of hematite in the ethylbenzene dehydrogenation |
title_sort |
The influence of dopants on the catalytic activity of hematite in the ethylbenzene dehydrogenation |
author |
Ramos, Márcia de Souza |
author_facet |
Ramos, Márcia de Souza Santos, Manuela de Santana Gomes, Lucimar Pacheco Albornoz, Alberto Varela, Maria do Carmo Rangel Santos |
author_role |
author |
author2 |
Santos, Manuela de Santana Gomes, Lucimar Pacheco Albornoz, Alberto Varela, Maria do Carmo Rangel Santos |
author2_role |
author author author author |
dc.contributor.author.fl_str_mv |
Ramos, Márcia de Souza Santos, Manuela de Santana Gomes, Lucimar Pacheco Albornoz, Alberto Varela, Maria do Carmo Rangel Santos Ramos, Márcia de Souza Santos, Manuela de Santana Gomes, Lucimar Pacheco Albornoz, Alberto Varela, Maria do Carmo Rangel Santos |
dc.subject.por.fl_str_mv |
Styrene Ethylbenzene Hematite |
topic |
Styrene Ethylbenzene Hematite |
description |
Acesso restrito: Texto completo. p. 12-17 |
publishDate |
2008 |
dc.date.issued.fl_str_mv |
2008 |
dc.date.accessioned.fl_str_mv |
2012-06-14T11:08:14Z |
dc.type.status.fl_str_mv |
info:eu-repo/semantics/publishedVersion |
dc.type.driver.fl_str_mv |
info:eu-repo/semantics/article |
format |
article |
status_str |
publishedVersion |
dc.identifier.uri.fl_str_mv |
http://www.repositorio.ufba.br/ri/handle/ri/6128 |
dc.identifier.issn.none.fl_str_mv |
0926-860X |
dc.identifier.number.pt_BR.fl_str_mv |
v. 341, n. 1-2 |
identifier_str_mv |
0926-860X v. 341, n. 1-2 |
url |
http://www.repositorio.ufba.br/ri/handle/ri/6128 |
dc.language.iso.fl_str_mv |
eng |
language |
eng |
dc.rights.driver.fl_str_mv |
info:eu-repo/semantics/openAccess |
eu_rights_str_mv |
openAccess |
dc.source.pt_BR.fl_str_mv |
http://dx.doi.org/10.1016/j.apcata.2007.12.035 |
dc.source.none.fl_str_mv |
reponame:Repositório Institucional da UFBA instname:Universidade Federal da Bahia (UFBA) instacron:UFBA |
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Universidade Federal da Bahia (UFBA) |
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UFBA |
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Repositório Institucional da UFBA |
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