Enhanced initial growth of atomic-layer-deposited metal oxides on hydrogen-terminated silicon
Autor(a) principal: | |
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Data de Publicação: | 2003 |
Outros Autores: | , , , , , , , , |
Tipo de documento: | Artigo |
Idioma: | eng |
Título da fonte: | Repositório Institucional da UFRGS |
Texto Completo: | http://hdl.handle.net/10183/141213 |
Resumo: | A route is presented for activation of hydrogen-terminated Si(100) prior to atomic layer deposition. It is based on our discovery from in situ infrared spectroscopy that organometallic precursors can effectively initiate oxide growth. Narrow nuclear resonance profiling and Rutherford backscattering spectrometry show that surface functionalization by pre-exposure to 108 Langmuir trimethylaluminum at 300 °C leads to enhanced nucleation and to nearly linear growth kinetics of the high-permittivity gate dielectrics aluminum oxide and hafnium oxide. |
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Frank, Martin M.Chabal, Yves JeanGreen, Martin L.Delabie, AnneliesBrijs, BertWilk, Glen D.Ho, Mun-YeeRosa, Elisa Brod Oliveira daBaumvol, Israel Jacob RabinStedile, Fernanda Chiarello2016-05-17T02:07:24Z20030003-6951http://hdl.handle.net/10183/141213000376604A route is presented for activation of hydrogen-terminated Si(100) prior to atomic layer deposition. It is based on our discovery from in situ infrared spectroscopy that organometallic precursors can effectively initiate oxide growth. Narrow nuclear resonance profiling and Rutherford backscattering spectrometry show that surface functionalization by pre-exposure to 108 Langmuir trimethylaluminum at 300 °C leads to enhanced nucleation and to nearly linear growth kinetics of the high-permittivity gate dielectrics aluminum oxide and hafnium oxide.application/pdfengApplied physics letters. Melville. Vol. 83, no. 4 (July 2003), p. 740-742Físico-químicaEnhanced initial growth of atomic-layer-deposited metal oxides on hydrogen-terminated siliconEstrangeiroinfo:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersioninfo:eu-repo/semantics/openAccessreponame:Repositório Institucional da UFRGSinstname:Universidade Federal do Rio Grande do Sul (UFRGS)instacron:UFRGSORIGINAL000376604.pdf000376604.pdfTexto completo (inglês)application/pdf543812http://www.lume.ufrgs.br/bitstream/10183/141213/1/000376604.pdfbebf8ac6656788dcf2a5a1052aa5f843MD51TEXT000376604.pdf.txt000376604.pdf.txtExtracted Texttext/plain19075http://www.lume.ufrgs.br/bitstream/10183/141213/2/000376604.pdf.txt83ade94a6b82b4bd1dc5f9d9cddf2e64MD52THUMBNAIL000376604.pdf.jpg000376604.pdf.jpgGenerated Thumbnailimage/jpeg2304http://www.lume.ufrgs.br/bitstream/10183/141213/3/000376604.pdf.jpg93b73e93736a2f94a248520ba92c56c8MD5310183/1412132020-01-16 05:09:24.165007oai:www.lume.ufrgs.br:10183/141213Repositório de PublicaçõesPUBhttps://lume.ufrgs.br/oai/requestopendoar:2020-01-16T07:09:24Repositório Institucional da UFRGS - Universidade Federal do Rio Grande do Sul (UFRGS)false |
dc.title.pt_BR.fl_str_mv |
Enhanced initial growth of atomic-layer-deposited metal oxides on hydrogen-terminated silicon |
title |
Enhanced initial growth of atomic-layer-deposited metal oxides on hydrogen-terminated silicon |
spellingShingle |
Enhanced initial growth of atomic-layer-deposited metal oxides on hydrogen-terminated silicon Frank, Martin M. Físico-química |
title_short |
Enhanced initial growth of atomic-layer-deposited metal oxides on hydrogen-terminated silicon |
title_full |
Enhanced initial growth of atomic-layer-deposited metal oxides on hydrogen-terminated silicon |
title_fullStr |
Enhanced initial growth of atomic-layer-deposited metal oxides on hydrogen-terminated silicon |
title_full_unstemmed |
Enhanced initial growth of atomic-layer-deposited metal oxides on hydrogen-terminated silicon |
title_sort |
Enhanced initial growth of atomic-layer-deposited metal oxides on hydrogen-terminated silicon |
author |
Frank, Martin M. |
author_facet |
Frank, Martin M. Chabal, Yves Jean Green, Martin L. Delabie, Annelies Brijs, Bert Wilk, Glen D. Ho, Mun-Yee Rosa, Elisa Brod Oliveira da Baumvol, Israel Jacob Rabin Stedile, Fernanda Chiarello |
author_role |
author |
author2 |
Chabal, Yves Jean Green, Martin L. Delabie, Annelies Brijs, Bert Wilk, Glen D. Ho, Mun-Yee Rosa, Elisa Brod Oliveira da Baumvol, Israel Jacob Rabin Stedile, Fernanda Chiarello |
author2_role |
author author author author author author author author author |
dc.contributor.author.fl_str_mv |
Frank, Martin M. Chabal, Yves Jean Green, Martin L. Delabie, Annelies Brijs, Bert Wilk, Glen D. Ho, Mun-Yee Rosa, Elisa Brod Oliveira da Baumvol, Israel Jacob Rabin Stedile, Fernanda Chiarello |
dc.subject.por.fl_str_mv |
Físico-química |
topic |
Físico-química |
description |
A route is presented for activation of hydrogen-terminated Si(100) prior to atomic layer deposition. It is based on our discovery from in situ infrared spectroscopy that organometallic precursors can effectively initiate oxide growth. Narrow nuclear resonance profiling and Rutherford backscattering spectrometry show that surface functionalization by pre-exposure to 108 Langmuir trimethylaluminum at 300 °C leads to enhanced nucleation and to nearly linear growth kinetics of the high-permittivity gate dielectrics aluminum oxide and hafnium oxide. |
publishDate |
2003 |
dc.date.issued.fl_str_mv |
2003 |
dc.date.accessioned.fl_str_mv |
2016-05-17T02:07:24Z |
dc.type.driver.fl_str_mv |
Estrangeiro info:eu-repo/semantics/article |
dc.type.status.fl_str_mv |
info:eu-repo/semantics/publishedVersion |
format |
article |
status_str |
publishedVersion |
dc.identifier.uri.fl_str_mv |
http://hdl.handle.net/10183/141213 |
dc.identifier.issn.pt_BR.fl_str_mv |
0003-6951 |
dc.identifier.nrb.pt_BR.fl_str_mv |
000376604 |
identifier_str_mv |
0003-6951 000376604 |
url |
http://hdl.handle.net/10183/141213 |
dc.language.iso.fl_str_mv |
eng |
language |
eng |
dc.relation.ispartof.pt_BR.fl_str_mv |
Applied physics letters. Melville. Vol. 83, no. 4 (July 2003), p. 740-742 |
dc.rights.driver.fl_str_mv |
info:eu-repo/semantics/openAccess |
eu_rights_str_mv |
openAccess |
dc.format.none.fl_str_mv |
application/pdf |
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Repositório Institucional da UFRGS |
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Repositório Institucional da UFRGS |
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