Oxidative coupling of methane for ethylene production : reviewing kinetic modelling approaches, thermodynamics and catalysts
Autor(a) principal: | |
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Data de Publicação: | 2021 |
Outros Autores: | , , , |
Tipo de documento: | Artigo |
Idioma: | eng |
Título da fonte: | Repositório Institucional da UFRGS |
Texto Completo: | http://hdl.handle.net/10183/250478 |
Resumo: | Ethylene production via oxidative coupling of methane (OCM) represents an interesting route for natural gas upscaling, being the focus of intensive research worldwide. Here, OCM developments are analysed in terms of kinetic mechanisms and respective applications in chemical reactor models, discussing current challenges and directions for further developments. Furthermore, some thermodynamic aspects of the OCM reactions are also revised, providing achievable olefins yields in a wide range of operational reaction conditions. Finally, OCM catalysts are reviewed in terms of respective catalytic performances and thermal stability, providing an executive summary for future studies on OCM economic feasibility. |
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Ros, Simoní daFontoura, Tahyná BarbalhoSchwaab, MarcioJesus, Normando José Castro dePinto, José Carlos2022-10-27T04:52:20Z20212227-9717http://hdl.handle.net/10183/250478001151133Ethylene production via oxidative coupling of methane (OCM) represents an interesting route for natural gas upscaling, being the focus of intensive research worldwide. Here, OCM developments are analysed in terms of kinetic mechanisms and respective applications in chemical reactor models, discussing current challenges and directions for further developments. Furthermore, some thermodynamic aspects of the OCM reactions are also revised, providing achievable olefins yields in a wide range of operational reaction conditions. Finally, OCM catalysts are reviewed in terms of respective catalytic performances and thermal stability, providing an executive summary for future studies on OCM economic feasibility.application/pdfengProcesses [recurso eletrônico]. Basel, Switzerland. Vol. 9, n. 12 (Dec. 2021), [Article] 2196, 48 p.EtilenoReações químicasCatalisadoresNatural gas upscalingEtheneChemical reactorsThermal effectsCatalyst stabilityOxidative coupling of methane for ethylene production : reviewing kinetic modelling approaches, thermodynamics and catalystsEstrangeiroinfo:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersioninfo:eu-repo/semantics/openAccessreponame:Repositório Institucional da UFRGSinstname:Universidade Federal do Rio Grande do Sul (UFRGS)instacron:UFRGSTEXT001151133.pdf.txt001151133.pdf.txtExtracted Texttext/plain203410http://www.lume.ufrgs.br/bitstream/10183/250478/2/001151133.pdf.txta4e85740ec503d01bd9438a3c3cebc65MD52ORIGINAL001151133.pdfTexto completoapplication/pdf8996088http://www.lume.ufrgs.br/bitstream/10183/250478/1/001151133.pdfc78acc776da29f5571a08ca3814e5c1dMD5110183/2504782022-10-28 04:47:47.161101oai:www.lume.ufrgs.br:10183/250478Repositório de PublicaçõesPUBhttps://lume.ufrgs.br/oai/requestopendoar:2022-10-28T07:47:47Repositório Institucional da UFRGS - Universidade Federal do Rio Grande do Sul (UFRGS)false |
dc.title.pt_BR.fl_str_mv |
Oxidative coupling of methane for ethylene production : reviewing kinetic modelling approaches, thermodynamics and catalysts |
title |
Oxidative coupling of methane for ethylene production : reviewing kinetic modelling approaches, thermodynamics and catalysts |
spellingShingle |
Oxidative coupling of methane for ethylene production : reviewing kinetic modelling approaches, thermodynamics and catalysts Ros, Simoní da Etileno Reações químicas Catalisadores Natural gas upscaling Ethene Chemical reactors Thermal effects Catalyst stability |
title_short |
Oxidative coupling of methane for ethylene production : reviewing kinetic modelling approaches, thermodynamics and catalysts |
title_full |
Oxidative coupling of methane for ethylene production : reviewing kinetic modelling approaches, thermodynamics and catalysts |
title_fullStr |
Oxidative coupling of methane for ethylene production : reviewing kinetic modelling approaches, thermodynamics and catalysts |
title_full_unstemmed |
Oxidative coupling of methane for ethylene production : reviewing kinetic modelling approaches, thermodynamics and catalysts |
title_sort |
Oxidative coupling of methane for ethylene production : reviewing kinetic modelling approaches, thermodynamics and catalysts |
author |
Ros, Simoní da |
author_facet |
Ros, Simoní da Fontoura, Tahyná Barbalho Schwaab, Marcio Jesus, Normando José Castro de Pinto, José Carlos |
author_role |
author |
author2 |
Fontoura, Tahyná Barbalho Schwaab, Marcio Jesus, Normando José Castro de Pinto, José Carlos |
author2_role |
author author author author |
dc.contributor.author.fl_str_mv |
Ros, Simoní da Fontoura, Tahyná Barbalho Schwaab, Marcio Jesus, Normando José Castro de Pinto, José Carlos |
dc.subject.por.fl_str_mv |
Etileno Reações químicas Catalisadores |
topic |
Etileno Reações químicas Catalisadores Natural gas upscaling Ethene Chemical reactors Thermal effects Catalyst stability |
dc.subject.eng.fl_str_mv |
Natural gas upscaling Ethene Chemical reactors Thermal effects Catalyst stability |
description |
Ethylene production via oxidative coupling of methane (OCM) represents an interesting route for natural gas upscaling, being the focus of intensive research worldwide. Here, OCM developments are analysed in terms of kinetic mechanisms and respective applications in chemical reactor models, discussing current challenges and directions for further developments. Furthermore, some thermodynamic aspects of the OCM reactions are also revised, providing achievable olefins yields in a wide range of operational reaction conditions. Finally, OCM catalysts are reviewed in terms of respective catalytic performances and thermal stability, providing an executive summary for future studies on OCM economic feasibility. |
publishDate |
2021 |
dc.date.issued.fl_str_mv |
2021 |
dc.date.accessioned.fl_str_mv |
2022-10-27T04:52:20Z |
dc.type.driver.fl_str_mv |
Estrangeiro info:eu-repo/semantics/article |
dc.type.status.fl_str_mv |
info:eu-repo/semantics/publishedVersion |
format |
article |
status_str |
publishedVersion |
dc.identifier.uri.fl_str_mv |
http://hdl.handle.net/10183/250478 |
dc.identifier.issn.pt_BR.fl_str_mv |
2227-9717 |
dc.identifier.nrb.pt_BR.fl_str_mv |
001151133 |
identifier_str_mv |
2227-9717 001151133 |
url |
http://hdl.handle.net/10183/250478 |
dc.language.iso.fl_str_mv |
eng |
language |
eng |
dc.relation.ispartof.pt_BR.fl_str_mv |
Processes [recurso eletrônico]. Basel, Switzerland. Vol. 9, n. 12 (Dec. 2021), [Article] 2196, 48 p. |
dc.rights.driver.fl_str_mv |
info:eu-repo/semantics/openAccess |
eu_rights_str_mv |
openAccess |
dc.format.none.fl_str_mv |
application/pdf |
dc.source.none.fl_str_mv |
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UFRGS |
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Repositório Institucional da UFRGS |
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Repositório Institucional da UFRGS |
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