Novel 3D‑fower shaped KTaO3 perovskite for highly efcient photocatalytic and ­H2 generation ability

Detalhes bibliográficos
Autor(a) principal: Sumedha, H. N.
Data de Publicação: 2022
Outros Autores: Shashank, Manjunatha, Teixeira, Sergio Ribeiro, Praveen, Beekanahalli Mokshanatha, Nagaraju, Ganganagappa
Tipo de documento: Artigo
Idioma: eng
Título da fonte: Repositório Institucional da UFRGS
Texto Completo: http://hdl.handle.net/10183/249617
Resumo: Treatment of industrial wastewater is one of the biggest challenges that mankind is facing today to prevent environmental pollution and its associated adverse efects on human health. Environmentalists across the world have given a clarion call for dye degradation, wastewater treatment and their efective management in our surrounding habitats. Despite signifcant progress in the development of new water treatment technologies, new materials haven’t matured enough for large scale industrial applications. Hence, the development of new scalable and sustainable multifunctional materials having the potential to treat wastewater and generate energy is the need of the hour. In this direction, novel 3D-fower shaped KTaO3 (3D-F-KT) material has been synthesized using areca seed powder as a green fuel. This new material has been successfully applied for the treatment of industrial wastewater contaminated with Rose Bengal. The efciency of the material was analysed using several parameters like catalytic loading, dye concentration, kinetic and scavenging experiments, photostability, efect of co-existing ions and recyclability. In addition, the material was subjected to optical studies and H2 generation, making it a highly versatile multifunctional material, exhibiting a degradation efciency of 94.12% in a short span of 150 min and a photocatalytic H2 generation efciency of 374 µmol ­g−1 through water splitting. With an immense potential, KTaO3 presents itself as a multifunctional catalyst that can be scaled up for a variety of industrial applications ranging from wastewater treatment to energy generation and storage.
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spelling Sumedha, H. N.Shashank, ManjunathaTeixeira, Sergio RibeiroPraveen, Beekanahalli MokshanathaNagaraju, Ganganagappa2022-10-03T04:49:02Z20222045-2322http://hdl.handle.net/10183/249617001147393Treatment of industrial wastewater is one of the biggest challenges that mankind is facing today to prevent environmental pollution and its associated adverse efects on human health. Environmentalists across the world have given a clarion call for dye degradation, wastewater treatment and their efective management in our surrounding habitats. Despite signifcant progress in the development of new water treatment technologies, new materials haven’t matured enough for large scale industrial applications. Hence, the development of new scalable and sustainable multifunctional materials having the potential to treat wastewater and generate energy is the need of the hour. In this direction, novel 3D-fower shaped KTaO3 (3D-F-KT) material has been synthesized using areca seed powder as a green fuel. This new material has been successfully applied for the treatment of industrial wastewater contaminated with Rose Bengal. The efciency of the material was analysed using several parameters like catalytic loading, dye concentration, kinetic and scavenging experiments, photostability, efect of co-existing ions and recyclability. In addition, the material was subjected to optical studies and H2 generation, making it a highly versatile multifunctional material, exhibiting a degradation efciency of 94.12% in a short span of 150 min and a photocatalytic H2 generation efciency of 374 µmol ­g−1 through water splitting. With an immense potential, KTaO3 presents itself as a multifunctional catalyst that can be scaled up for a variety of industrial applications ranging from wastewater treatment to energy generation and storage.application/pdfengScientific reports. London. Vol. 12 (June 2022), 10776, 16 p.FotocatáliseProdução de hidrogênioTratamento de efluentes industriaisNovel 3D‑fower shaped KTaO3 perovskite for highly efcient photocatalytic and ­H2 generation abilityEstrangeiroinfo:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersioninfo:eu-repo/semantics/openAccessreponame:Repositório Institucional da UFRGSinstname:Universidade Federal do Rio Grande do Sul (UFRGS)instacron:UFRGSTEXT001147393.pdf.txt001147393.pdf.txtExtracted Texttext/plain51272http://www.lume.ufrgs.br/bitstream/10183/249617/2/001147393.pdf.txt86dad7e6e456d2a9cc6709eda968663cMD52ORIGINAL001147393.pdfTexto completo (inglês)application/pdf10871359http://www.lume.ufrgs.br/bitstream/10183/249617/1/001147393.pdf2ee4bb52106264ce516700edf49de706MD5110183/2496172022-10-04 05:02:09.933322oai:www.lume.ufrgs.br:10183/249617Repositório de PublicaçõesPUBhttps://lume.ufrgs.br/oai/requestopendoar:2022-10-04T08:02:09Repositório Institucional da UFRGS - Universidade Federal do Rio Grande do Sul (UFRGS)false
dc.title.pt_BR.fl_str_mv Novel 3D‑fower shaped KTaO3 perovskite for highly efcient photocatalytic and ­H2 generation ability
title Novel 3D‑fower shaped KTaO3 perovskite for highly efcient photocatalytic and ­H2 generation ability
spellingShingle Novel 3D‑fower shaped KTaO3 perovskite for highly efcient photocatalytic and ­H2 generation ability
Sumedha, H. N.
Fotocatálise
Produção de hidrogênio
Tratamento de efluentes industriais
title_short Novel 3D‑fower shaped KTaO3 perovskite for highly efcient photocatalytic and ­H2 generation ability
title_full Novel 3D‑fower shaped KTaO3 perovskite for highly efcient photocatalytic and ­H2 generation ability
title_fullStr Novel 3D‑fower shaped KTaO3 perovskite for highly efcient photocatalytic and ­H2 generation ability
title_full_unstemmed Novel 3D‑fower shaped KTaO3 perovskite for highly efcient photocatalytic and ­H2 generation ability
title_sort Novel 3D‑fower shaped KTaO3 perovskite for highly efcient photocatalytic and ­H2 generation ability
author Sumedha, H. N.
author_facet Sumedha, H. N.
Shashank, Manjunatha
Teixeira, Sergio Ribeiro
Praveen, Beekanahalli Mokshanatha
Nagaraju, Ganganagappa
author_role author
author2 Shashank, Manjunatha
Teixeira, Sergio Ribeiro
Praveen, Beekanahalli Mokshanatha
Nagaraju, Ganganagappa
author2_role author
author
author
author
dc.contributor.author.fl_str_mv Sumedha, H. N.
Shashank, Manjunatha
Teixeira, Sergio Ribeiro
Praveen, Beekanahalli Mokshanatha
Nagaraju, Ganganagappa
dc.subject.por.fl_str_mv Fotocatálise
Produção de hidrogênio
Tratamento de efluentes industriais
topic Fotocatálise
Produção de hidrogênio
Tratamento de efluentes industriais
description Treatment of industrial wastewater is one of the biggest challenges that mankind is facing today to prevent environmental pollution and its associated adverse efects on human health. Environmentalists across the world have given a clarion call for dye degradation, wastewater treatment and their efective management in our surrounding habitats. Despite signifcant progress in the development of new water treatment technologies, new materials haven’t matured enough for large scale industrial applications. Hence, the development of new scalable and sustainable multifunctional materials having the potential to treat wastewater and generate energy is the need of the hour. In this direction, novel 3D-fower shaped KTaO3 (3D-F-KT) material has been synthesized using areca seed powder as a green fuel. This new material has been successfully applied for the treatment of industrial wastewater contaminated with Rose Bengal. The efciency of the material was analysed using several parameters like catalytic loading, dye concentration, kinetic and scavenging experiments, photostability, efect of co-existing ions and recyclability. In addition, the material was subjected to optical studies and H2 generation, making it a highly versatile multifunctional material, exhibiting a degradation efciency of 94.12% in a short span of 150 min and a photocatalytic H2 generation efciency of 374 µmol ­g−1 through water splitting. With an immense potential, KTaO3 presents itself as a multifunctional catalyst that can be scaled up for a variety of industrial applications ranging from wastewater treatment to energy generation and storage.
publishDate 2022
dc.date.accessioned.fl_str_mv 2022-10-03T04:49:02Z
dc.date.issued.fl_str_mv 2022
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dc.relation.ispartof.pt_BR.fl_str_mv Scientific reports. London. Vol. 12 (June 2022), 10776, 16 p.
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