Magnetocaloric effect of thin Terbium films
Autor(a) principal: | |
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Data de Publicação: | 2017 |
Outros Autores: | , , |
Tipo de documento: | Artigo |
Idioma: | eng |
Título da fonte: | Repositório Institucional da UFRN |
Texto Completo: | https://repositorio.ufrn.br/jspui/handle/123456789/29133 |
Resumo: | We report a theoretical study of the magnetocaloric effect of Terbium (Tb) thin films due to finite size and surface effects in the helimagnetic phase, corresponding to a temperature range from TC=219 K to TN=231 K, for external fields of the order of kOe. For a Tb thin film of 6 monolayers submitted to an applied field (ΔH=30 kOe, ΔH=50 kOe and ΔH = 70 kOe) we report a significative change in adiabatic temperature, ΔT/ΔH, near the Néel temperature, of the order ten times higher than that observed for Tb bulk. On the other hand, for small values of the magnetic field, large thickness effects are found. For external field strength around few kOe, we have found that the thermal caloric efficiency increases remarkably for ultrathin films. For an ultrathin film with 6 monolayers, we have found ΔT/ΔH = 43 K/T while for thicker films, with 20 monolayers, ΔT/ΔH = 22 K/T. Our results suggest that thin films of Tb are a promising material for magnetocaloric effect devices for applications at intermediate temperatures |
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Anselmo, Dory Hélio Aires de LimaMello, V. D.Vasconcelos, Manoel Silva deAlmeida, N. S.2020-06-04T00:51:31Z2020-06-04T00:51:31Z2017-12MELLO, V.D.; ANSELMO, D.H.A.L.; VASCONCELOS, M.S.; ALMEIDA, N.S.. Magnetocaloric effect of thin Terbium films. Solid State Communications, [s.l.], v. 268, p. 56-60, dez. 2017. Disponível em: https://www.sciencedirect.com/science/article/pii/S0038109817302879?via%3Dihub. Acesso em: 03 Jun 2020. http://dx.doi.org/10.1016/j.ssc.2017.09.004.0038-1098https://repositorio.ufrn.br/jspui/handle/123456789/2913310.1016/j.ssc.2017.09.004ElsevierAttribution 3.0 Brazilhttp://creativecommons.org/licenses/by/3.0/br/info:eu-repo/semantics/openAccessMagnetocaloric effectRare earthMagnetic measurementsThin filmsMagnetocaloric effect of thin Terbium filmsinfo:eu-repo/semantics/publishedVersioninfo:eu-repo/semantics/articleWe report a theoretical study of the magnetocaloric effect of Terbium (Tb) thin films due to finite size and surface effects in the helimagnetic phase, corresponding to a temperature range from TC=219 K to TN=231 K, for external fields of the order of kOe. For a Tb thin film of 6 monolayers submitted to an applied field (ΔH=30 kOe, ΔH=50 kOe and ΔH = 70 kOe) we report a significative change in adiabatic temperature, ΔT/ΔH, near the Néel temperature, of the order ten times higher than that observed for Tb bulk. On the other hand, for small values of the magnetic field, large thickness effects are found. For external field strength around few kOe, we have found that the thermal caloric efficiency increases remarkably for ultrathin films. For an ultrathin film with 6 monolayers, we have found ΔT/ΔH = 43 K/T while for thicker films, with 20 monolayers, ΔT/ΔH = 22 K/T. Our results suggest that thin films of Tb are a promising material for magnetocaloric effect devices for applications at intermediate temperaturesengreponame:Repositório Institucional da UFRNinstname:Universidade Federal do Rio Grande do Norte (UFRN)instacron:UFRNCC-LICENSElicense_rdflicense_rdfapplication/rdf+xml; charset=utf-8914https://repositorio.ufrn.br/bitstream/123456789/29133/2/license_rdf4d2950bda3d176f570a9f8b328dfbbefMD52ORIGINALMagnetocaloricEffect_Anselmo_2017.pdfMagnetocaloricEffect_Anselmo_2017.pdfapplication/pdf789109https://repositorio.ufrn.br/bitstream/123456789/29133/4/MagnetocaloricEffect_Anselmo_2017.pdf4791054abea4f30c44d22981e107b3b8MD54LICENSElicense.txtlicense.txttext/plain; charset=utf-81484https://repositorio.ufrn.br/bitstream/123456789/29133/5/license.txte9597aa2854d128fd968be5edc8a28d9MD55TEXTMagnetocaloricEffect_Anselmo_2017.pdf.txtMagnetocaloricEffect_Anselmo_2017.pdf.txtExtracted texttext/plain22449https://repositorio.ufrn.br/bitstream/123456789/29133/6/MagnetocaloricEffect_Anselmo_2017.pdf.txtb2b5741d305bba6dae4a4ab4ff0dff4aMD56THUMBNAILMagnetocaloricEffect_Anselmo_2017.pdf.jpgMagnetocaloricEffect_Anselmo_2017.pdf.jpgGenerated Thumbnailimage/jpeg1700https://repositorio.ufrn.br/bitstream/123456789/29133/7/MagnetocaloricEffect_Anselmo_2017.pdf.jpg77140a3075d9bcc141c4fba17428031aMD57123456789/291332020-06-07 04:36:16.031oai:https://repositorio.ufrn.br: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Repositório de PublicaçõesPUBhttp://repositorio.ufrn.br/oai/opendoar:2020-06-07T07:36:16Repositório Institucional da UFRN - Universidade Federal do Rio Grande do Norte (UFRN)false |
dc.title.pt_BR.fl_str_mv |
Magnetocaloric effect of thin Terbium films |
title |
Magnetocaloric effect of thin Terbium films |
spellingShingle |
Magnetocaloric effect of thin Terbium films Anselmo, Dory Hélio Aires de Lima Magnetocaloric effect Rare earth Magnetic measurements Thin films |
title_short |
Magnetocaloric effect of thin Terbium films |
title_full |
Magnetocaloric effect of thin Terbium films |
title_fullStr |
Magnetocaloric effect of thin Terbium films |
title_full_unstemmed |
Magnetocaloric effect of thin Terbium films |
title_sort |
Magnetocaloric effect of thin Terbium films |
author |
Anselmo, Dory Hélio Aires de Lima |
author_facet |
Anselmo, Dory Hélio Aires de Lima Mello, V. D. Vasconcelos, Manoel Silva de Almeida, N. S. |
author_role |
author |
author2 |
Mello, V. D. Vasconcelos, Manoel Silva de Almeida, N. S. |
author2_role |
author author author |
dc.contributor.author.fl_str_mv |
Anselmo, Dory Hélio Aires de Lima Mello, V. D. Vasconcelos, Manoel Silva de Almeida, N. S. |
dc.subject.por.fl_str_mv |
Magnetocaloric effect Rare earth Magnetic measurements Thin films |
topic |
Magnetocaloric effect Rare earth Magnetic measurements Thin films |
description |
We report a theoretical study of the magnetocaloric effect of Terbium (Tb) thin films due to finite size and surface effects in the helimagnetic phase, corresponding to a temperature range from TC=219 K to TN=231 K, for external fields of the order of kOe. For a Tb thin film of 6 monolayers submitted to an applied field (ΔH=30 kOe, ΔH=50 kOe and ΔH = 70 kOe) we report a significative change in adiabatic temperature, ΔT/ΔH, near the Néel temperature, of the order ten times higher than that observed for Tb bulk. On the other hand, for small values of the magnetic field, large thickness effects are found. For external field strength around few kOe, we have found that the thermal caloric efficiency increases remarkably for ultrathin films. For an ultrathin film with 6 monolayers, we have found ΔT/ΔH = 43 K/T while for thicker films, with 20 monolayers, ΔT/ΔH = 22 K/T. Our results suggest that thin films of Tb are a promising material for magnetocaloric effect devices for applications at intermediate temperatures |
publishDate |
2017 |
dc.date.issued.fl_str_mv |
2017-12 |
dc.date.accessioned.fl_str_mv |
2020-06-04T00:51:31Z |
dc.date.available.fl_str_mv |
2020-06-04T00:51:31Z |
dc.type.status.fl_str_mv |
info:eu-repo/semantics/publishedVersion |
dc.type.driver.fl_str_mv |
info:eu-repo/semantics/article |
format |
article |
status_str |
publishedVersion |
dc.identifier.citation.fl_str_mv |
MELLO, V.D.; ANSELMO, D.H.A.L.; VASCONCELOS, M.S.; ALMEIDA, N.S.. Magnetocaloric effect of thin Terbium films. Solid State Communications, [s.l.], v. 268, p. 56-60, dez. 2017. Disponível em: https://www.sciencedirect.com/science/article/pii/S0038109817302879?via%3Dihub. Acesso em: 03 Jun 2020. http://dx.doi.org/10.1016/j.ssc.2017.09.004. |
dc.identifier.uri.fl_str_mv |
https://repositorio.ufrn.br/jspui/handle/123456789/29133 |
dc.identifier.issn.none.fl_str_mv |
0038-1098 |
dc.identifier.doi.none.fl_str_mv |
10.1016/j.ssc.2017.09.004 |
identifier_str_mv |
MELLO, V.D.; ANSELMO, D.H.A.L.; VASCONCELOS, M.S.; ALMEIDA, N.S.. Magnetocaloric effect of thin Terbium films. Solid State Communications, [s.l.], v. 268, p. 56-60, dez. 2017. Disponível em: https://www.sciencedirect.com/science/article/pii/S0038109817302879?via%3Dihub. Acesso em: 03 Jun 2020. http://dx.doi.org/10.1016/j.ssc.2017.09.004. 0038-1098 10.1016/j.ssc.2017.09.004 |
url |
https://repositorio.ufrn.br/jspui/handle/123456789/29133 |
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eng |
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eng |
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Attribution 3.0 Brazil http://creativecommons.org/licenses/by/3.0/br/ info:eu-repo/semantics/openAccess |
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Attribution 3.0 Brazil http://creativecommons.org/licenses/by/3.0/br/ |
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openAccess |
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Elsevier |
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Elsevier |
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