Magnetocaloric effect of thin Terbium films

Detalhes bibliográficos
Autor(a) principal: Anselmo, Dory Hélio Aires de Lima
Data de Publicação: 2017
Outros Autores: Mello, V. D., Vasconcelos, Manoel Silva de, Almeida, N. S.
Tipo de documento: Artigo
Idioma: eng
Título da fonte: Repositório Institucional da UFRN
Texto Completo: https://repositorio.ufrn.br/jspui/handle/123456789/29133
Resumo: We report a theoretical study of the magnetocaloric effect of Terbium (Tb) thin films due to finite size and surface effects in the helimagnetic phase, corresponding to a temperature range from TC=219 K to TN=231 K, for external fields of the order of kOe. For a Tb thin film of 6 monolayers submitted to an applied field (ΔH=30 kOe, ΔH=50 kOe and ΔH = 70 kOe) we report a significative change in adiabatic temperature, ΔT/ΔH, near the Néel temperature, of the order ten times higher than that observed for Tb bulk. On the other hand, for small values of the magnetic field, large thickness effects are found. For external field strength around few kOe, we have found that the thermal caloric efficiency increases remarkably for ultrathin films. For an ultrathin film with 6 monolayers, we have found ΔT/ΔH = 43 K/T while for thicker films, with 20 monolayers, ΔT/ΔH = 22 K/T. Our results suggest that thin films of Tb are a promising material for magnetocaloric effect devices for applications at intermediate temperatures
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spelling Anselmo, Dory Hélio Aires de LimaMello, V. D.Vasconcelos, Manoel Silva deAlmeida, N. S.2020-06-04T00:51:31Z2020-06-04T00:51:31Z2017-12MELLO, V.D.; ANSELMO, D.H.A.L.; VASCONCELOS, M.S.; ALMEIDA, N.S.. Magnetocaloric effect of thin Terbium films. Solid State Communications, [s.l.], v. 268, p. 56-60, dez. 2017. Disponível em: https://www.sciencedirect.com/science/article/pii/S0038109817302879?via%3Dihub. Acesso em: 03 Jun 2020. http://dx.doi.org/10.1016/j.ssc.2017.09.004.0038-1098https://repositorio.ufrn.br/jspui/handle/123456789/2913310.1016/j.ssc.2017.09.004ElsevierAttribution 3.0 Brazilhttp://creativecommons.org/licenses/by/3.0/br/info:eu-repo/semantics/openAccessMagnetocaloric effectRare earthMagnetic measurementsThin filmsMagnetocaloric effect of thin Terbium filmsinfo:eu-repo/semantics/publishedVersioninfo:eu-repo/semantics/articleWe report a theoretical study of the magnetocaloric effect of Terbium (Tb) thin films due to finite size and surface effects in the helimagnetic phase, corresponding to a temperature range from TC=219 K to TN=231 K, for external fields of the order of kOe. For a Tb thin film of 6 monolayers submitted to an applied field (ΔH=30 kOe, ΔH=50 kOe and ΔH = 70 kOe) we report a significative change in adiabatic temperature, ΔT/ΔH, near the Néel temperature, of the order ten times higher than that observed for Tb bulk. On the other hand, for small values of the magnetic field, large thickness effects are found. For external field strength around few kOe, we have found that the thermal caloric efficiency increases remarkably for ultrathin films. For an ultrathin film with 6 monolayers, we have found ΔT/ΔH = 43 K/T while for thicker films, with 20 monolayers, ΔT/ΔH = 22 K/T. Our results suggest that thin films of Tb are a promising material for magnetocaloric effect devices for applications at intermediate temperaturesengreponame:Repositório Institucional da UFRNinstname:Universidade Federal do Rio Grande do Norte (UFRN)instacron:UFRNCC-LICENSElicense_rdflicense_rdfapplication/rdf+xml; charset=utf-8914https://repositorio.ufrn.br/bitstream/123456789/29133/2/license_rdf4d2950bda3d176f570a9f8b328dfbbefMD52ORIGINALMagnetocaloricEffect_Anselmo_2017.pdfMagnetocaloricEffect_Anselmo_2017.pdfapplication/pdf789109https://repositorio.ufrn.br/bitstream/123456789/29133/4/MagnetocaloricEffect_Anselmo_2017.pdf4791054abea4f30c44d22981e107b3b8MD54LICENSElicense.txtlicense.txttext/plain; charset=utf-81484https://repositorio.ufrn.br/bitstream/123456789/29133/5/license.txte9597aa2854d128fd968be5edc8a28d9MD55TEXTMagnetocaloricEffect_Anselmo_2017.pdf.txtMagnetocaloricEffect_Anselmo_2017.pdf.txtExtracted texttext/plain22449https://repositorio.ufrn.br/bitstream/123456789/29133/6/MagnetocaloricEffect_Anselmo_2017.pdf.txtb2b5741d305bba6dae4a4ab4ff0dff4aMD56THUMBNAILMagnetocaloricEffect_Anselmo_2017.pdf.jpgMagnetocaloricEffect_Anselmo_2017.pdf.jpgGenerated Thumbnailimage/jpeg1700https://repositorio.ufrn.br/bitstream/123456789/29133/7/MagnetocaloricEffect_Anselmo_2017.pdf.jpg77140a3075d9bcc141c4fba17428031aMD57123456789/291332020-06-07 04:36:16.031oai:https://repositorio.ufrn.br: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Repositório de PublicaçõesPUBhttp://repositorio.ufrn.br/oai/opendoar:2020-06-07T07:36:16Repositório Institucional da UFRN - Universidade Federal do Rio Grande do Norte (UFRN)false
dc.title.pt_BR.fl_str_mv Magnetocaloric effect of thin Terbium films
title Magnetocaloric effect of thin Terbium films
spellingShingle Magnetocaloric effect of thin Terbium films
Anselmo, Dory Hélio Aires de Lima
Magnetocaloric effect
Rare earth
Magnetic measurements
Thin films
title_short Magnetocaloric effect of thin Terbium films
title_full Magnetocaloric effect of thin Terbium films
title_fullStr Magnetocaloric effect of thin Terbium films
title_full_unstemmed Magnetocaloric effect of thin Terbium films
title_sort Magnetocaloric effect of thin Terbium films
author Anselmo, Dory Hélio Aires de Lima
author_facet Anselmo, Dory Hélio Aires de Lima
Mello, V. D.
Vasconcelos, Manoel Silva de
Almeida, N. S.
author_role author
author2 Mello, V. D.
Vasconcelos, Manoel Silva de
Almeida, N. S.
author2_role author
author
author
dc.contributor.author.fl_str_mv Anselmo, Dory Hélio Aires de Lima
Mello, V. D.
Vasconcelos, Manoel Silva de
Almeida, N. S.
dc.subject.por.fl_str_mv Magnetocaloric effect
Rare earth
Magnetic measurements
Thin films
topic Magnetocaloric effect
Rare earth
Magnetic measurements
Thin films
description We report a theoretical study of the magnetocaloric effect of Terbium (Tb) thin films due to finite size and surface effects in the helimagnetic phase, corresponding to a temperature range from TC=219 K to TN=231 K, for external fields of the order of kOe. For a Tb thin film of 6 monolayers submitted to an applied field (ΔH=30 kOe, ΔH=50 kOe and ΔH = 70 kOe) we report a significative change in adiabatic temperature, ΔT/ΔH, near the Néel temperature, of the order ten times higher than that observed for Tb bulk. On the other hand, for small values of the magnetic field, large thickness effects are found. For external field strength around few kOe, we have found that the thermal caloric efficiency increases remarkably for ultrathin films. For an ultrathin film with 6 monolayers, we have found ΔT/ΔH = 43 K/T while for thicker films, with 20 monolayers, ΔT/ΔH = 22 K/T. Our results suggest that thin films of Tb are a promising material for magnetocaloric effect devices for applications at intermediate temperatures
publishDate 2017
dc.date.issued.fl_str_mv 2017-12
dc.date.accessioned.fl_str_mv 2020-06-04T00:51:31Z
dc.date.available.fl_str_mv 2020-06-04T00:51:31Z
dc.type.status.fl_str_mv info:eu-repo/semantics/publishedVersion
dc.type.driver.fl_str_mv info:eu-repo/semantics/article
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dc.identifier.citation.fl_str_mv MELLO, V.D.; ANSELMO, D.H.A.L.; VASCONCELOS, M.S.; ALMEIDA, N.S.. Magnetocaloric effect of thin Terbium films. Solid State Communications, [s.l.], v. 268, p. 56-60, dez. 2017. Disponível em: https://www.sciencedirect.com/science/article/pii/S0038109817302879?via%3Dihub. Acesso em: 03 Jun 2020. http://dx.doi.org/10.1016/j.ssc.2017.09.004.
dc.identifier.uri.fl_str_mv https://repositorio.ufrn.br/jspui/handle/123456789/29133
dc.identifier.issn.none.fl_str_mv 0038-1098
dc.identifier.doi.none.fl_str_mv 10.1016/j.ssc.2017.09.004
identifier_str_mv MELLO, V.D.; ANSELMO, D.H.A.L.; VASCONCELOS, M.S.; ALMEIDA, N.S.. Magnetocaloric effect of thin Terbium films. Solid State Communications, [s.l.], v. 268, p. 56-60, dez. 2017. Disponível em: https://www.sciencedirect.com/science/article/pii/S0038109817302879?via%3Dihub. Acesso em: 03 Jun 2020. http://dx.doi.org/10.1016/j.ssc.2017.09.004.
0038-1098
10.1016/j.ssc.2017.09.004
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