Synthesis and structure determination via ultrafast electron diffraction of the new microporous zeolitic germanosilicate ITQ-62
Autor(a) principal: | |
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Data de Publicação: | 2018 |
Outros Autores: | , , , , , , , , |
Tipo de documento: | Artigo |
Idioma: | eng |
Título da fonte: | Repositório Institucional da UFRN |
Texto Completo: | https://repositorio.ufrn.br/jspui/handle/123456789/29585 |
Resumo: | Here, we present the synthesis and structure determination of the new zeolite ITQ-62. Its structure was determined via ultra-fast electron diffraction tomography and refined using powder XRD data of the calcined material. This new zeolite contains a tridirectional channel system of highly distorted 8-rings, as well as a monodirectional 12-ring channel system |
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Pergher, Sibele Berenice CastellãBieseki, LindianeSimancas, RaquelJorda, Jose L.Bereciartua, Pablo J.Cantín, AngelSimancas, JorgeValencia, SusanaRey, FernandoCorma, Avelino2020-07-13T18:37:24Z2020-07-13T18:37:24Z2018-01-26BIESEKI, Lindiane; SIMANCAS, Raquel; JORDÁ, Jose L.; BERECIARTUA, Pablo J.; CANTÍN, Ángel; SIMANCAS, Jorge; PERGHER, Sibele Berenice Castellã; VALENCIA, Susana; REY, Fernando; CORMA, Avelino. Synthesis and structure determination via ultra-fast electron diffraction of the new microporous zeolitic germanosilicate ITQ-62. Chemical Communications, [s.l.], v. 54, n. 17, p. 2122-2125, 2018.ISSN 1364-548X versão online. Disponível em: https://pubs.rsc.org/en/content/articlelanding/2018/CC/C7CC09240G#!divAbstract. Acesso em: 16 jul. 2020. http://dx.doi.org/10.1039/c7cc09240g.1359-7345 (print), 1364-548X (online)https://repositorio.ufrn.br/jspui/handle/123456789/2958510.1039/c7cc09240gRoyal Society of ChemistryAttribution-NonCommercial 3.0 Brazilhttp://creativecommons.org/licenses/by-nc/3.0/br/info:eu-repo/semantics/openAccessElectron diffractionZeolitic germanosilicateMicroporous zeoliticSynthesis and structure determination via ultrafast electron diffraction of the new microporous zeolitic germanosilicate ITQ-62info:eu-repo/semantics/publishedVersioninfo:eu-repo/semantics/articleHere, we present the synthesis and structure determination of the new zeolite ITQ-62. Its structure was determined via ultra-fast electron diffraction tomography and refined using powder XRD data of the calcined material. This new zeolite contains a tridirectional channel system of highly distorted 8-rings, as well as a monodirectional 12-ring channel systemengreponame:Repositório Institucional da UFRNinstname:Universidade Federal do Rio Grande do Norte (UFRN)instacron:UFRNORIGINALZeoliticGermanosilicateITQ62_Pergher_2018.pdfZeoliticGermanosilicateITQ62_Pergher_2018.pdfapplication/pdf2081664https://repositorio.ufrn.br/bitstream/123456789/29585/1/ZeoliticGermanosilicateITQ62_Pergher_2018.pdfc28c20c923956c51055842dee29402f0MD51CC-LICENSElicense_rdflicense_rdfapplication/rdf+xml; charset=utf-8920https://repositorio.ufrn.br/bitstream/123456789/29585/2/license_rdf728dfda2fa81b274c619d08d1dfc1a03MD52LICENSElicense.txtlicense.txttext/plain; charset=utf-81484https://repositorio.ufrn.br/bitstream/123456789/29585/3/license.txte9597aa2854d128fd968be5edc8a28d9MD53TEXTZeoliticGermanosilicateITQ62_Pergher_2018.pdf.txtZeoliticGermanosilicateITQ62_Pergher_2018.pdf.txtExtracted texttext/plain20390https://repositorio.ufrn.br/bitstream/123456789/29585/4/ZeoliticGermanosilicateITQ62_Pergher_2018.pdf.txtd99c1046ab26ebb453122291dba565eaMD54THUMBNAILZeoliticGermanosilicateITQ62_Pergher_2018.pdf.jpgZeoliticGermanosilicateITQ62_Pergher_2018.pdf.jpgGenerated Thumbnailimage/jpeg1907https://repositorio.ufrn.br/bitstream/123456789/29585/5/ZeoliticGermanosilicateITQ62_Pergher_2018.pdf.jpg76621718272ed9643dd15191e0dbebf0MD55123456789/295852021-02-15 19:00:33.164oai:https://repositorio.ufrn.br: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Repositório de PublicaçõesPUBhttp://repositorio.ufrn.br/oai/opendoar:2021-02-15T22:00:33Repositório Institucional da UFRN - Universidade Federal do Rio Grande do Norte (UFRN)false |
dc.title.pt_BR.fl_str_mv |
Synthesis and structure determination via ultrafast electron diffraction of the new microporous zeolitic germanosilicate ITQ-62 |
title |
Synthesis and structure determination via ultrafast electron diffraction of the new microporous zeolitic germanosilicate ITQ-62 |
spellingShingle |
Synthesis and structure determination via ultrafast electron diffraction of the new microporous zeolitic germanosilicate ITQ-62 Pergher, Sibele Berenice Castellã Electron diffraction Zeolitic germanosilicate Microporous zeolitic |
title_short |
Synthesis and structure determination via ultrafast electron diffraction of the new microporous zeolitic germanosilicate ITQ-62 |
title_full |
Synthesis and structure determination via ultrafast electron diffraction of the new microporous zeolitic germanosilicate ITQ-62 |
title_fullStr |
Synthesis and structure determination via ultrafast electron diffraction of the new microporous zeolitic germanosilicate ITQ-62 |
title_full_unstemmed |
Synthesis and structure determination via ultrafast electron diffraction of the new microporous zeolitic germanosilicate ITQ-62 |
title_sort |
Synthesis and structure determination via ultrafast electron diffraction of the new microporous zeolitic germanosilicate ITQ-62 |
author |
Pergher, Sibele Berenice Castellã |
author_facet |
Pergher, Sibele Berenice Castellã Bieseki, Lindiane Simancas, Raquel Jorda, Jose L. Bereciartua, Pablo J. Cantín, Angel Simancas, Jorge Valencia, Susana Rey, Fernando Corma, Avelino |
author_role |
author |
author2 |
Bieseki, Lindiane Simancas, Raquel Jorda, Jose L. Bereciartua, Pablo J. Cantín, Angel Simancas, Jorge Valencia, Susana Rey, Fernando Corma, Avelino |
author2_role |
author author author author author author author author author |
dc.contributor.author.fl_str_mv |
Pergher, Sibele Berenice Castellã Bieseki, Lindiane Simancas, Raquel Jorda, Jose L. Bereciartua, Pablo J. Cantín, Angel Simancas, Jorge Valencia, Susana Rey, Fernando Corma, Avelino |
dc.subject.por.fl_str_mv |
Electron diffraction Zeolitic germanosilicate Microporous zeolitic |
topic |
Electron diffraction Zeolitic germanosilicate Microporous zeolitic |
description |
Here, we present the synthesis and structure determination of the new zeolite ITQ-62. Its structure was determined via ultra-fast electron diffraction tomography and refined using powder XRD data of the calcined material. This new zeolite contains a tridirectional channel system of highly distorted 8-rings, as well as a monodirectional 12-ring channel system |
publishDate |
2018 |
dc.date.issued.fl_str_mv |
2018-01-26 |
dc.date.accessioned.fl_str_mv |
2020-07-13T18:37:24Z |
dc.date.available.fl_str_mv |
2020-07-13T18:37:24Z |
dc.type.status.fl_str_mv |
info:eu-repo/semantics/publishedVersion |
dc.type.driver.fl_str_mv |
info:eu-repo/semantics/article |
format |
article |
status_str |
publishedVersion |
dc.identifier.citation.fl_str_mv |
BIESEKI, Lindiane; SIMANCAS, Raquel; JORDÁ, Jose L.; BERECIARTUA, Pablo J.; CANTÍN, Ángel; SIMANCAS, Jorge; PERGHER, Sibele Berenice Castellã; VALENCIA, Susana; REY, Fernando; CORMA, Avelino. Synthesis and structure determination via ultra-fast electron diffraction of the new microporous zeolitic germanosilicate ITQ-62. Chemical Communications, [s.l.], v. 54, n. 17, p. 2122-2125, 2018.ISSN 1364-548X versão online. Disponível em: https://pubs.rsc.org/en/content/articlelanding/2018/CC/C7CC09240G#!divAbstract. Acesso em: 16 jul. 2020. http://dx.doi.org/10.1039/c7cc09240g. |
dc.identifier.uri.fl_str_mv |
https://repositorio.ufrn.br/jspui/handle/123456789/29585 |
dc.identifier.issn.none.fl_str_mv |
1359-7345 (print), 1364-548X (online) |
dc.identifier.doi.none.fl_str_mv |
10.1039/c7cc09240g |
identifier_str_mv |
BIESEKI, Lindiane; SIMANCAS, Raquel; JORDÁ, Jose L.; BERECIARTUA, Pablo J.; CANTÍN, Ángel; SIMANCAS, Jorge; PERGHER, Sibele Berenice Castellã; VALENCIA, Susana; REY, Fernando; CORMA, Avelino. Synthesis and structure determination via ultra-fast electron diffraction of the new microporous zeolitic germanosilicate ITQ-62. Chemical Communications, [s.l.], v. 54, n. 17, p. 2122-2125, 2018.ISSN 1364-548X versão online. Disponível em: https://pubs.rsc.org/en/content/articlelanding/2018/CC/C7CC09240G#!divAbstract. Acesso em: 16 jul. 2020. http://dx.doi.org/10.1039/c7cc09240g. 1359-7345 (print), 1364-548X (online) 10.1039/c7cc09240g |
url |
https://repositorio.ufrn.br/jspui/handle/123456789/29585 |
dc.language.iso.fl_str_mv |
eng |
language |
eng |
dc.rights.driver.fl_str_mv |
Attribution-NonCommercial 3.0 Brazil http://creativecommons.org/licenses/by-nc/3.0/br/ info:eu-repo/semantics/openAccess |
rights_invalid_str_mv |
Attribution-NonCommercial 3.0 Brazil http://creativecommons.org/licenses/by-nc/3.0/br/ |
eu_rights_str_mv |
openAccess |
dc.publisher.none.fl_str_mv |
Royal Society of Chemistry |
publisher.none.fl_str_mv |
Royal Society of Chemistry |
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reponame:Repositório Institucional da UFRN instname:Universidade Federal do Rio Grande do Norte (UFRN) instacron:UFRN |
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Universidade Federal do Rio Grande do Norte (UFRN) |
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UFRN |
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UFRN |
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