Synthesis, characterization, optical properties investigation and reusability photocatalyst capacity of AgCl‐xGO composite
Autor(a) principal: | |
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Data de Publicação: | 2019 |
Outros Autores: | , , , , |
Tipo de documento: | Artigo |
Idioma: | eng |
Título da fonte: | Repositório Institucional da UFRN |
Texto Completo: | https://repositorio.ufrn.br/handle/123456789/43753 |
Resumo: | In this work, we report the photocatalytic reuse study of AgCl-xGO composite with diferent GO concentration (x=1, 2, 4 and 8 mass %) to degrade cationic dyes. X-ray difraction and scanning electron microscopy analysis were performed to characterize the formation and morphological features of the synthesized AgCl-xGO composite. Raman spectroscopy and UV–Vis studies were used to characterize the AgCl optical properties. It was observed an Increasing in the photocatalytic efciency due to interface created by AgCl-GO composite associated to the impeding recombination of the electron–hole pair. Additionally, we notice that after 3 min of exposure to UV radiation, the AgCl-8%GO composite completely degraded the methylene blue dye while pure AgCl sample degraded 75.3%. The AgCl-8%GO composite showed stable photocatalytic activity even after the fourth cycle, indicating a high potential for application in consecutive photocatalytic cycles |
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Andrade Neto, Nivaldo Freire deOliveira, Y. G.Nascimento, José Heriberto Oliveira doCarvalho, Bruno Ribeiro deDelmonte, Maurício Roberto BomioMotta, Fabiana Villela da2021-10-08T18:20:50Z2021-10-08T18:20:50Z2019-07-20ANDRADE NETO, N. F.; OLIVEIRA, Y. G.; NASCIMENTO, J. H. O.; CARVALHO, B. R.; BOMIO, M. R. D.; MOTTA, F. V.. Synthesis, characterization, optical properties investigation and reusability photocatalyst capacity of AgCl-xGO composite. Journal of Materials Science: Materials in Electronics, [S.L.], v. 30, n. 16, p. 15214-15223, 20 jul. 2019. Disponível em: https://link.springer.com/article/10.1007%2Fs10854-019-01894-w. Acesso em: 22 abr. 2021. http://dx.doi.org/10.1007/s10854-019-01894-w.1573-482X0957-4522https://repositorio.ufrn.br/handle/123456789/4375310.1007/s10854-019-01894-wSpringerAttribution 3.0 Brazilhttp://creativecommons.org/licenses/by/3.0/br/info:eu-repo/semantics/openAccessReusability photocatalystSynthesis, characterization, optical properties investigation and reusability photocatalyst capacity of AgCl‐xGO compositeinfo:eu-repo/semantics/publishedVersioninfo:eu-repo/semantics/articleIn this work, we report the photocatalytic reuse study of AgCl-xGO composite with diferent GO concentration (x=1, 2, 4 and 8 mass %) to degrade cationic dyes. X-ray difraction and scanning electron microscopy analysis were performed to characterize the formation and morphological features of the synthesized AgCl-xGO composite. Raman spectroscopy and UV–Vis studies were used to characterize the AgCl optical properties. It was observed an Increasing in the photocatalytic efciency due to interface created by AgCl-GO composite associated to the impeding recombination of the electron–hole pair. Additionally, we notice that after 3 min of exposure to UV radiation, the AgCl-8%GO composite completely degraded the methylene blue dye while pure AgCl sample degraded 75.3%. The AgCl-8%GO composite showed stable photocatalytic activity even after the fourth cycle, indicating a high potential for application in consecutive photocatalytic cyclesengreponame:Repositório Institucional da UFRNinstname:Universidade Federal do Rio Grande do Norte (UFRN)instacron:UFRNORIGINALSynthesisCharacterizationOptical_BOMIO_2019.pdfSynthesisCharacterizationOptical_BOMIO_2019.pdfapplication/pdf4325872https://repositorio.ufrn.br/bitstream/123456789/43753/1/SynthesisCharacterizationOptical_BOMIO_2019.pdf062656e65aec4b424f62a63e00afd802MD51CC-LICENSElicense_rdflicense_rdfapplication/rdf+xml; charset=utf-8914https://repositorio.ufrn.br/bitstream/123456789/43753/2/license_rdf4d2950bda3d176f570a9f8b328dfbbefMD52LICENSElicense.txtlicense.txttext/plain; charset=utf-81484https://repositorio.ufrn.br/bitstream/123456789/43753/3/license.txte9597aa2854d128fd968be5edc8a28d9MD53123456789/437532021-10-08 15:20:51.149oai:https://repositorio.ufrn.br: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Repositório de PublicaçõesPUBhttp://repositorio.ufrn.br/oai/opendoar:2021-10-08T18:20:51Repositório Institucional da UFRN - Universidade Federal do Rio Grande do Norte (UFRN)false |
dc.title.pt_BR.fl_str_mv |
Synthesis, characterization, optical properties investigation and reusability photocatalyst capacity of AgCl‐xGO composite |
title |
Synthesis, characterization, optical properties investigation and reusability photocatalyst capacity of AgCl‐xGO composite |
spellingShingle |
Synthesis, characterization, optical properties investigation and reusability photocatalyst capacity of AgCl‐xGO composite Andrade Neto, Nivaldo Freire de Reusability photocatalyst |
title_short |
Synthesis, characterization, optical properties investigation and reusability photocatalyst capacity of AgCl‐xGO composite |
title_full |
Synthesis, characterization, optical properties investigation and reusability photocatalyst capacity of AgCl‐xGO composite |
title_fullStr |
Synthesis, characterization, optical properties investigation and reusability photocatalyst capacity of AgCl‐xGO composite |
title_full_unstemmed |
Synthesis, characterization, optical properties investigation and reusability photocatalyst capacity of AgCl‐xGO composite |
title_sort |
Synthesis, characterization, optical properties investigation and reusability photocatalyst capacity of AgCl‐xGO composite |
author |
Andrade Neto, Nivaldo Freire de |
author_facet |
Andrade Neto, Nivaldo Freire de Oliveira, Y. G. Nascimento, José Heriberto Oliveira do Carvalho, Bruno Ribeiro de Delmonte, Maurício Roberto Bomio Motta, Fabiana Villela da |
author_role |
author |
author2 |
Oliveira, Y. G. Nascimento, José Heriberto Oliveira do Carvalho, Bruno Ribeiro de Delmonte, Maurício Roberto Bomio Motta, Fabiana Villela da |
author2_role |
author author author author author |
dc.contributor.author.fl_str_mv |
Andrade Neto, Nivaldo Freire de Oliveira, Y. G. Nascimento, José Heriberto Oliveira do Carvalho, Bruno Ribeiro de Delmonte, Maurício Roberto Bomio Motta, Fabiana Villela da |
dc.subject.por.fl_str_mv |
Reusability photocatalyst |
topic |
Reusability photocatalyst |
description |
In this work, we report the photocatalytic reuse study of AgCl-xGO composite with diferent GO concentration (x=1, 2, 4 and 8 mass %) to degrade cationic dyes. X-ray difraction and scanning electron microscopy analysis were performed to characterize the formation and morphological features of the synthesized AgCl-xGO composite. Raman spectroscopy and UV–Vis studies were used to characterize the AgCl optical properties. It was observed an Increasing in the photocatalytic efciency due to interface created by AgCl-GO composite associated to the impeding recombination of the electron–hole pair. Additionally, we notice that after 3 min of exposure to UV radiation, the AgCl-8%GO composite completely degraded the methylene blue dye while pure AgCl sample degraded 75.3%. The AgCl-8%GO composite showed stable photocatalytic activity even after the fourth cycle, indicating a high potential for application in consecutive photocatalytic cycles |
publishDate |
2019 |
dc.date.issued.fl_str_mv |
2019-07-20 |
dc.date.accessioned.fl_str_mv |
2021-10-08T18:20:50Z |
dc.date.available.fl_str_mv |
2021-10-08T18:20:50Z |
dc.type.status.fl_str_mv |
info:eu-repo/semantics/publishedVersion |
dc.type.driver.fl_str_mv |
info:eu-repo/semantics/article |
format |
article |
status_str |
publishedVersion |
dc.identifier.citation.fl_str_mv |
ANDRADE NETO, N. F.; OLIVEIRA, Y. G.; NASCIMENTO, J. H. O.; CARVALHO, B. R.; BOMIO, M. R. D.; MOTTA, F. V.. Synthesis, characterization, optical properties investigation and reusability photocatalyst capacity of AgCl-xGO composite. Journal of Materials Science: Materials in Electronics, [S.L.], v. 30, n. 16, p. 15214-15223, 20 jul. 2019. Disponível em: https://link.springer.com/article/10.1007%2Fs10854-019-01894-w. Acesso em: 22 abr. 2021. http://dx.doi.org/10.1007/s10854-019-01894-w. |
dc.identifier.uri.fl_str_mv |
https://repositorio.ufrn.br/handle/123456789/43753 |
dc.identifier.issn.none.fl_str_mv |
1573-482X 0957-4522 |
dc.identifier.doi.none.fl_str_mv |
10.1007/s10854-019-01894-w |
identifier_str_mv |
ANDRADE NETO, N. F.; OLIVEIRA, Y. G.; NASCIMENTO, J. H. O.; CARVALHO, B. R.; BOMIO, M. R. D.; MOTTA, F. V.. Synthesis, characterization, optical properties investigation and reusability photocatalyst capacity of AgCl-xGO composite. Journal of Materials Science: Materials in Electronics, [S.L.], v. 30, n. 16, p. 15214-15223, 20 jul. 2019. Disponível em: https://link.springer.com/article/10.1007%2Fs10854-019-01894-w. Acesso em: 22 abr. 2021. http://dx.doi.org/10.1007/s10854-019-01894-w. 1573-482X 0957-4522 10.1007/s10854-019-01894-w |
url |
https://repositorio.ufrn.br/handle/123456789/43753 |
dc.language.iso.fl_str_mv |
eng |
language |
eng |
dc.rights.driver.fl_str_mv |
Attribution 3.0 Brazil http://creativecommons.org/licenses/by/3.0/br/ info:eu-repo/semantics/openAccess |
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Attribution 3.0 Brazil http://creativecommons.org/licenses/by/3.0/br/ |
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openAccess |
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Springer |
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Springer |
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