Synthesis, characterization, optical properties investigation and reusability photocatalyst capacity of AgCl‐xGO composite

Detalhes bibliográficos
Autor(a) principal: Andrade Neto, Nivaldo Freire de
Data de Publicação: 2019
Outros Autores: Oliveira, Y. G., Nascimento, José Heriberto Oliveira do, Carvalho, Bruno Ribeiro de, Delmonte, Maurício Roberto Bomio, Motta, Fabiana Villela da
Tipo de documento: Artigo
Idioma: eng
Título da fonte: Repositório Institucional da UFRN
Texto Completo: https://repositorio.ufrn.br/handle/123456789/43753
Resumo: In this work, we report the photocatalytic reuse study of AgCl-xGO composite with diferent GO concentration (x=1, 2, 4 and 8 mass %) to degrade cationic dyes. X-ray difraction and scanning electron microscopy analysis were performed to characterize the formation and morphological features of the synthesized AgCl-xGO composite. Raman spectroscopy and UV–Vis studies were used to characterize the AgCl optical properties. It was observed an Increasing in the photocatalytic efciency due to interface created by AgCl-GO composite associated to the impeding recombination of the electron–hole pair. Additionally, we notice that after 3 min of exposure to UV radiation, the AgCl-8%GO composite completely degraded the methylene blue dye while pure AgCl sample degraded 75.3%. The AgCl-8%GO composite showed stable photocatalytic activity even after the fourth cycle, indicating a high potential for application in consecutive photocatalytic cycles
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spelling Andrade Neto, Nivaldo Freire deOliveira, Y. G.Nascimento, José Heriberto Oliveira doCarvalho, Bruno Ribeiro deDelmonte, Maurício Roberto BomioMotta, Fabiana Villela da2021-10-08T18:20:50Z2021-10-08T18:20:50Z2019-07-20ANDRADE NETO, N. F.; OLIVEIRA, Y. G.; NASCIMENTO, J. H. O.; CARVALHO, B. R.; BOMIO, M. R. D.; MOTTA, F. V.. Synthesis, characterization, optical properties investigation and reusability photocatalyst capacity of AgCl-xGO composite. Journal of Materials Science: Materials in Electronics, [S.L.], v. 30, n. 16, p. 15214-15223, 20 jul. 2019. Disponível em: https://link.springer.com/article/10.1007%2Fs10854-019-01894-w. Acesso em: 22 abr. 2021. http://dx.doi.org/10.1007/s10854-019-01894-w.1573-482X0957-4522https://repositorio.ufrn.br/handle/123456789/4375310.1007/s10854-019-01894-wSpringerAttribution 3.0 Brazilhttp://creativecommons.org/licenses/by/3.0/br/info:eu-repo/semantics/openAccessReusability photocatalystSynthesis, characterization, optical properties investigation and reusability photocatalyst capacity of AgCl‐xGO compositeinfo:eu-repo/semantics/publishedVersioninfo:eu-repo/semantics/articleIn this work, we report the photocatalytic reuse study of AgCl-xGO composite with diferent GO concentration (x=1, 2, 4 and 8 mass %) to degrade cationic dyes. X-ray difraction and scanning electron microscopy analysis were performed to characterize the formation and morphological features of the synthesized AgCl-xGO composite. Raman spectroscopy and UV–Vis studies were used to characterize the AgCl optical properties. It was observed an Increasing in the photocatalytic efciency due to interface created by AgCl-GO composite associated to the impeding recombination of the electron–hole pair. Additionally, we notice that after 3 min of exposure to UV radiation, the AgCl-8%GO composite completely degraded the methylene blue dye while pure AgCl sample degraded 75.3%. The AgCl-8%GO composite showed stable photocatalytic activity even after the fourth cycle, indicating a high potential for application in consecutive photocatalytic cyclesengreponame:Repositório Institucional da UFRNinstname:Universidade Federal do Rio Grande do Norte (UFRN)instacron:UFRNORIGINALSynthesisCharacterizationOptical_BOMIO_2019.pdfSynthesisCharacterizationOptical_BOMIO_2019.pdfapplication/pdf4325872https://repositorio.ufrn.br/bitstream/123456789/43753/1/SynthesisCharacterizationOptical_BOMIO_2019.pdf062656e65aec4b424f62a63e00afd802MD51CC-LICENSElicense_rdflicense_rdfapplication/rdf+xml; charset=utf-8914https://repositorio.ufrn.br/bitstream/123456789/43753/2/license_rdf4d2950bda3d176f570a9f8b328dfbbefMD52LICENSElicense.txtlicense.txttext/plain; charset=utf-81484https://repositorio.ufrn.br/bitstream/123456789/43753/3/license.txte9597aa2854d128fd968be5edc8a28d9MD53123456789/437532021-10-08 15:20:51.149oai:https://repositorio.ufrn.br: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Repositório de PublicaçõesPUBhttp://repositorio.ufrn.br/oai/opendoar:2021-10-08T18:20:51Repositório Institucional da UFRN - Universidade Federal do Rio Grande do Norte (UFRN)false
dc.title.pt_BR.fl_str_mv Synthesis, characterization, optical properties investigation and reusability photocatalyst capacity of AgCl‐xGO composite
title Synthesis, characterization, optical properties investigation and reusability photocatalyst capacity of AgCl‐xGO composite
spellingShingle Synthesis, characterization, optical properties investigation and reusability photocatalyst capacity of AgCl‐xGO composite
Andrade Neto, Nivaldo Freire de
Reusability photocatalyst
title_short Synthesis, characterization, optical properties investigation and reusability photocatalyst capacity of AgCl‐xGO composite
title_full Synthesis, characterization, optical properties investigation and reusability photocatalyst capacity of AgCl‐xGO composite
title_fullStr Synthesis, characterization, optical properties investigation and reusability photocatalyst capacity of AgCl‐xGO composite
title_full_unstemmed Synthesis, characterization, optical properties investigation and reusability photocatalyst capacity of AgCl‐xGO composite
title_sort Synthesis, characterization, optical properties investigation and reusability photocatalyst capacity of AgCl‐xGO composite
author Andrade Neto, Nivaldo Freire de
author_facet Andrade Neto, Nivaldo Freire de
Oliveira, Y. G.
Nascimento, José Heriberto Oliveira do
Carvalho, Bruno Ribeiro de
Delmonte, Maurício Roberto Bomio
Motta, Fabiana Villela da
author_role author
author2 Oliveira, Y. G.
Nascimento, José Heriberto Oliveira do
Carvalho, Bruno Ribeiro de
Delmonte, Maurício Roberto Bomio
Motta, Fabiana Villela da
author2_role author
author
author
author
author
dc.contributor.author.fl_str_mv Andrade Neto, Nivaldo Freire de
Oliveira, Y. G.
Nascimento, José Heriberto Oliveira do
Carvalho, Bruno Ribeiro de
Delmonte, Maurício Roberto Bomio
Motta, Fabiana Villela da
dc.subject.por.fl_str_mv Reusability photocatalyst
topic Reusability photocatalyst
description In this work, we report the photocatalytic reuse study of AgCl-xGO composite with diferent GO concentration (x=1, 2, 4 and 8 mass %) to degrade cationic dyes. X-ray difraction and scanning electron microscopy analysis were performed to characterize the formation and morphological features of the synthesized AgCl-xGO composite. Raman spectroscopy and UV–Vis studies were used to characterize the AgCl optical properties. It was observed an Increasing in the photocatalytic efciency due to interface created by AgCl-GO composite associated to the impeding recombination of the electron–hole pair. Additionally, we notice that after 3 min of exposure to UV radiation, the AgCl-8%GO composite completely degraded the methylene blue dye while pure AgCl sample degraded 75.3%. The AgCl-8%GO composite showed stable photocatalytic activity even after the fourth cycle, indicating a high potential for application in consecutive photocatalytic cycles
publishDate 2019
dc.date.issued.fl_str_mv 2019-07-20
dc.date.accessioned.fl_str_mv 2021-10-08T18:20:50Z
dc.date.available.fl_str_mv 2021-10-08T18:20:50Z
dc.type.status.fl_str_mv info:eu-repo/semantics/publishedVersion
dc.type.driver.fl_str_mv info:eu-repo/semantics/article
format article
status_str publishedVersion
dc.identifier.citation.fl_str_mv ANDRADE NETO, N. F.; OLIVEIRA, Y. G.; NASCIMENTO, J. H. O.; CARVALHO, B. R.; BOMIO, M. R. D.; MOTTA, F. V.. Synthesis, characterization, optical properties investigation and reusability photocatalyst capacity of AgCl-xGO composite. Journal of Materials Science: Materials in Electronics, [S.L.], v. 30, n. 16, p. 15214-15223, 20 jul. 2019. Disponível em: https://link.springer.com/article/10.1007%2Fs10854-019-01894-w. Acesso em: 22 abr. 2021. http://dx.doi.org/10.1007/s10854-019-01894-w.
dc.identifier.uri.fl_str_mv https://repositorio.ufrn.br/handle/123456789/43753
dc.identifier.issn.none.fl_str_mv 1573-482X
0957-4522
dc.identifier.doi.none.fl_str_mv 10.1007/s10854-019-01894-w
identifier_str_mv ANDRADE NETO, N. F.; OLIVEIRA, Y. G.; NASCIMENTO, J. H. O.; CARVALHO, B. R.; BOMIO, M. R. D.; MOTTA, F. V.. Synthesis, characterization, optical properties investigation and reusability photocatalyst capacity of AgCl-xGO composite. Journal of Materials Science: Materials in Electronics, [S.L.], v. 30, n. 16, p. 15214-15223, 20 jul. 2019. Disponível em: https://link.springer.com/article/10.1007%2Fs10854-019-01894-w. Acesso em: 22 abr. 2021. http://dx.doi.org/10.1007/s10854-019-01894-w.
1573-482X
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