Evidence of magnetic polaronic states in La_{0.70}Sr_{0.30}Mn_{1-x}Fe_{x}O_{3} manganites
Autor(a) principal: | |
---|---|
Data de Publicação: | 2003 |
Outros Autores: | , , , , , , , , , |
Tipo de documento: | Artigo |
Idioma: | eng |
Título da fonte: | Repositório Institucional da UFRN |
Texto Completo: | https://repositorio.ufrn.br/handle/123456789/45360 |
Resumo: | We have performed x-ray, electrical resistivity, and Raman scattering measurements in La0.70Sr0.30Mn12xFexO3 manganites, with x varying from 0 to 0.40. The appearance of new peaks in the Raman spectra as the Fe content increases is attributed to either otherwise forbidden Raman modes that become active due to symmetry breaking effect or to the phonon density of states features, which arise due to a disorder-induced phenomenon. The softening of some phonon modes suggests the evidence of magnetic polaronic states in the insulating paramagnetic phase of these manganites. Our observations are discussed in connection with the x-ray diffraction and electrical resistivity data. |
id |
UFRN_bb823351ef757677276a419bb44ead3f |
---|---|
oai_identifier_str |
oai:https://repositorio.ufrn.br:123456789/45360 |
network_acronym_str |
UFRN |
network_name_str |
Repositório Institucional da UFRN |
repository_id_str |
|
spelling |
Araújo, José Humberto deSouza Filho, A. G.Faria, J. L. B.Guedes, I.Sasaki, José MarcosFreire, P. T. C.Mendes Filho, J.Xavier Jr, M. M.Cabral, Francisco de Assis OlímpioCosta, J. A. P. daFreire, V. N.2021-12-14T14:54:22Z2021-12-14T14:54:22Z2003-02-19SOUZA FILHO, A. G.; FARIA, J. L. B.; GUEDES, I.; SASAKI, J. M.; FREIRE, P. T. C.; FREIRE, V. N.; MENDES FILHO, J.; XAVIER JUNIOR, M. M.; CABRAL; F. A. O.; ARAÚJO, J. H. de; COSTA, J. A. P. da. Evidence of magnetic polaronic states in La0.70Sr0.30Mn1ÀxFexO3 manganites. Physical Review. B, Condensed Matter and Materials Physics, EUA, v. 67, n.052405, p. 052405, 2003. Disponivel em: https://journals.aps.org/prb/abstract/10.1103/PhysRevB.67.052405 Acesso em: 27 abr 2020.2469-9969 (online), 2469-9950 (print)https://repositorio.ufrn.br/handle/123456789/4536010.1103/PhysRevB.67.052405We have performed x-ray, electrical resistivity, and Raman scattering measurements in La0.70Sr0.30Mn12xFexO3 manganites, with x varying from 0 to 0.40. The appearance of new peaks in the Raman spectra as the Fe content increases is attributed to either otherwise forbidden Raman modes that become active due to symmetry breaking effect or to the phonon density of states features, which arise due to a disorder-induced phenomenon. The softening of some phonon modes suggests the evidence of magnetic polaronic states in the insulating paramagnetic phase of these manganites. Our observations are discussed in connection with the x-ray diffraction and electrical resistivity data.We have performed x-ray, electrical resistivity, and Raman scattering measurements in La0.70Sr0.30Mn12xFexO3 manganites, with x varying from 0 to 0.40. The appearance of new peaks in the Raman spectra as the Fe content increases is attributed to either otherwise forbidden Raman modes that become active due to symmetry breaking effect or to the phonon density of states features, which arise due to a disorder-induced phenomenon. The softening of some phonon modes suggests the evidence of magnetic polaronic states in the insulating paramagnetic phase of these manganites. Our observations are discussed in connection with the x-ray diffraction and electrical resistivity data.American Physical SocietyMagnetic polaronicManganitesEvidence of magnetic polaronic states in La_{0.70}Sr_{0.30}Mn_{1-x}Fe_{x}O_{3} manganitesinfo:eu-repo/semantics/publishedVersioninfo:eu-repo/semantics/articleengreponame:Repositório Institucional da UFRNinstname:Universidade Federal do Rio Grande do Norte (UFRN)instacron:UFRNinfo:eu-repo/semantics/openAccessORIGINALEvidenceOfMagneticPolaronicStates_2003.pdfEvidenceOfMagneticPolaronicStates_2003.pdfapplication/pdf63018https://repositorio.ufrn.br/bitstream/123456789/45360/1/EvidenceOfMagneticPolaronicStates_2003.pdf9eb7afd2ccc20faa8574c78155f120a9MD51LICENSElicense.txtlicense.txttext/plain; charset=utf-81484https://repositorio.ufrn.br/bitstream/123456789/45360/2/license.txte9597aa2854d128fd968be5edc8a28d9MD52123456789/453602021-12-14 12:01:56.853oai:https://repositorio.ufrn.br:123456789/45360Tk9OLUVYQ0xVU0lWRSBESVNUUklCVVRJT04gTElDRU5TRQoKCkJ5IHNpZ25pbmcgYW5kIGRlbGl2ZXJpbmcgdGhpcyBsaWNlbnNlLCBNci4gKGF1dGhvciBvciBjb3B5cmlnaHQgaG9sZGVyKToKCgphKSBHcmFudHMgdGhlIFVuaXZlcnNpZGFkZSBGZWRlcmFsIFJpbyBHcmFuZGUgZG8gTm9ydGUgdGhlIG5vbi1leGNsdXNpdmUgcmlnaHQgb2YKcmVwcm9kdWNlLCBjb252ZXJ0IChhcyBkZWZpbmVkIGJlbG93KSwgY29tbXVuaWNhdGUgYW5kIC8gb3IKZGlzdHJpYnV0ZSB0aGUgZGVsaXZlcmVkIGRvY3VtZW50IChpbmNsdWRpbmcgYWJzdHJhY3QgLyBhYnN0cmFjdCkgaW4KZGlnaXRhbCBvciBwcmludGVkIGZvcm1hdCBhbmQgaW4gYW55IG1lZGl1bS4KCmIpIERlY2xhcmVzIHRoYXQgdGhlIGRvY3VtZW50IHN1Ym1pdHRlZCBpcyBpdHMgb3JpZ2luYWwgd29yaywgYW5kIHRoYXQKeW91IGhhdmUgdGhlIHJpZ2h0IHRvIGdyYW50IHRoZSByaWdodHMgY29udGFpbmVkIGluIHRoaXMgbGljZW5zZS4gRGVjbGFyZXMKdGhhdCB0aGUgZGVsaXZlcnkgb2YgdGhlIGRvY3VtZW50IGRvZXMgbm90IGluZnJpbmdlLCBhcyBmYXIgYXMgaXQgaXMKdGhlIHJpZ2h0cyBvZiBhbnkgb3RoZXIgcGVyc29uIG9yIGVudGl0eS4KCmMpIElmIHRoZSBkb2N1bWVudCBkZWxpdmVyZWQgY29udGFpbnMgbWF0ZXJpYWwgd2hpY2ggZG9lcyBub3QKcmlnaHRzLCBkZWNsYXJlcyB0aGF0IGl0IGhhcyBvYnRhaW5lZCBhdXRob3JpemF0aW9uIGZyb20gdGhlIGhvbGRlciBvZiB0aGUKY29weXJpZ2h0IHRvIGdyYW50IHRoZSBVbml2ZXJzaWRhZGUgRmVkZXJhbCBkbyBSaW8gR3JhbmRlIGRvIE5vcnRlIHRoZSByaWdodHMgcmVxdWlyZWQgYnkgdGhpcyBsaWNlbnNlLCBhbmQgdGhhdCB0aGlzIG1hdGVyaWFsIHdob3NlIHJpZ2h0cyBhcmUgb2YKdGhpcmQgcGFydGllcyBpcyBjbGVhcmx5IGlkZW50aWZpZWQgYW5kIHJlY29nbml6ZWQgaW4gdGhlIHRleHQgb3IKY29udGVudCBvZiB0aGUgZG9jdW1lbnQgZGVsaXZlcmVkLgoKSWYgdGhlIGRvY3VtZW50IHN1Ym1pdHRlZCBpcyBiYXNlZCBvbiBmdW5kZWQgb3Igc3VwcG9ydGVkIHdvcmsKYnkgYW5vdGhlciBpbnN0aXR1dGlvbiBvdGhlciB0aGFuIHRoZSBVbml2ZXJzaWRhZGUgRmVkZXJhbCBkbyBSaW8gR3JhbmRlIGRvIE5vcnRlLCBkZWNsYXJlcyB0aGF0IGl0IGhhcyBmdWxmaWxsZWQgYW55IG9ibGlnYXRpb25zIHJlcXVpcmVkIGJ5IHRoZSByZXNwZWN0aXZlIGFncmVlbWVudCBvciBhZ3JlZW1lbnQuCgpUaGUgVW5pdmVyc2lkYWRlIEZlZGVyYWwgZG8gUmlvIEdyYW5kZSBkbyBOb3J0ZSB3aWxsIGNsZWFybHkgaWRlbnRpZnkgaXRzIG5hbWUgKHMpIGFzIHRoZSBhdXRob3IgKHMpIG9yIGhvbGRlciAocykgb2YgdGhlIGRvY3VtZW50J3MgcmlnaHRzCmRlbGl2ZXJlZCwgYW5kIHdpbGwgbm90IG1ha2UgYW55IGNoYW5nZXMsIG90aGVyIHRoYW4gdGhvc2UgcGVybWl0dGVkIGJ5CnRoaXMgbGljZW5zZQo=Repositório de PublicaçõesPUBhttp://repositorio.ufrn.br/oai/opendoar:2021-12-14T15:01:56Repositório Institucional da UFRN - Universidade Federal do Rio Grande do Norte (UFRN)false |
dc.title.pt_BR.fl_str_mv |
Evidence of magnetic polaronic states in La_{0.70}Sr_{0.30}Mn_{1-x}Fe_{x}O_{3} manganites |
title |
Evidence of magnetic polaronic states in La_{0.70}Sr_{0.30}Mn_{1-x}Fe_{x}O_{3} manganites |
spellingShingle |
Evidence of magnetic polaronic states in La_{0.70}Sr_{0.30}Mn_{1-x}Fe_{x}O_{3} manganites Araújo, José Humberto de Magnetic polaronic Manganites |
title_short |
Evidence of magnetic polaronic states in La_{0.70}Sr_{0.30}Mn_{1-x}Fe_{x}O_{3} manganites |
title_full |
Evidence of magnetic polaronic states in La_{0.70}Sr_{0.30}Mn_{1-x}Fe_{x}O_{3} manganites |
title_fullStr |
Evidence of magnetic polaronic states in La_{0.70}Sr_{0.30}Mn_{1-x}Fe_{x}O_{3} manganites |
title_full_unstemmed |
Evidence of magnetic polaronic states in La_{0.70}Sr_{0.30}Mn_{1-x}Fe_{x}O_{3} manganites |
title_sort |
Evidence of magnetic polaronic states in La_{0.70}Sr_{0.30}Mn_{1-x}Fe_{x}O_{3} manganites |
author |
Araújo, José Humberto de |
author_facet |
Araújo, José Humberto de Souza Filho, A. G. Faria, J. L. B. Guedes, I. Sasaki, José Marcos Freire, P. T. C. Mendes Filho, J. Xavier Jr, M. M. Cabral, Francisco de Assis Olímpio Costa, J. A. P. da Freire, V. N. |
author_role |
author |
author2 |
Souza Filho, A. G. Faria, J. L. B. Guedes, I. Sasaki, José Marcos Freire, P. T. C. Mendes Filho, J. Xavier Jr, M. M. Cabral, Francisco de Assis Olímpio Costa, J. A. P. da Freire, V. N. |
author2_role |
author author author author author author author author author author |
dc.contributor.author.fl_str_mv |
Araújo, José Humberto de Souza Filho, A. G. Faria, J. L. B. Guedes, I. Sasaki, José Marcos Freire, P. T. C. Mendes Filho, J. Xavier Jr, M. M. Cabral, Francisco de Assis Olímpio Costa, J. A. P. da Freire, V. N. |
dc.subject.por.fl_str_mv |
Magnetic polaronic Manganites |
topic |
Magnetic polaronic Manganites |
description |
We have performed x-ray, electrical resistivity, and Raman scattering measurements in La0.70Sr0.30Mn12xFexO3 manganites, with x varying from 0 to 0.40. The appearance of new peaks in the Raman spectra as the Fe content increases is attributed to either otherwise forbidden Raman modes that become active due to symmetry breaking effect or to the phonon density of states features, which arise due to a disorder-induced phenomenon. The softening of some phonon modes suggests the evidence of magnetic polaronic states in the insulating paramagnetic phase of these manganites. Our observations are discussed in connection with the x-ray diffraction and electrical resistivity data. |
publishDate |
2003 |
dc.date.issued.fl_str_mv |
2003-02-19 |
dc.date.accessioned.fl_str_mv |
2021-12-14T14:54:22Z |
dc.date.available.fl_str_mv |
2021-12-14T14:54:22Z |
dc.type.status.fl_str_mv |
info:eu-repo/semantics/publishedVersion |
dc.type.driver.fl_str_mv |
info:eu-repo/semantics/article |
format |
article |
status_str |
publishedVersion |
dc.identifier.citation.fl_str_mv |
SOUZA FILHO, A. G.; FARIA, J. L. B.; GUEDES, I.; SASAKI, J. M.; FREIRE, P. T. C.; FREIRE, V. N.; MENDES FILHO, J.; XAVIER JUNIOR, M. M.; CABRAL; F. A. O.; ARAÚJO, J. H. de; COSTA, J. A. P. da. Evidence of magnetic polaronic states in La0.70Sr0.30Mn1ÀxFexO3 manganites. Physical Review. B, Condensed Matter and Materials Physics, EUA, v. 67, n.052405, p. 052405, 2003. Disponivel em: https://journals.aps.org/prb/abstract/10.1103/PhysRevB.67.052405 Acesso em: 27 abr 2020. |
dc.identifier.uri.fl_str_mv |
https://repositorio.ufrn.br/handle/123456789/45360 |
dc.identifier.issn.none.fl_str_mv |
2469-9969 (online), 2469-9950 (print) |
dc.identifier.doi.none.fl_str_mv |
10.1103/PhysRevB.67.052405 |
identifier_str_mv |
SOUZA FILHO, A. G.; FARIA, J. L. B.; GUEDES, I.; SASAKI, J. M.; FREIRE, P. T. C.; FREIRE, V. N.; MENDES FILHO, J.; XAVIER JUNIOR, M. M.; CABRAL; F. A. O.; ARAÚJO, J. H. de; COSTA, J. A. P. da. Evidence of magnetic polaronic states in La0.70Sr0.30Mn1ÀxFexO3 manganites. Physical Review. B, Condensed Matter and Materials Physics, EUA, v. 67, n.052405, p. 052405, 2003. Disponivel em: https://journals.aps.org/prb/abstract/10.1103/PhysRevB.67.052405 Acesso em: 27 abr 2020. 2469-9969 (online), 2469-9950 (print) 10.1103/PhysRevB.67.052405 |
url |
https://repositorio.ufrn.br/handle/123456789/45360 |
dc.language.iso.fl_str_mv |
eng |
language |
eng |
dc.rights.driver.fl_str_mv |
info:eu-repo/semantics/openAccess |
eu_rights_str_mv |
openAccess |
dc.publisher.none.fl_str_mv |
American Physical Society |
publisher.none.fl_str_mv |
American Physical Society |
dc.source.none.fl_str_mv |
reponame:Repositório Institucional da UFRN instname:Universidade Federal do Rio Grande do Norte (UFRN) instacron:UFRN |
instname_str |
Universidade Federal do Rio Grande do Norte (UFRN) |
instacron_str |
UFRN |
institution |
UFRN |
reponame_str |
Repositório Institucional da UFRN |
collection |
Repositório Institucional da UFRN |
bitstream.url.fl_str_mv |
https://repositorio.ufrn.br/bitstream/123456789/45360/1/EvidenceOfMagneticPolaronicStates_2003.pdf https://repositorio.ufrn.br/bitstream/123456789/45360/2/license.txt |
bitstream.checksum.fl_str_mv |
9eb7afd2ccc20faa8574c78155f120a9 e9597aa2854d128fd968be5edc8a28d9 |
bitstream.checksumAlgorithm.fl_str_mv |
MD5 MD5 |
repository.name.fl_str_mv |
Repositório Institucional da UFRN - Universidade Federal do Rio Grande do Norte (UFRN) |
repository.mail.fl_str_mv |
|
_version_ |
1814833060294688768 |