Fractionation of green coconut fiber using sequential hydrothermal/alkaline pretreatments and amberlite XAD-7HP resin
Autor(a) principal: | |
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Data de Publicação: | 2019 |
Outros Autores: | , , , , , , |
Tipo de documento: | Artigo |
Idioma: | eng |
Título da fonte: | Repositório Institucional da UFRN |
Texto Completo: | https://repositorio.ufrn.br/handle/123456789/45164 |
Resumo: | The fractionation of agroindustrial and forest residues is a premise of the biorefinery concept. Thus, the present study focuses on pretreatments (hydrothermal and alkaline) and detoxification processes in order to transform green coconut fiber (GCF) into cellulose-rich material, dye biosorbent, bioactive phenolic compounds, lignin and arabinoxylan. The adsorption onto Amberlite XAD-7HP resin allowed the best recovery of phenolic compounds from hydrothermal pretreatment liquor, which presented potent antioxidant activities such as inhibition of hydroxyl and superoxide radicals of 77.05% and 76.88%, respectively. Acid precipitation was effective to recover 41.23% of the initial lignin content from alkaline pretreatment liquor. The detoxified hydrothermal pretreatment liquor was used as an additional source of glucose, increasing the final concentration of ethanol by 79.6% in simultaneous saccharification and fermentation of delignified GCF. Using delignified GCF as biosorbent, made it possible to obtain a static adsorption capacity of 200 mg of methylene blue dye per gram of biosorbent and good recyclability in dynamic experiments. Therefore, the proposed methodology guarantees a practical way of manufacturing value-added products from lignocellulosic materials |
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Souza, Domingos Fabiano de SantanaPadilha, Carlos Eduardo de AraújoNogueira, Cleitiane da CostaOliveira Filho, Marcos AntônioSousa Júnior, Francisco Canindé deAssis, Cristiane Fernandes deOliveira, Jackson Araújo deSantos, Everaldo Silvino dos2021-12-03T19:05:18Z2021-12-03T19:05:18Z2019-12PADILHA, Carlos Eduardo de Araújo; NOGUEIRA, Cleitiane da Costa; OLIVEIRA FILHO, Marcos Antônio; SOUSA JÚNIOR, Francisco Canindé de; ASSIS, Cristiane Fernandes de; SOUZA, Domingos Fabiano de Santana; OLIVEIRA, Jackson Araújo de; SANTOS, Everaldo Silvino dos. Fractionation of green coconut fiber using sequential hydrothermal/alkaline pretreatments and Amberlite XAD-7HP resin. Journal Of Environmental Chemical Engineering, [S.L.], v. 7, n. 6, p. 103474, dez. 2019. Elsevier BV. http://dx.doi.org/10.1016/j.jece.2019.103474. Disponível em <https://www.sciencedirect.com/science/article/abs/pii/S2213343719305974?via%3Dihub>. Acesso em 05 nov. 2021.2213-3437https://repositorio.ufrn.br/handle/123456789/4516410.1016/j.jece.2019.103474ElsevierAlkaline pretreatmentEthanol productionPhenolic compoundsLignin recoveryArabinoxylan recoveryMethylene blue dyeFractionation of green coconut fiber using sequential hydrothermal/alkaline pretreatments and amberlite XAD-7HP resininfo:eu-repo/semantics/publishedVersioninfo:eu-repo/semantics/articleThe fractionation of agroindustrial and forest residues is a premise of the biorefinery concept. Thus, the present study focuses on pretreatments (hydrothermal and alkaline) and detoxification processes in order to transform green coconut fiber (GCF) into cellulose-rich material, dye biosorbent, bioactive phenolic compounds, lignin and arabinoxylan. The adsorption onto Amberlite XAD-7HP resin allowed the best recovery of phenolic compounds from hydrothermal pretreatment liquor, which presented potent antioxidant activities such as inhibition of hydroxyl and superoxide radicals of 77.05% and 76.88%, respectively. Acid precipitation was effective to recover 41.23% of the initial lignin content from alkaline pretreatment liquor. The detoxified hydrothermal pretreatment liquor was used as an additional source of glucose, increasing the final concentration of ethanol by 79.6% in simultaneous saccharification and fermentation of delignified GCF. Using delignified GCF as biosorbent, made it possible to obtain a static adsorption capacity of 200 mg of methylene blue dye per gram of biosorbent and good recyclability in dynamic experiments. Therefore, the proposed methodology guarantees a practical way of manufacturing value-added products from lignocellulosic materialsengreponame:Repositório Institucional da UFRNinstname:Universidade Federal do Rio Grande do Norte (UFRN)instacron:UFRNinfo:eu-repo/semantics/openAccessCC-LICENSElicense_rdflicense_rdfapplication/rdf+xml; charset=utf-8914https://repositorio.ufrn.br/bitstream/123456789/45164/2/license_rdf4d2950bda3d176f570a9f8b328dfbbefMD52LICENSElicense.txtlicense.txttext/plain; charset=utf-81484https://repositorio.ufrn.br/bitstream/123456789/45164/3/license.txte9597aa2854d128fd968be5edc8a28d9MD53123456789/451642023-02-14 16:11:39.306oai:https://repositorio.ufrn.br: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Repositório de PublicaçõesPUBhttp://repositorio.ufrn.br/oai/opendoar:2023-02-14T19:11:39Repositório Institucional da UFRN - Universidade Federal do Rio Grande do Norte (UFRN)false |
dc.title.pt_BR.fl_str_mv |
Fractionation of green coconut fiber using sequential hydrothermal/alkaline pretreatments and amberlite XAD-7HP resin |
title |
Fractionation of green coconut fiber using sequential hydrothermal/alkaline pretreatments and amberlite XAD-7HP resin |
spellingShingle |
Fractionation of green coconut fiber using sequential hydrothermal/alkaline pretreatments and amberlite XAD-7HP resin Souza, Domingos Fabiano de Santana Alkaline pretreatment Ethanol production Phenolic compounds Lignin recovery Arabinoxylan recovery Methylene blue dye |
title_short |
Fractionation of green coconut fiber using sequential hydrothermal/alkaline pretreatments and amberlite XAD-7HP resin |
title_full |
Fractionation of green coconut fiber using sequential hydrothermal/alkaline pretreatments and amberlite XAD-7HP resin |
title_fullStr |
Fractionation of green coconut fiber using sequential hydrothermal/alkaline pretreatments and amberlite XAD-7HP resin |
title_full_unstemmed |
Fractionation of green coconut fiber using sequential hydrothermal/alkaline pretreatments and amberlite XAD-7HP resin |
title_sort |
Fractionation of green coconut fiber using sequential hydrothermal/alkaline pretreatments and amberlite XAD-7HP resin |
author |
Souza, Domingos Fabiano de Santana |
author_facet |
Souza, Domingos Fabiano de Santana Padilha, Carlos Eduardo de Araújo Nogueira, Cleitiane da Costa Oliveira Filho, Marcos Antônio Sousa Júnior, Francisco Canindé de Assis, Cristiane Fernandes de Oliveira, Jackson Araújo de Santos, Everaldo Silvino dos |
author_role |
author |
author2 |
Padilha, Carlos Eduardo de Araújo Nogueira, Cleitiane da Costa Oliveira Filho, Marcos Antônio Sousa Júnior, Francisco Canindé de Assis, Cristiane Fernandes de Oliveira, Jackson Araújo de Santos, Everaldo Silvino dos |
author2_role |
author author author author author author author |
dc.contributor.author.fl_str_mv |
Souza, Domingos Fabiano de Santana Padilha, Carlos Eduardo de Araújo Nogueira, Cleitiane da Costa Oliveira Filho, Marcos Antônio Sousa Júnior, Francisco Canindé de Assis, Cristiane Fernandes de Oliveira, Jackson Araújo de Santos, Everaldo Silvino dos |
dc.subject.por.fl_str_mv |
Alkaline pretreatment Ethanol production Phenolic compounds Lignin recovery Arabinoxylan recovery Methylene blue dye |
topic |
Alkaline pretreatment Ethanol production Phenolic compounds Lignin recovery Arabinoxylan recovery Methylene blue dye |
description |
The fractionation of agroindustrial and forest residues is a premise of the biorefinery concept. Thus, the present study focuses on pretreatments (hydrothermal and alkaline) and detoxification processes in order to transform green coconut fiber (GCF) into cellulose-rich material, dye biosorbent, bioactive phenolic compounds, lignin and arabinoxylan. The adsorption onto Amberlite XAD-7HP resin allowed the best recovery of phenolic compounds from hydrothermal pretreatment liquor, which presented potent antioxidant activities such as inhibition of hydroxyl and superoxide radicals of 77.05% and 76.88%, respectively. Acid precipitation was effective to recover 41.23% of the initial lignin content from alkaline pretreatment liquor. The detoxified hydrothermal pretreatment liquor was used as an additional source of glucose, increasing the final concentration of ethanol by 79.6% in simultaneous saccharification and fermentation of delignified GCF. Using delignified GCF as biosorbent, made it possible to obtain a static adsorption capacity of 200 mg of methylene blue dye per gram of biosorbent and good recyclability in dynamic experiments. Therefore, the proposed methodology guarantees a practical way of manufacturing value-added products from lignocellulosic materials |
publishDate |
2019 |
dc.date.issued.fl_str_mv |
2019-12 |
dc.date.accessioned.fl_str_mv |
2021-12-03T19:05:18Z |
dc.date.available.fl_str_mv |
2021-12-03T19:05:18Z |
dc.type.status.fl_str_mv |
info:eu-repo/semantics/publishedVersion |
dc.type.driver.fl_str_mv |
info:eu-repo/semantics/article |
format |
article |
status_str |
publishedVersion |
dc.identifier.citation.fl_str_mv |
PADILHA, Carlos Eduardo de Araújo; NOGUEIRA, Cleitiane da Costa; OLIVEIRA FILHO, Marcos Antônio; SOUSA JÚNIOR, Francisco Canindé de; ASSIS, Cristiane Fernandes de; SOUZA, Domingos Fabiano de Santana; OLIVEIRA, Jackson Araújo de; SANTOS, Everaldo Silvino dos. Fractionation of green coconut fiber using sequential hydrothermal/alkaline pretreatments and Amberlite XAD-7HP resin. Journal Of Environmental Chemical Engineering, [S.L.], v. 7, n. 6, p. 103474, dez. 2019. Elsevier BV. http://dx.doi.org/10.1016/j.jece.2019.103474. Disponível em <https://www.sciencedirect.com/science/article/abs/pii/S2213343719305974?via%3Dihub>. Acesso em 05 nov. 2021. |
dc.identifier.uri.fl_str_mv |
https://repositorio.ufrn.br/handle/123456789/45164 |
dc.identifier.issn.none.fl_str_mv |
2213-3437 |
dc.identifier.doi.none.fl_str_mv |
10.1016/j.jece.2019.103474 |
identifier_str_mv |
PADILHA, Carlos Eduardo de Araújo; NOGUEIRA, Cleitiane da Costa; OLIVEIRA FILHO, Marcos Antônio; SOUSA JÚNIOR, Francisco Canindé de; ASSIS, Cristiane Fernandes de; SOUZA, Domingos Fabiano de Santana; OLIVEIRA, Jackson Araújo de; SANTOS, Everaldo Silvino dos. Fractionation of green coconut fiber using sequential hydrothermal/alkaline pretreatments and Amberlite XAD-7HP resin. Journal Of Environmental Chemical Engineering, [S.L.], v. 7, n. 6, p. 103474, dez. 2019. Elsevier BV. http://dx.doi.org/10.1016/j.jece.2019.103474. Disponível em <https://www.sciencedirect.com/science/article/abs/pii/S2213343719305974?via%3Dihub>. Acesso em 05 nov. 2021. 2213-3437 10.1016/j.jece.2019.103474 |
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https://repositorio.ufrn.br/handle/123456789/45164 |
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