Effects of the mean free path and relaxation in a model for the aggregation of particles in superfluid media
Autor(a) principal: | |
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Data de Publicação: | 2009 |
Outros Autores: | , |
Tipo de documento: | Artigo |
Idioma: | eng |
Título da fonte: | LOCUS Repositório Institucional da UFV |
Texto Completo: | https://doi.org/10.1063/1.3158359 http://www.locus.ufv.br/handle/123456789/19329 |
Resumo: | In this paper, we study a two-dimensional model for the growth of molecular clusters in superfluid helium at low temperature. In the model, particles of diameter a follow random ballistic moves of length ␦ = a − 256a. Upon attachment on the cluster surface, particles allow one-step relaxation to the nearest twofold coordinated site. Average coordination numbers of particles show that in the presence of relaxation the screening for incoming particles modifies the microscopic structure of the cluster. These results are in qualitative agreement with experimental aggregation of methane in He droplets, in which large abundance of fully coordinated sites is observed. The average coordination number increases with ␦ , showing that screening is relevant when relaxation is present. As the cluster size increases, the corresponding structure clusters changes from a compact to a fractal, typical of ballistic and diffusion limited models, respectively. A scaling ansatz describing the crossover between the two regimes is proposed. |
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Effects of the mean free path and relaxation in a model for the aggregation of particles in superfluid mediaAggregation of particlesSuperfluid mediaIn this paper, we study a two-dimensional model for the growth of molecular clusters in superfluid helium at low temperature. In the model, particles of diameter a follow random ballistic moves of length ␦ = a − 256a. Upon attachment on the cluster surface, particles allow one-step relaxation to the nearest twofold coordinated site. Average coordination numbers of particles show that in the presence of relaxation the screening for incoming particles modifies the microscopic structure of the cluster. These results are in qualitative agreement with experimental aggregation of methane in He droplets, in which large abundance of fully coordinated sites is observed. The average coordination number increases with ␦ , showing that screening is relevant when relaxation is present. As the cluster size increases, the corresponding structure clusters changes from a compact to a fractal, typical of ballistic and diffusion limited models, respectively. A scaling ansatz describing the crossover between the two regimes is proposed.The Journal of Chemical Physics2018-05-04T13:23:57Z2018-05-04T13:23:57Z2009-06-30info:eu-repo/semantics/publishedVersioninfo:eu-repo/semantics/articlepdfapplication/pdf10897690https://doi.org/10.1063/1.3158359http://www.locus.ufv.br/handle/123456789/19329engv. 130, n. 24, p. 2445061- 2445066 , June 2009American Institute of Physicsinfo:eu-repo/semantics/openAccessAlves, S. G.Vilesov, A. F.Ferreira Jr., S. C.reponame:LOCUS Repositório Institucional da UFVinstname:Universidade Federal de Viçosa (UFV)instacron:UFV2024-07-12T06:46:46Zoai:locus.ufv.br:123456789/19329Repositório InstitucionalPUBhttps://www.locus.ufv.br/oai/requestfabiojreis@ufv.bropendoar:21452024-07-12T06:46:46LOCUS Repositório Institucional da UFV - Universidade Federal de Viçosa (UFV)false |
dc.title.none.fl_str_mv |
Effects of the mean free path and relaxation in a model for the aggregation of particles in superfluid media |
title |
Effects of the mean free path and relaxation in a model for the aggregation of particles in superfluid media |
spellingShingle |
Effects of the mean free path and relaxation in a model for the aggregation of particles in superfluid media Alves, S. G. Aggregation of particles Superfluid media |
title_short |
Effects of the mean free path and relaxation in a model for the aggregation of particles in superfluid media |
title_full |
Effects of the mean free path and relaxation in a model for the aggregation of particles in superfluid media |
title_fullStr |
Effects of the mean free path and relaxation in a model for the aggregation of particles in superfluid media |
title_full_unstemmed |
Effects of the mean free path and relaxation in a model for the aggregation of particles in superfluid media |
title_sort |
Effects of the mean free path and relaxation in a model for the aggregation of particles in superfluid media |
author |
Alves, S. G. |
author_facet |
Alves, S. G. Vilesov, A. F. Ferreira Jr., S. C. |
author_role |
author |
author2 |
Vilesov, A. F. Ferreira Jr., S. C. |
author2_role |
author author |
dc.contributor.author.fl_str_mv |
Alves, S. G. Vilesov, A. F. Ferreira Jr., S. C. |
dc.subject.por.fl_str_mv |
Aggregation of particles Superfluid media |
topic |
Aggregation of particles Superfluid media |
description |
In this paper, we study a two-dimensional model for the growth of molecular clusters in superfluid helium at low temperature. In the model, particles of diameter a follow random ballistic moves of length ␦ = a − 256a. Upon attachment on the cluster surface, particles allow one-step relaxation to the nearest twofold coordinated site. Average coordination numbers of particles show that in the presence of relaxation the screening for incoming particles modifies the microscopic structure of the cluster. These results are in qualitative agreement with experimental aggregation of methane in He droplets, in which large abundance of fully coordinated sites is observed. The average coordination number increases with ␦ , showing that screening is relevant when relaxation is present. As the cluster size increases, the corresponding structure clusters changes from a compact to a fractal, typical of ballistic and diffusion limited models, respectively. A scaling ansatz describing the crossover between the two regimes is proposed. |
publishDate |
2009 |
dc.date.none.fl_str_mv |
2009-06-30 2018-05-04T13:23:57Z 2018-05-04T13:23:57Z |
dc.type.status.fl_str_mv |
info:eu-repo/semantics/publishedVersion |
dc.type.driver.fl_str_mv |
info:eu-repo/semantics/article |
format |
article |
status_str |
publishedVersion |
dc.identifier.uri.fl_str_mv |
10897690 https://doi.org/10.1063/1.3158359 http://www.locus.ufv.br/handle/123456789/19329 |
identifier_str_mv |
10897690 |
url |
https://doi.org/10.1063/1.3158359 http://www.locus.ufv.br/handle/123456789/19329 |
dc.language.iso.fl_str_mv |
eng |
language |
eng |
dc.relation.none.fl_str_mv |
v. 130, n. 24, p. 2445061- 2445066 , June 2009 |
dc.rights.driver.fl_str_mv |
American Institute of Physics info:eu-repo/semantics/openAccess |
rights_invalid_str_mv |
American Institute of Physics |
eu_rights_str_mv |
openAccess |
dc.format.none.fl_str_mv |
pdf application/pdf |
dc.publisher.none.fl_str_mv |
The Journal of Chemical Physics |
publisher.none.fl_str_mv |
The Journal of Chemical Physics |
dc.source.none.fl_str_mv |
reponame:LOCUS Repositório Institucional da UFV instname:Universidade Federal de Viçosa (UFV) instacron:UFV |
instname_str |
Universidade Federal de Viçosa (UFV) |
instacron_str |
UFV |
institution |
UFV |
reponame_str |
LOCUS Repositório Institucional da UFV |
collection |
LOCUS Repositório Institucional da UFV |
repository.name.fl_str_mv |
LOCUS Repositório Institucional da UFV - Universidade Federal de Viçosa (UFV) |
repository.mail.fl_str_mv |
fabiojreis@ufv.br |
_version_ |
1817559869034594304 |