Effects of the mean free path and relaxation in a model for the aggregation of particles in superfluid media

Detalhes bibliográficos
Autor(a) principal: Alves, S. G.
Data de Publicação: 2009
Outros Autores: Vilesov, A. F., Ferreira Jr., S. C.
Tipo de documento: Artigo
Idioma: eng
Título da fonte: LOCUS Repositório Institucional da UFV
Texto Completo: https://doi.org/10.1063/1.3158359
http://www.locus.ufv.br/handle/123456789/19329
Resumo: In this paper, we study a two-dimensional model for the growth of molecular clusters in superfluid helium at low temperature. In the model, particles of diameter a follow random ballistic moves of length ␦ = a − 256a. Upon attachment on the cluster surface, particles allow one-step relaxation to the nearest twofold coordinated site. Average coordination numbers of particles show that in the presence of relaxation the screening for incoming particles modifies the microscopic structure of the cluster. These results are in qualitative agreement with experimental aggregation of methane in He droplets, in which large abundance of fully coordinated sites is observed. The average coordination number increases with ␦ , showing that screening is relevant when relaxation is present. As the cluster size increases, the corresponding structure clusters changes from a compact to a fractal, typical of ballistic and diffusion limited models, respectively. A scaling ansatz describing the crossover between the two regimes is proposed.
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spelling Effects of the mean free path and relaxation in a model for the aggregation of particles in superfluid mediaAggregation of particlesSuperfluid mediaIn this paper, we study a two-dimensional model for the growth of molecular clusters in superfluid helium at low temperature. In the model, particles of diameter a follow random ballistic moves of length ␦ = a − 256a. Upon attachment on the cluster surface, particles allow one-step relaxation to the nearest twofold coordinated site. Average coordination numbers of particles show that in the presence of relaxation the screening for incoming particles modifies the microscopic structure of the cluster. These results are in qualitative agreement with experimental aggregation of methane in He droplets, in which large abundance of fully coordinated sites is observed. The average coordination number increases with ␦ , showing that screening is relevant when relaxation is present. As the cluster size increases, the corresponding structure clusters changes from a compact to a fractal, typical of ballistic and diffusion limited models, respectively. A scaling ansatz describing the crossover between the two regimes is proposed.The Journal of Chemical Physics2018-05-04T13:23:57Z2018-05-04T13:23:57Z2009-06-30info:eu-repo/semantics/publishedVersioninfo:eu-repo/semantics/articlepdfapplication/pdf10897690https://doi.org/10.1063/1.3158359http://www.locus.ufv.br/handle/123456789/19329engv. 130, n. 24, p. 2445061- 2445066 , June 2009American Institute of Physicsinfo:eu-repo/semantics/openAccessAlves, S. G.Vilesov, A. F.Ferreira Jr., S. C.reponame:LOCUS Repositório Institucional da UFVinstname:Universidade Federal de Viçosa (UFV)instacron:UFV2024-07-12T06:46:46Zoai:locus.ufv.br:123456789/19329Repositório InstitucionalPUBhttps://www.locus.ufv.br/oai/requestfabiojreis@ufv.bropendoar:21452024-07-12T06:46:46LOCUS Repositório Institucional da UFV - Universidade Federal de Viçosa (UFV)false
dc.title.none.fl_str_mv Effects of the mean free path and relaxation in a model for the aggregation of particles in superfluid media
title Effects of the mean free path and relaxation in a model for the aggregation of particles in superfluid media
spellingShingle Effects of the mean free path and relaxation in a model for the aggregation of particles in superfluid media
Alves, S. G.
Aggregation of particles
Superfluid media
title_short Effects of the mean free path and relaxation in a model for the aggregation of particles in superfluid media
title_full Effects of the mean free path and relaxation in a model for the aggregation of particles in superfluid media
title_fullStr Effects of the mean free path and relaxation in a model for the aggregation of particles in superfluid media
title_full_unstemmed Effects of the mean free path and relaxation in a model for the aggregation of particles in superfluid media
title_sort Effects of the mean free path and relaxation in a model for the aggregation of particles in superfluid media
author Alves, S. G.
author_facet Alves, S. G.
Vilesov, A. F.
Ferreira Jr., S. C.
author_role author
author2 Vilesov, A. F.
Ferreira Jr., S. C.
author2_role author
author
dc.contributor.author.fl_str_mv Alves, S. G.
Vilesov, A. F.
Ferreira Jr., S. C.
dc.subject.por.fl_str_mv Aggregation of particles
Superfluid media
topic Aggregation of particles
Superfluid media
description In this paper, we study a two-dimensional model for the growth of molecular clusters in superfluid helium at low temperature. In the model, particles of diameter a follow random ballistic moves of length ␦ = a − 256a. Upon attachment on the cluster surface, particles allow one-step relaxation to the nearest twofold coordinated site. Average coordination numbers of particles show that in the presence of relaxation the screening for incoming particles modifies the microscopic structure of the cluster. These results are in qualitative agreement with experimental aggregation of methane in He droplets, in which large abundance of fully coordinated sites is observed. The average coordination number increases with ␦ , showing that screening is relevant when relaxation is present. As the cluster size increases, the corresponding structure clusters changes from a compact to a fractal, typical of ballistic and diffusion limited models, respectively. A scaling ansatz describing the crossover between the two regimes is proposed.
publishDate 2009
dc.date.none.fl_str_mv 2009-06-30
2018-05-04T13:23:57Z
2018-05-04T13:23:57Z
dc.type.status.fl_str_mv info:eu-repo/semantics/publishedVersion
dc.type.driver.fl_str_mv info:eu-repo/semantics/article
format article
status_str publishedVersion
dc.identifier.uri.fl_str_mv 10897690
https://doi.org/10.1063/1.3158359
http://www.locus.ufv.br/handle/123456789/19329
identifier_str_mv 10897690
url https://doi.org/10.1063/1.3158359
http://www.locus.ufv.br/handle/123456789/19329
dc.language.iso.fl_str_mv eng
language eng
dc.relation.none.fl_str_mv v. 130, n. 24, p. 2445061- 2445066 , June 2009
dc.rights.driver.fl_str_mv American Institute of Physics
info:eu-repo/semantics/openAccess
rights_invalid_str_mv American Institute of Physics
eu_rights_str_mv openAccess
dc.format.none.fl_str_mv pdf
application/pdf
dc.publisher.none.fl_str_mv The Journal of Chemical Physics
publisher.none.fl_str_mv The Journal of Chemical Physics
dc.source.none.fl_str_mv reponame:LOCUS Repositório Institucional da UFV
instname:Universidade Federal de Viçosa (UFV)
instacron:UFV
instname_str Universidade Federal de Viçosa (UFV)
instacron_str UFV
institution UFV
reponame_str LOCUS Repositório Institucional da UFV
collection LOCUS Repositório Institucional da UFV
repository.name.fl_str_mv LOCUS Repositório Institucional da UFV - Universidade Federal de Viçosa (UFV)
repository.mail.fl_str_mv fabiojreis@ufv.br
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