Structure and photoluminescence properties of PbO–Bi2O3–Ga2O3 glass-ceramics containing silver nanoparticles, free lead and bismuth ions

Detalhes bibliográficos
Autor(a) principal: Naranjo-Riaño, Luz Patricia
Data de Publicação: 2023
Outros Autores: Oliveira, Nathália T.C., Echeverry, Camilo E., Kassab, Luciana R.P. [UNESP], de Araújo, Cid B.
Tipo de documento: Artigo
Idioma: eng
Título da fonte: Repositório Institucional da UNESP
Texto Completo: http://dx.doi.org/10.1016/j.optmat.2023.113929
http://hdl.handle.net/11449/247465
Resumo: We report the synthesis, structural characterization, and optical properties of PbO–Bi2O3–Ga2O3 glass-ceramics (GCs) containing PbO and Bi2O3 crystallites, free lead (Pb2+) and bismuth (Bi3+) ions, and silver nanoparticles (Ag-NPs). The samples were prepared by applying the melt-quenching method followed by suitable heat-treatment of the samples. Transmission Electron Microscopy, X-ray diffraction, linear optical absorption, and photoluminescence (PL) were the techniques applied to characterize the samples. When the samples were excited at 330 nm a large PL intensity, due to the Pb2+ and Bi3+, is observed. Moreover, large PL intensity enhancement of about 1000% for the samples containing Ag-NPs is observed in comparison with the PL intensity from the samples without Ag-NPs. This is the first time that this behavior is reported for a GCs based on heavy-metal oxides. The potential of this class of materials for photonic applications is discussed.
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spelling Structure and photoluminescence properties of PbO–Bi2O3–Ga2O3 glass-ceramics containing silver nanoparticles, free lead and bismuth ionsHeavy metal oxide glass-ceramicsLuminescent Pb2+ and Bi3+ ionsPbO and Bi2O3 crystalsSilver nanoparticlesWe report the synthesis, structural characterization, and optical properties of PbO–Bi2O3–Ga2O3 glass-ceramics (GCs) containing PbO and Bi2O3 crystallites, free lead (Pb2+) and bismuth (Bi3+) ions, and silver nanoparticles (Ag-NPs). The samples were prepared by applying the melt-quenching method followed by suitable heat-treatment of the samples. Transmission Electron Microscopy, X-ray diffraction, linear optical absorption, and photoluminescence (PL) were the techniques applied to characterize the samples. When the samples were excited at 330 nm a large PL intensity, due to the Pb2+ and Bi3+, is observed. Moreover, large PL intensity enhancement of about 1000% for the samples containing Ag-NPs is observed in comparison with the PL intensity from the samples without Ag-NPs. This is the first time that this behavior is reported for a GCs based on heavy-metal oxides. The potential of this class of materials for photonic applications is discussed.Coordenação de Aperfeiçoamento de Pessoal de Nível Superior (CAPES)Conselho Nacional de Desenvolvimento Científico e Tecnológico (CNPq)Fundação de Amparo à Ciência e Tecnologia do Estado de PernambucoFacultad de Ciencias Naturales y Matemáticas Universidad de Ibagué, Carrera 22 Calle 67 B/AmbaláPrograma de Pós-Graduação em Ciência de Materiais Universidade Federal de Pernambuco, PEDepartamento de Física Universidade Federal do Ceara, CEFaculdade de Tecnologia de São Paulo CEETEPS/UNESP, SPDepartamento de Física Universidade Federal de Pernambuco, PEFaculdade de Tecnologia de São Paulo CEETEPS/UNESP, SPUniversidad de IbaguéUniversidade Federal de Pernambuco (UFPE)Universidade Federal do CearaUniversidade Estadual Paulista (UNESP)Naranjo-Riaño, Luz PatriciaOliveira, Nathália T.C.Echeverry, Camilo E.Kassab, Luciana R.P. [UNESP]de Araújo, Cid B.2023-07-29T13:16:50Z2023-07-29T13:16:50Z2023-07-01info:eu-repo/semantics/publishedVersioninfo:eu-repo/semantics/articlehttp://dx.doi.org/10.1016/j.optmat.2023.113929Optical Materials, v. 141.0925-3467http://hdl.handle.net/11449/24746510.1016/j.optmat.2023.1139292-s2.0-85160434424Scopusreponame:Repositório Institucional da UNESPinstname:Universidade Estadual Paulista (UNESP)instacron:UNESPengOptical Materialsinfo:eu-repo/semantics/openAccess2023-07-29T13:16:50Zoai:repositorio.unesp.br:11449/247465Repositório InstitucionalPUBhttp://repositorio.unesp.br/oai/requestopendoar:29462024-08-05T18:39:15.184694Repositório Institucional da UNESP - Universidade Estadual Paulista (UNESP)false
dc.title.none.fl_str_mv Structure and photoluminescence properties of PbO–Bi2O3–Ga2O3 glass-ceramics containing silver nanoparticles, free lead and bismuth ions
title Structure and photoluminescence properties of PbO–Bi2O3–Ga2O3 glass-ceramics containing silver nanoparticles, free lead and bismuth ions
spellingShingle Structure and photoluminescence properties of PbO–Bi2O3–Ga2O3 glass-ceramics containing silver nanoparticles, free lead and bismuth ions
Naranjo-Riaño, Luz Patricia
Heavy metal oxide glass-ceramics
Luminescent Pb2+ and Bi3+ ions
PbO and Bi2O3 crystals
Silver nanoparticles
title_short Structure and photoluminescence properties of PbO–Bi2O3–Ga2O3 glass-ceramics containing silver nanoparticles, free lead and bismuth ions
title_full Structure and photoluminescence properties of PbO–Bi2O3–Ga2O3 glass-ceramics containing silver nanoparticles, free lead and bismuth ions
title_fullStr Structure and photoluminescence properties of PbO–Bi2O3–Ga2O3 glass-ceramics containing silver nanoparticles, free lead and bismuth ions
title_full_unstemmed Structure and photoluminescence properties of PbO–Bi2O3–Ga2O3 glass-ceramics containing silver nanoparticles, free lead and bismuth ions
title_sort Structure and photoluminescence properties of PbO–Bi2O3–Ga2O3 glass-ceramics containing silver nanoparticles, free lead and bismuth ions
author Naranjo-Riaño, Luz Patricia
author_facet Naranjo-Riaño, Luz Patricia
Oliveira, Nathália T.C.
Echeverry, Camilo E.
Kassab, Luciana R.P. [UNESP]
de Araújo, Cid B.
author_role author
author2 Oliveira, Nathália T.C.
Echeverry, Camilo E.
Kassab, Luciana R.P. [UNESP]
de Araújo, Cid B.
author2_role author
author
author
author
dc.contributor.none.fl_str_mv Universidad de Ibagué
Universidade Federal de Pernambuco (UFPE)
Universidade Federal do Ceara
Universidade Estadual Paulista (UNESP)
dc.contributor.author.fl_str_mv Naranjo-Riaño, Luz Patricia
Oliveira, Nathália T.C.
Echeverry, Camilo E.
Kassab, Luciana R.P. [UNESP]
de Araújo, Cid B.
dc.subject.por.fl_str_mv Heavy metal oxide glass-ceramics
Luminescent Pb2+ and Bi3+ ions
PbO and Bi2O3 crystals
Silver nanoparticles
topic Heavy metal oxide glass-ceramics
Luminescent Pb2+ and Bi3+ ions
PbO and Bi2O3 crystals
Silver nanoparticles
description We report the synthesis, structural characterization, and optical properties of PbO–Bi2O3–Ga2O3 glass-ceramics (GCs) containing PbO and Bi2O3 crystallites, free lead (Pb2+) and bismuth (Bi3+) ions, and silver nanoparticles (Ag-NPs). The samples were prepared by applying the melt-quenching method followed by suitable heat-treatment of the samples. Transmission Electron Microscopy, X-ray diffraction, linear optical absorption, and photoluminescence (PL) were the techniques applied to characterize the samples. When the samples were excited at 330 nm a large PL intensity, due to the Pb2+ and Bi3+, is observed. Moreover, large PL intensity enhancement of about 1000% for the samples containing Ag-NPs is observed in comparison with the PL intensity from the samples without Ag-NPs. This is the first time that this behavior is reported for a GCs based on heavy-metal oxides. The potential of this class of materials for photonic applications is discussed.
publishDate 2023
dc.date.none.fl_str_mv 2023-07-29T13:16:50Z
2023-07-29T13:16:50Z
2023-07-01
dc.type.status.fl_str_mv info:eu-repo/semantics/publishedVersion
dc.type.driver.fl_str_mv info:eu-repo/semantics/article
format article
status_str publishedVersion
dc.identifier.uri.fl_str_mv http://dx.doi.org/10.1016/j.optmat.2023.113929
Optical Materials, v. 141.
0925-3467
http://hdl.handle.net/11449/247465
10.1016/j.optmat.2023.113929
2-s2.0-85160434424
url http://dx.doi.org/10.1016/j.optmat.2023.113929
http://hdl.handle.net/11449/247465
identifier_str_mv Optical Materials, v. 141.
0925-3467
10.1016/j.optmat.2023.113929
2-s2.0-85160434424
dc.language.iso.fl_str_mv eng
language eng
dc.relation.none.fl_str_mv Optical Materials
dc.rights.driver.fl_str_mv info:eu-repo/semantics/openAccess
eu_rights_str_mv openAccess
dc.source.none.fl_str_mv Scopus
reponame:Repositório Institucional da UNESP
instname:Universidade Estadual Paulista (UNESP)
instacron:UNESP
instname_str Universidade Estadual Paulista (UNESP)
instacron_str UNESP
institution UNESP
reponame_str Repositório Institucional da UNESP
collection Repositório Institucional da UNESP
repository.name.fl_str_mv Repositório Institucional da UNESP - Universidade Estadual Paulista (UNESP)
repository.mail.fl_str_mv
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