Functionalized Mesoporous Silicon Nanomaterials in Inorganic Soil Pollution Research: Opportunities for Soil Protection and Advanced Chemical Imaging

Detalhes bibliográficos
Autor(a) principal: Yang, Jia-Wei
Data de Publicação: 2020
Outros Autores: Fang, Wen, Williams, Paul N., McGrath, John W., Eismann, Carlos Eduardo [UNESP], Menegário, Amauri Antonio [UNESP], Elias, Lucas Pellegrini [UNESP], Luo, Jun, Xu, Yingjian
Tipo de documento: Artigo
Idioma: eng
Título da fonte: Repositório Institucional da UNESP
Texto Completo: http://dx.doi.org/10.1007/s40726-020-00152-6
http://hdl.handle.net/11449/201931
Resumo: “Innovative actions towards a pollution free-planet” is a goal of the United Nations Environment Assembly (UNEA). Aided by both the Food and Agricultural Organisation (FAO) and its Global Soil Partnership under the 3rd UNEA resolution, a consensus from > 170 countries have agreed a need for accelerated action and collaboration to combat soil pollution. This initiative has been tasked to find new and improved solutions to prevent and reduce soil pollution, and it is in this context that this review provides an updated perspective on an emerging technology platform that has already provided demonstrable utility for measurement, mapping, and monitoring of toxic trace elements (TTEs) in soils, in addition to the entrapment, removal, and remediation of pollutant sources. In this article, the development and characteristics of functionalized mesoporous silica nanomaterials (FMSN) will be discussed and compared with other common metal scavenging materials. The chemistries of the common functionalizations will be reviewed, in addition to providing an outlook on some of the future directions/applications of FMSN. The use of FMSN in soil will be considered with some specific case studies focusing on Hg and As. Finally, the advantages and developments of FMSN in the widely used diffusive gradients-in-thin films (DGT) technique will be discussed, in particular, its advantages as a DGT substrate for integration with oxygen planar optodes in multilayer systems that provide 2D mapping of metal pollutant fluxes at submillimeter resolution, which can be used to measure detailed sediment-water fluxes as well as soil-root interactions, to predict plant uptake and bioavailability.
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spelling Functionalized Mesoporous Silicon Nanomaterials in Inorganic Soil Pollution Research: Opportunities for Soil Protection and Advanced Chemical ImagingDiffusive gradient in thin films (DGT)Functional mesoporous silicon nanomaterials (FMSN)Heavy metalsSoil pollutionX-ray fluorescence spectrometry (XRF)“Innovative actions towards a pollution free-planet” is a goal of the United Nations Environment Assembly (UNEA). Aided by both the Food and Agricultural Organisation (FAO) and its Global Soil Partnership under the 3rd UNEA resolution, a consensus from > 170 countries have agreed a need for accelerated action and collaboration to combat soil pollution. This initiative has been tasked to find new and improved solutions to prevent and reduce soil pollution, and it is in this context that this review provides an updated perspective on an emerging technology platform that has already provided demonstrable utility for measurement, mapping, and monitoring of toxic trace elements (TTEs) in soils, in addition to the entrapment, removal, and remediation of pollutant sources. In this article, the development and characteristics of functionalized mesoporous silica nanomaterials (FMSN) will be discussed and compared with other common metal scavenging materials. The chemistries of the common functionalizations will be reviewed, in addition to providing an outlook on some of the future directions/applications of FMSN. The use of FMSN in soil will be considered with some specific case studies focusing on Hg and As. Finally, the advantages and developments of FMSN in the widely used diffusive gradients-in-thin films (DGT) technique will be discussed, in particular, its advantages as a DGT substrate for integration with oxygen planar optodes in multilayer systems that provide 2D mapping of metal pollutant fluxes at submillimeter resolution, which can be used to measure detailed sediment-water fluxes as well as soil-root interactions, to predict plant uptake and bioavailability.Science Foundation IrelandFundação de Amparo à Pesquisa do Estado de São Paulo (FAPESP)Institute for Global Food Security School of Biological Sciences Queen’s University BelfastState Key Laboratory of Pollution Control and Resource Reuse School of the Environment Nanjing UniversityEnvironmental Studies Center (CEA) São Paulo State University (UNESP), Avenida 24-A, 1515Department of Chemistry University of WarwickGoldenKeys High-Tech Materials Co. Ltd., Building B, Innovation & Entrepreneurship Park, Guian New AreaEnvironmental Studies Center (CEA) São Paulo State University (UNESP), Avenida 24-A, 1515Science Foundation Ireland: 14/IA/2371FAPESP: FAPESP-2018/17069-7Queen’s University BelfastNanjing UniversityUniversidade Estadual Paulista (Unesp)University of WarwickLtd.Yang, Jia-WeiFang, WenWilliams, Paul N.McGrath, John W.Eismann, Carlos Eduardo [UNESP]Menegário, Amauri Antonio [UNESP]Elias, Lucas Pellegrini [UNESP]Luo, JunXu, Yingjian2020-12-12T02:45:33Z2020-12-12T02:45:33Z2020-09-01info:eu-repo/semantics/publishedVersioninfo:eu-repo/semantics/article264-280http://dx.doi.org/10.1007/s40726-020-00152-6Current Pollution Reports, v. 6, n. 3, p. 264-280, 2020.2198-6592http://hdl.handle.net/11449/20193110.1007/s40726-020-00152-62-s2.0-85087382598Scopusreponame:Repositório Institucional da UNESPinstname:Universidade Estadual Paulista (UNESP)instacron:UNESPengCurrent Pollution Reportsinfo:eu-repo/semantics/openAccess2024-04-10T19:22:25Zoai:repositorio.unesp.br:11449/201931Repositório InstitucionalPUBhttp://repositorio.unesp.br/oai/requestopendoar:29462024-08-05T16:59:56.999086Repositório Institucional da UNESP - Universidade Estadual Paulista (UNESP)false
dc.title.none.fl_str_mv Functionalized Mesoporous Silicon Nanomaterials in Inorganic Soil Pollution Research: Opportunities for Soil Protection and Advanced Chemical Imaging
title Functionalized Mesoporous Silicon Nanomaterials in Inorganic Soil Pollution Research: Opportunities for Soil Protection and Advanced Chemical Imaging
spellingShingle Functionalized Mesoporous Silicon Nanomaterials in Inorganic Soil Pollution Research: Opportunities for Soil Protection and Advanced Chemical Imaging
Yang, Jia-Wei
Diffusive gradient in thin films (DGT)
Functional mesoporous silicon nanomaterials (FMSN)
Heavy metals
Soil pollution
X-ray fluorescence spectrometry (XRF)
title_short Functionalized Mesoporous Silicon Nanomaterials in Inorganic Soil Pollution Research: Opportunities for Soil Protection and Advanced Chemical Imaging
title_full Functionalized Mesoporous Silicon Nanomaterials in Inorganic Soil Pollution Research: Opportunities for Soil Protection and Advanced Chemical Imaging
title_fullStr Functionalized Mesoporous Silicon Nanomaterials in Inorganic Soil Pollution Research: Opportunities for Soil Protection and Advanced Chemical Imaging
title_full_unstemmed Functionalized Mesoporous Silicon Nanomaterials in Inorganic Soil Pollution Research: Opportunities for Soil Protection and Advanced Chemical Imaging
title_sort Functionalized Mesoporous Silicon Nanomaterials in Inorganic Soil Pollution Research: Opportunities for Soil Protection and Advanced Chemical Imaging
author Yang, Jia-Wei
author_facet Yang, Jia-Wei
Fang, Wen
Williams, Paul N.
McGrath, John W.
Eismann, Carlos Eduardo [UNESP]
Menegário, Amauri Antonio [UNESP]
Elias, Lucas Pellegrini [UNESP]
Luo, Jun
Xu, Yingjian
author_role author
author2 Fang, Wen
Williams, Paul N.
McGrath, John W.
Eismann, Carlos Eduardo [UNESP]
Menegário, Amauri Antonio [UNESP]
Elias, Lucas Pellegrini [UNESP]
Luo, Jun
Xu, Yingjian
author2_role author
author
author
author
author
author
author
author
dc.contributor.none.fl_str_mv Queen’s University Belfast
Nanjing University
Universidade Estadual Paulista (Unesp)
University of Warwick
Ltd.
dc.contributor.author.fl_str_mv Yang, Jia-Wei
Fang, Wen
Williams, Paul N.
McGrath, John W.
Eismann, Carlos Eduardo [UNESP]
Menegário, Amauri Antonio [UNESP]
Elias, Lucas Pellegrini [UNESP]
Luo, Jun
Xu, Yingjian
dc.subject.por.fl_str_mv Diffusive gradient in thin films (DGT)
Functional mesoporous silicon nanomaterials (FMSN)
Heavy metals
Soil pollution
X-ray fluorescence spectrometry (XRF)
topic Diffusive gradient in thin films (DGT)
Functional mesoporous silicon nanomaterials (FMSN)
Heavy metals
Soil pollution
X-ray fluorescence spectrometry (XRF)
description “Innovative actions towards a pollution free-planet” is a goal of the United Nations Environment Assembly (UNEA). Aided by both the Food and Agricultural Organisation (FAO) and its Global Soil Partnership under the 3rd UNEA resolution, a consensus from > 170 countries have agreed a need for accelerated action and collaboration to combat soil pollution. This initiative has been tasked to find new and improved solutions to prevent and reduce soil pollution, and it is in this context that this review provides an updated perspective on an emerging technology platform that has already provided demonstrable utility for measurement, mapping, and monitoring of toxic trace elements (TTEs) in soils, in addition to the entrapment, removal, and remediation of pollutant sources. In this article, the development and characteristics of functionalized mesoporous silica nanomaterials (FMSN) will be discussed and compared with other common metal scavenging materials. The chemistries of the common functionalizations will be reviewed, in addition to providing an outlook on some of the future directions/applications of FMSN. The use of FMSN in soil will be considered with some specific case studies focusing on Hg and As. Finally, the advantages and developments of FMSN in the widely used diffusive gradients-in-thin films (DGT) technique will be discussed, in particular, its advantages as a DGT substrate for integration with oxygen planar optodes in multilayer systems that provide 2D mapping of metal pollutant fluxes at submillimeter resolution, which can be used to measure detailed sediment-water fluxes as well as soil-root interactions, to predict plant uptake and bioavailability.
publishDate 2020
dc.date.none.fl_str_mv 2020-12-12T02:45:33Z
2020-12-12T02:45:33Z
2020-09-01
dc.type.status.fl_str_mv info:eu-repo/semantics/publishedVersion
dc.type.driver.fl_str_mv info:eu-repo/semantics/article
format article
status_str publishedVersion
dc.identifier.uri.fl_str_mv http://dx.doi.org/10.1007/s40726-020-00152-6
Current Pollution Reports, v. 6, n. 3, p. 264-280, 2020.
2198-6592
http://hdl.handle.net/11449/201931
10.1007/s40726-020-00152-6
2-s2.0-85087382598
url http://dx.doi.org/10.1007/s40726-020-00152-6
http://hdl.handle.net/11449/201931
identifier_str_mv Current Pollution Reports, v. 6, n. 3, p. 264-280, 2020.
2198-6592
10.1007/s40726-020-00152-6
2-s2.0-85087382598
dc.language.iso.fl_str_mv eng
language eng
dc.relation.none.fl_str_mv Current Pollution Reports
dc.rights.driver.fl_str_mv info:eu-repo/semantics/openAccess
eu_rights_str_mv openAccess
dc.format.none.fl_str_mv 264-280
dc.source.none.fl_str_mv Scopus
reponame:Repositório Institucional da UNESP
instname:Universidade Estadual Paulista (UNESP)
instacron:UNESP
instname_str Universidade Estadual Paulista (UNESP)
instacron_str UNESP
institution UNESP
reponame_str Repositório Institucional da UNESP
collection Repositório Institucional da UNESP
repository.name.fl_str_mv Repositório Institucional da UNESP - Universidade Estadual Paulista (UNESP)
repository.mail.fl_str_mv
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