Strain engineering of quantum confinement in WSe2on nano-roughness glass substrates
Autor(a) principal: | |
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Data de Publicação: | 2022 |
Outros Autores: | , , , , , |
Tipo de documento: | Artigo |
Idioma: | eng |
Título da fonte: | Repositório Institucional da UNESP |
Texto Completo: | http://dx.doi.org/10.1063/5.0107201 http://hdl.handle.net/11449/240756 |
Resumo: | Strain engineering is a powerful tool for generating single-photon emitters in monolayer (ML) transition metal dichalcogenides. Here, we report on a simple method for generating sharp emission lines (linewidths ≈ 150-500 μeV) in a monolayer (ML) WSe2 on nano-roughness regions of Tb3+-borogermanate glasses. We performed a polarization-resolved magneto-luminescence study in WSe2/glass at low temperature. Remarkably, we observed several stable and linearly polarized doublet emission peaks in strained regions that are associated with a fine structure splitting due to the anisotropic electron-hole exchange interaction with g-factors of ∼8.4-9.8. Our results indicate that strain engineering on glass substrates is a promising tool for generating quantum dot-like emitters in ML WSe2 for possible integration with photonics systems for quantum information technology. |
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Repositório Institucional da UNESP |
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2946 |
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Strain engineering of quantum confinement in WSe2on nano-roughness glass substratesStrain engineering is a powerful tool for generating single-photon emitters in monolayer (ML) transition metal dichalcogenides. Here, we report on a simple method for generating sharp emission lines (linewidths ≈ 150-500 μeV) in a monolayer (ML) WSe2 on nano-roughness regions of Tb3+-borogermanate glasses. We performed a polarization-resolved magneto-luminescence study in WSe2/glass at low temperature. Remarkably, we observed several stable and linearly polarized doublet emission peaks in strained regions that are associated with a fine structure splitting due to the anisotropic electron-hole exchange interaction with g-factors of ∼8.4-9.8. Our results indicate that strain engineering on glass substrates is a promising tool for generating quantum dot-like emitters in ML WSe2 for possible integration with photonics systems for quantum information technology.Department of Physics Federal University of São CarlosInstitute of Chemistry São Paulo State University UNESP, SPBrazilian Synchrotron Light Laboratory (LNLS) Brazilian Center for Research in Energy and Materials (CNPEM)Institute of Chemistry São Paulo State University UNESP, SPUniversidade Federal de São Carlos (UFSCar)Universidade Estadual Paulista (UNESP)Brazilian Center for Research in Energy and Materials (CNPEM)Brito, Caique Serati deRabahi, Cesar RicardoTeodoro, Marcio DaldinFranco, Douglas F. [UNESP]Nalin, Marcelo [UNESP]Barcelos, Ingrid D.Gobato, Yara Galvão2023-03-01T20:31:29Z2023-03-01T20:31:29Z2022-08-15info:eu-repo/semantics/publishedVersioninfo:eu-repo/semantics/articlehttp://dx.doi.org/10.1063/5.0107201Applied Physics Letters, v. 121, n. 7, 2022.0003-6951http://hdl.handle.net/11449/24075610.1063/5.01072012-s2.0-85137158656Scopusreponame:Repositório Institucional da UNESPinstname:Universidade Estadual Paulista (UNESP)instacron:UNESPengApplied Physics Lettersinfo:eu-repo/semantics/openAccess2023-03-01T20:31:30Zoai:repositorio.unesp.br:11449/240756Repositório InstitucionalPUBhttp://repositorio.unesp.br/oai/requestopendoar:29462024-08-05T16:44:49.304417Repositório Institucional da UNESP - Universidade Estadual Paulista (UNESP)false |
dc.title.none.fl_str_mv |
Strain engineering of quantum confinement in WSe2on nano-roughness glass substrates |
title |
Strain engineering of quantum confinement in WSe2on nano-roughness glass substrates |
spellingShingle |
Strain engineering of quantum confinement in WSe2on nano-roughness glass substrates Brito, Caique Serati de |
title_short |
Strain engineering of quantum confinement in WSe2on nano-roughness glass substrates |
title_full |
Strain engineering of quantum confinement in WSe2on nano-roughness glass substrates |
title_fullStr |
Strain engineering of quantum confinement in WSe2on nano-roughness glass substrates |
title_full_unstemmed |
Strain engineering of quantum confinement in WSe2on nano-roughness glass substrates |
title_sort |
Strain engineering of quantum confinement in WSe2on nano-roughness glass substrates |
author |
Brito, Caique Serati de |
author_facet |
Brito, Caique Serati de Rabahi, Cesar Ricardo Teodoro, Marcio Daldin Franco, Douglas F. [UNESP] Nalin, Marcelo [UNESP] Barcelos, Ingrid D. Gobato, Yara Galvão |
author_role |
author |
author2 |
Rabahi, Cesar Ricardo Teodoro, Marcio Daldin Franco, Douglas F. [UNESP] Nalin, Marcelo [UNESP] Barcelos, Ingrid D. Gobato, Yara Galvão |
author2_role |
author author author author author author |
dc.contributor.none.fl_str_mv |
Universidade Federal de São Carlos (UFSCar) Universidade Estadual Paulista (UNESP) Brazilian Center for Research in Energy and Materials (CNPEM) |
dc.contributor.author.fl_str_mv |
Brito, Caique Serati de Rabahi, Cesar Ricardo Teodoro, Marcio Daldin Franco, Douglas F. [UNESP] Nalin, Marcelo [UNESP] Barcelos, Ingrid D. Gobato, Yara Galvão |
description |
Strain engineering is a powerful tool for generating single-photon emitters in monolayer (ML) transition metal dichalcogenides. Here, we report on a simple method for generating sharp emission lines (linewidths ≈ 150-500 μeV) in a monolayer (ML) WSe2 on nano-roughness regions of Tb3+-borogermanate glasses. We performed a polarization-resolved magneto-luminescence study in WSe2/glass at low temperature. Remarkably, we observed several stable and linearly polarized doublet emission peaks in strained regions that are associated with a fine structure splitting due to the anisotropic electron-hole exchange interaction with g-factors of ∼8.4-9.8. Our results indicate that strain engineering on glass substrates is a promising tool for generating quantum dot-like emitters in ML WSe2 for possible integration with photonics systems for quantum information technology. |
publishDate |
2022 |
dc.date.none.fl_str_mv |
2022-08-15 2023-03-01T20:31:29Z 2023-03-01T20:31:29Z |
dc.type.status.fl_str_mv |
info:eu-repo/semantics/publishedVersion |
dc.type.driver.fl_str_mv |
info:eu-repo/semantics/article |
format |
article |
status_str |
publishedVersion |
dc.identifier.uri.fl_str_mv |
http://dx.doi.org/10.1063/5.0107201 Applied Physics Letters, v. 121, n. 7, 2022. 0003-6951 http://hdl.handle.net/11449/240756 10.1063/5.0107201 2-s2.0-85137158656 |
url |
http://dx.doi.org/10.1063/5.0107201 http://hdl.handle.net/11449/240756 |
identifier_str_mv |
Applied Physics Letters, v. 121, n. 7, 2022. 0003-6951 10.1063/5.0107201 2-s2.0-85137158656 |
dc.language.iso.fl_str_mv |
eng |
language |
eng |
dc.relation.none.fl_str_mv |
Applied Physics Letters |
dc.rights.driver.fl_str_mv |
info:eu-repo/semantics/openAccess |
eu_rights_str_mv |
openAccess |
dc.source.none.fl_str_mv |
Scopus reponame:Repositório Institucional da UNESP instname:Universidade Estadual Paulista (UNESP) instacron:UNESP |
instname_str |
Universidade Estadual Paulista (UNESP) |
instacron_str |
UNESP |
institution |
UNESP |
reponame_str |
Repositório Institucional da UNESP |
collection |
Repositório Institucional da UNESP |
repository.name.fl_str_mv |
Repositório Institucional da UNESP - Universidade Estadual Paulista (UNESP) |
repository.mail.fl_str_mv |
|
_version_ |
1808128695444963328 |