Strain engineering of quantum confinement in WSe2on nano-roughness glass substrates

Detalhes bibliográficos
Autor(a) principal: Brito, Caique Serati de
Data de Publicação: 2022
Outros Autores: Rabahi, Cesar Ricardo, Teodoro, Marcio Daldin, Franco, Douglas F. [UNESP], Nalin, Marcelo [UNESP], Barcelos, Ingrid D., Gobato, Yara Galvão
Tipo de documento: Artigo
Idioma: eng
Título da fonte: Repositório Institucional da UNESP
Texto Completo: http://dx.doi.org/10.1063/5.0107201
http://hdl.handle.net/11449/240756
Resumo: Strain engineering is a powerful tool for generating single-photon emitters in monolayer (ML) transition metal dichalcogenides. Here, we report on a simple method for generating sharp emission lines (linewidths ≈ 150-500 μeV) in a monolayer (ML) WSe2 on nano-roughness regions of Tb3+-borogermanate glasses. We performed a polarization-resolved magneto-luminescence study in WSe2/glass at low temperature. Remarkably, we observed several stable and linearly polarized doublet emission peaks in strained regions that are associated with a fine structure splitting due to the anisotropic electron-hole exchange interaction with g-factors of ∼8.4-9.8. Our results indicate that strain engineering on glass substrates is a promising tool for generating quantum dot-like emitters in ML WSe2 for possible integration with photonics systems for quantum information technology.
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spelling Strain engineering of quantum confinement in WSe2on nano-roughness glass substratesStrain engineering is a powerful tool for generating single-photon emitters in monolayer (ML) transition metal dichalcogenides. Here, we report on a simple method for generating sharp emission lines (linewidths ≈ 150-500 μeV) in a monolayer (ML) WSe2 on nano-roughness regions of Tb3+-borogermanate glasses. We performed a polarization-resolved magneto-luminescence study in WSe2/glass at low temperature. Remarkably, we observed several stable and linearly polarized doublet emission peaks in strained regions that are associated with a fine structure splitting due to the anisotropic electron-hole exchange interaction with g-factors of ∼8.4-9.8. Our results indicate that strain engineering on glass substrates is a promising tool for generating quantum dot-like emitters in ML WSe2 for possible integration with photonics systems for quantum information technology.Department of Physics Federal University of São CarlosInstitute of Chemistry São Paulo State University UNESP, SPBrazilian Synchrotron Light Laboratory (LNLS) Brazilian Center for Research in Energy and Materials (CNPEM)Institute of Chemistry São Paulo State University UNESP, SPUniversidade Federal de São Carlos (UFSCar)Universidade Estadual Paulista (UNESP)Brazilian Center for Research in Energy and Materials (CNPEM)Brito, Caique Serati deRabahi, Cesar RicardoTeodoro, Marcio DaldinFranco, Douglas F. [UNESP]Nalin, Marcelo [UNESP]Barcelos, Ingrid D.Gobato, Yara Galvão2023-03-01T20:31:29Z2023-03-01T20:31:29Z2022-08-15info:eu-repo/semantics/publishedVersioninfo:eu-repo/semantics/articlehttp://dx.doi.org/10.1063/5.0107201Applied Physics Letters, v. 121, n. 7, 2022.0003-6951http://hdl.handle.net/11449/24075610.1063/5.01072012-s2.0-85137158656Scopusreponame:Repositório Institucional da UNESPinstname:Universidade Estadual Paulista (UNESP)instacron:UNESPengApplied Physics Lettersinfo:eu-repo/semantics/openAccess2023-03-01T20:31:30Zoai:repositorio.unesp.br:11449/240756Repositório InstitucionalPUBhttp://repositorio.unesp.br/oai/requestopendoar:29462024-08-05T16:44:49.304417Repositório Institucional da UNESP - Universidade Estadual Paulista (UNESP)false
dc.title.none.fl_str_mv Strain engineering of quantum confinement in WSe2on nano-roughness glass substrates
title Strain engineering of quantum confinement in WSe2on nano-roughness glass substrates
spellingShingle Strain engineering of quantum confinement in WSe2on nano-roughness glass substrates
Brito, Caique Serati de
title_short Strain engineering of quantum confinement in WSe2on nano-roughness glass substrates
title_full Strain engineering of quantum confinement in WSe2on nano-roughness glass substrates
title_fullStr Strain engineering of quantum confinement in WSe2on nano-roughness glass substrates
title_full_unstemmed Strain engineering of quantum confinement in WSe2on nano-roughness glass substrates
title_sort Strain engineering of quantum confinement in WSe2on nano-roughness glass substrates
author Brito, Caique Serati de
author_facet Brito, Caique Serati de
Rabahi, Cesar Ricardo
Teodoro, Marcio Daldin
Franco, Douglas F. [UNESP]
Nalin, Marcelo [UNESP]
Barcelos, Ingrid D.
Gobato, Yara Galvão
author_role author
author2 Rabahi, Cesar Ricardo
Teodoro, Marcio Daldin
Franco, Douglas F. [UNESP]
Nalin, Marcelo [UNESP]
Barcelos, Ingrid D.
Gobato, Yara Galvão
author2_role author
author
author
author
author
author
dc.contributor.none.fl_str_mv Universidade Federal de São Carlos (UFSCar)
Universidade Estadual Paulista (UNESP)
Brazilian Center for Research in Energy and Materials (CNPEM)
dc.contributor.author.fl_str_mv Brito, Caique Serati de
Rabahi, Cesar Ricardo
Teodoro, Marcio Daldin
Franco, Douglas F. [UNESP]
Nalin, Marcelo [UNESP]
Barcelos, Ingrid D.
Gobato, Yara Galvão
description Strain engineering is a powerful tool for generating single-photon emitters in monolayer (ML) transition metal dichalcogenides. Here, we report on a simple method for generating sharp emission lines (linewidths ≈ 150-500 μeV) in a monolayer (ML) WSe2 on nano-roughness regions of Tb3+-borogermanate glasses. We performed a polarization-resolved magneto-luminescence study in WSe2/glass at low temperature. Remarkably, we observed several stable and linearly polarized doublet emission peaks in strained regions that are associated with a fine structure splitting due to the anisotropic electron-hole exchange interaction with g-factors of ∼8.4-9.8. Our results indicate that strain engineering on glass substrates is a promising tool for generating quantum dot-like emitters in ML WSe2 for possible integration with photonics systems for quantum information technology.
publishDate 2022
dc.date.none.fl_str_mv 2022-08-15
2023-03-01T20:31:29Z
2023-03-01T20:31:29Z
dc.type.status.fl_str_mv info:eu-repo/semantics/publishedVersion
dc.type.driver.fl_str_mv info:eu-repo/semantics/article
format article
status_str publishedVersion
dc.identifier.uri.fl_str_mv http://dx.doi.org/10.1063/5.0107201
Applied Physics Letters, v. 121, n. 7, 2022.
0003-6951
http://hdl.handle.net/11449/240756
10.1063/5.0107201
2-s2.0-85137158656
url http://dx.doi.org/10.1063/5.0107201
http://hdl.handle.net/11449/240756
identifier_str_mv Applied Physics Letters, v. 121, n. 7, 2022.
0003-6951
10.1063/5.0107201
2-s2.0-85137158656
dc.language.iso.fl_str_mv eng
language eng
dc.relation.none.fl_str_mv Applied Physics Letters
dc.rights.driver.fl_str_mv info:eu-repo/semantics/openAccess
eu_rights_str_mv openAccess
dc.source.none.fl_str_mv Scopus
reponame:Repositório Institucional da UNESP
instname:Universidade Estadual Paulista (UNESP)
instacron:UNESP
instname_str Universidade Estadual Paulista (UNESP)
instacron_str UNESP
institution UNESP
reponame_str Repositório Institucional da UNESP
collection Repositório Institucional da UNESP
repository.name.fl_str_mv Repositório Institucional da UNESP - Universidade Estadual Paulista (UNESP)
repository.mail.fl_str_mv
_version_ 1808128695444963328