Parylene-Sealed Perovskite Nanocrystals Down-Shifting Layer for Luminescent Spectral Matching in Thin Film Photovoltaics

Detalhes bibliográficos
Autor(a) principal: Pinheiro, Ana
Data de Publicação: 2023
Outros Autores: Ruivo, Andreia, Rocha, João, Ferro, Marta, Pinto, Joana Vaz, Deuermeier, Jonas, Mateus, Tiago, Santa, Ana, Mendes, Manuel J., Martins, Rodrigo, Gago, Sandra, Laia, César A.T., Águas, Hugo
Tipo de documento: Artigo
Idioma: eng
Título da fonte: Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos)
Texto Completo: http://hdl.handle.net/10362/154611
Resumo: Funding Information: This work was also financed by national funds from FCT/MCETS (Fundação para a Ciência e Tecnologia and Ministério da Ciência, Tecnologia e Ensino Superior) in the scope of the projects LA/P/0037/2020, Nanomodelling and Nanofabrication, i3N, LA/P/0006/2020, CICECO-Aveiro Institute of Materials. Publisher Copyright: © 2023 by the authors.
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spelling Parylene-Sealed Perovskite Nanocrystals Down-Shifting Layer for Luminescent Spectral Matching in Thin Film Photovoltaicsluminescent materialsparylene type Cperovskite nanocrystalsphotovoltaicssilicon solar cellsChemical Engineering(all)Materials Science(all)SDG 7 - Affordable and Clean EnergyFunding Information: This work was also financed by national funds from FCT/MCETS (Fundação para a Ciência e Tecnologia and Ministério da Ciência, Tecnologia e Ensino Superior) in the scope of the projects LA/P/0037/2020, Nanomodelling and Nanofabrication, i3N, LA/P/0006/2020, CICECO-Aveiro Institute of Materials. Publisher Copyright: © 2023 by the authors.The present contribution aims to enhance solar cells’ performance via the development of advanced luminescent down-shifting based on encapsulated nanostructured perovskite materials. Here, thin films of inorganic lead halide (CsPbBr3) perovskite nanocrystal luminophores were synthetized, by hot-injection, deposited on glass substrates by spin-coating, and encapsulated with parylene type C, via chemical vapor deposition, to protect and stabilize the films. The optical properties of these thin films were characterized by absorption, emission and 2D contour spectra, their structure by X-ray diffraction and X-ray photoelectron spectroscopy, and the morphology by Scanning Transmission Electron microscopy. I–V curve and spectral response nanocrystalline silicon photovoltaic (nc-Si:H PV) cells were studied in the absence and presence of the perovskite and parylene luminescent down-shifting layers. The incorporation of the CsPbBr3 nanocrystals and their encapsulation with the parylene type C polymeric coating led to an increase in the current generated and the spectral response of the PV cells in the regime of the nanocrystals’ fluorescence emission. A 3.1% increase in the short circuit current density and a 5.6% increase in the power conversion efficiency were observed.VICARTE - Vidro e Cerâmica para as ArtesLAQV@REQUIMTECENIMAT-i3N - Centro de Investigação de Materiais (Lab. Associado I3N)UNINOVA-Instituto de Desenvolvimento de Novas TecnologiasRUNPinheiro, AnaRuivo, AndreiaRocha, JoãoFerro, MartaPinto, Joana VazDeuermeier, JonasMateus, TiagoSanta, AnaMendes, Manuel J.Martins, RodrigoGago, SandraLaia, César A.T.Águas, Hugo2023-06-29T22:15:57Z2023-01-032023-01-03T00:00:00Zinfo:eu-repo/semantics/publishedVersioninfo:eu-repo/semantics/article15application/pdfhttp://hdl.handle.net/10362/154611eng2079-4991PURE: 64808501https://doi.org/10.3390/nano13010210info:eu-repo/semantics/openAccessreponame:Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos)instname:Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informaçãoinstacron:RCAAP2024-03-18T01:43:03Zoai:run.unl.pt:10362/154611Portal AgregadorONGhttps://www.rcaap.pt/oai/openaireopendoar:71602024-03-20T03:55:41.559329Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) - Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informaçãofalse
dc.title.none.fl_str_mv Parylene-Sealed Perovskite Nanocrystals Down-Shifting Layer for Luminescent Spectral Matching in Thin Film Photovoltaics
title Parylene-Sealed Perovskite Nanocrystals Down-Shifting Layer for Luminescent Spectral Matching in Thin Film Photovoltaics
spellingShingle Parylene-Sealed Perovskite Nanocrystals Down-Shifting Layer for Luminescent Spectral Matching in Thin Film Photovoltaics
Pinheiro, Ana
luminescent materials
parylene type C
perovskite nanocrystals
photovoltaics
silicon solar cells
Chemical Engineering(all)
Materials Science(all)
SDG 7 - Affordable and Clean Energy
title_short Parylene-Sealed Perovskite Nanocrystals Down-Shifting Layer for Luminescent Spectral Matching in Thin Film Photovoltaics
title_full Parylene-Sealed Perovskite Nanocrystals Down-Shifting Layer for Luminescent Spectral Matching in Thin Film Photovoltaics
title_fullStr Parylene-Sealed Perovskite Nanocrystals Down-Shifting Layer for Luminescent Spectral Matching in Thin Film Photovoltaics
title_full_unstemmed Parylene-Sealed Perovskite Nanocrystals Down-Shifting Layer for Luminescent Spectral Matching in Thin Film Photovoltaics
title_sort Parylene-Sealed Perovskite Nanocrystals Down-Shifting Layer for Luminescent Spectral Matching in Thin Film Photovoltaics
author Pinheiro, Ana
author_facet Pinheiro, Ana
Ruivo, Andreia
Rocha, João
Ferro, Marta
Pinto, Joana Vaz
Deuermeier, Jonas
Mateus, Tiago
Santa, Ana
Mendes, Manuel J.
Martins, Rodrigo
Gago, Sandra
Laia, César A.T.
Águas, Hugo
author_role author
author2 Ruivo, Andreia
Rocha, João
Ferro, Marta
Pinto, Joana Vaz
Deuermeier, Jonas
Mateus, Tiago
Santa, Ana
Mendes, Manuel J.
Martins, Rodrigo
Gago, Sandra
Laia, César A.T.
Águas, Hugo
author2_role author
author
author
author
author
author
author
author
author
author
author
author
dc.contributor.none.fl_str_mv VICARTE - Vidro e Cerâmica para as Artes
LAQV@REQUIMTE
CENIMAT-i3N - Centro de Investigação de Materiais (Lab. Associado I3N)
UNINOVA-Instituto de Desenvolvimento de Novas Tecnologias
RUN
dc.contributor.author.fl_str_mv Pinheiro, Ana
Ruivo, Andreia
Rocha, João
Ferro, Marta
Pinto, Joana Vaz
Deuermeier, Jonas
Mateus, Tiago
Santa, Ana
Mendes, Manuel J.
Martins, Rodrigo
Gago, Sandra
Laia, César A.T.
Águas, Hugo
dc.subject.por.fl_str_mv luminescent materials
parylene type C
perovskite nanocrystals
photovoltaics
silicon solar cells
Chemical Engineering(all)
Materials Science(all)
SDG 7 - Affordable and Clean Energy
topic luminescent materials
parylene type C
perovskite nanocrystals
photovoltaics
silicon solar cells
Chemical Engineering(all)
Materials Science(all)
SDG 7 - Affordable and Clean Energy
description Funding Information: This work was also financed by national funds from FCT/MCETS (Fundação para a Ciência e Tecnologia and Ministério da Ciência, Tecnologia e Ensino Superior) in the scope of the projects LA/P/0037/2020, Nanomodelling and Nanofabrication, i3N, LA/P/0006/2020, CICECO-Aveiro Institute of Materials. Publisher Copyright: © 2023 by the authors.
publishDate 2023
dc.date.none.fl_str_mv 2023-06-29T22:15:57Z
2023-01-03
2023-01-03T00:00:00Z
dc.type.status.fl_str_mv info:eu-repo/semantics/publishedVersion
dc.type.driver.fl_str_mv info:eu-repo/semantics/article
format article
status_str publishedVersion
dc.identifier.uri.fl_str_mv http://hdl.handle.net/10362/154611
url http://hdl.handle.net/10362/154611
dc.language.iso.fl_str_mv eng
language eng
dc.relation.none.fl_str_mv 2079-4991
PURE: 64808501
https://doi.org/10.3390/nano13010210
dc.rights.driver.fl_str_mv info:eu-repo/semantics/openAccess
eu_rights_str_mv openAccess
dc.format.none.fl_str_mv 15
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repository.name.fl_str_mv Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) - Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informação
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