Piezoelectricity Enhancement of Nanogenerators Based on PDMS and ZnSnO3 Nanowires through Microstructuration
Autor(a) principal: | |
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Data de Publicação: | 2020 |
Outros Autores: | , , , , , , , , , |
Tipo de documento: | Artigo |
Idioma: | eng |
Título da fonte: | Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) |
Texto Completo: | http://hdl.handle.net/10362/117017 |
Resumo: | SFRH/BD/131836/2017 SFRH/BD/122286/2016 PD/BD/105876/2014 |
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Piezoelectricity Enhancement of Nanogenerators Based on PDMS and ZnSnO3 Nanowires through Microstructurationmicro-structurationnanogeneratornanowiresPDMSpiezoelectricityZnSnO3Materials Science(all)SFRH/BD/131836/2017 SFRH/BD/122286/2016 PD/BD/105876/2014The current trend for smart, self-sustainable, and multifunctional technology demands for the development of energy harvesters based on widely available and environmentally friendly materials. In this context, ZnSnO3 nanostructures show promising potential because of their high polarization, which can be explored in piezoelectric devices. Nevertheless, a pure phase of ZnSnO3 is hard to achieve because of its metastability, and obtaining it in the form of nanowires is even more challenging. Although some groups have already reported the mixing of ZnSnO3 nanostructures with polydimethylsiloxane (PDMS) to produce a nanogenerator, the resultant polymeric film is usually flat and does not take advantage of an enhanced piezoelectric contribution achieved through its microstructuration. Herein, a microstructured composite of nanowires synthesized by a seed-layer free hydrothermal route mixed with PDMS (ZnSnO3@PDMS) is proposed to produce nanogenerators. PFM measurements show a clear enhancement of d33 for single ZnSnO3 versus ZnO nanowires (23 ± 4 pm/V vs 9 ± 2 pm/V). The microstructuration introduced herein results in an enhancement of the piezoelectric effect of the ZnSnO3 nanowires, enabling nanogenerators with an output voltage, current, and instantaneous power density of 120 V, 13 μA, and 230 μW·cm-2, respectively. Even using an active area smaller than 1 cm2, the performance of this nanogenerator enables lighting up multiple LEDs and other small electronic devices, thus proving great potential for wearables and portable electronics.UNINOVA-Instituto de Desenvolvimento de Novas TecnologiasDCM - Departamento de Ciência dos MateriaisCENIMAT-i3N - Centro de Investigação de Materiais (Lab. Associado I3N)RUNRovisco, AnaDos Santos, AndreiaCramer, TobiasMartins, JorgeBranquinho, RitaÁguas, HugoFraboni, BeatriceFortunato, ElviraMartins, RodrigoIgreja, RuiBarquinha, Pedro2021-05-04T22:53:54Z2020-04-222020-04-22T00:00:00Zinfo:eu-repo/semantics/publishedVersioninfo:eu-repo/semantics/article10application/pdfhttp://hdl.handle.net/10362/117017eng1944-8244PURE: 18416957https://doi.org/10.1021/acsami.9b21636info:eu-repo/semantics/openAccessreponame:Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos)instname:Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informaçãoinstacron:RCAAP2024-03-11T04:59:56Zoai:run.unl.pt:10362/117017Portal AgregadorONGhttps://www.rcaap.pt/oai/openaireopendoar:71602024-03-20T03:43:25.387142Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) - Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informaçãofalse |
dc.title.none.fl_str_mv |
Piezoelectricity Enhancement of Nanogenerators Based on PDMS and ZnSnO3 Nanowires through Microstructuration |
title |
Piezoelectricity Enhancement of Nanogenerators Based on PDMS and ZnSnO3 Nanowires through Microstructuration |
spellingShingle |
Piezoelectricity Enhancement of Nanogenerators Based on PDMS and ZnSnO3 Nanowires through Microstructuration Rovisco, Ana micro-structuration nanogenerator nanowires PDMS piezoelectricity ZnSnO3 Materials Science(all) |
title_short |
Piezoelectricity Enhancement of Nanogenerators Based on PDMS and ZnSnO3 Nanowires through Microstructuration |
title_full |
Piezoelectricity Enhancement of Nanogenerators Based on PDMS and ZnSnO3 Nanowires through Microstructuration |
title_fullStr |
Piezoelectricity Enhancement of Nanogenerators Based on PDMS and ZnSnO3 Nanowires through Microstructuration |
title_full_unstemmed |
Piezoelectricity Enhancement of Nanogenerators Based on PDMS and ZnSnO3 Nanowires through Microstructuration |
title_sort |
Piezoelectricity Enhancement of Nanogenerators Based on PDMS and ZnSnO3 Nanowires through Microstructuration |
author |
Rovisco, Ana |
author_facet |
Rovisco, Ana Dos Santos, Andreia Cramer, Tobias Martins, Jorge Branquinho, Rita Águas, Hugo Fraboni, Beatrice Fortunato, Elvira Martins, Rodrigo Igreja, Rui Barquinha, Pedro |
author_role |
author |
author2 |
Dos Santos, Andreia Cramer, Tobias Martins, Jorge Branquinho, Rita Águas, Hugo Fraboni, Beatrice Fortunato, Elvira Martins, Rodrigo Igreja, Rui Barquinha, Pedro |
author2_role |
author author author author author author author author author author |
dc.contributor.none.fl_str_mv |
UNINOVA-Instituto de Desenvolvimento de Novas Tecnologias DCM - Departamento de Ciência dos Materiais CENIMAT-i3N - Centro de Investigação de Materiais (Lab. Associado I3N) RUN |
dc.contributor.author.fl_str_mv |
Rovisco, Ana Dos Santos, Andreia Cramer, Tobias Martins, Jorge Branquinho, Rita Águas, Hugo Fraboni, Beatrice Fortunato, Elvira Martins, Rodrigo Igreja, Rui Barquinha, Pedro |
dc.subject.por.fl_str_mv |
micro-structuration nanogenerator nanowires PDMS piezoelectricity ZnSnO3 Materials Science(all) |
topic |
micro-structuration nanogenerator nanowires PDMS piezoelectricity ZnSnO3 Materials Science(all) |
description |
SFRH/BD/131836/2017 SFRH/BD/122286/2016 PD/BD/105876/2014 |
publishDate |
2020 |
dc.date.none.fl_str_mv |
2020-04-22 2020-04-22T00:00:00Z 2021-05-04T22:53:54Z |
dc.type.status.fl_str_mv |
info:eu-repo/semantics/publishedVersion |
dc.type.driver.fl_str_mv |
info:eu-repo/semantics/article |
format |
article |
status_str |
publishedVersion |
dc.identifier.uri.fl_str_mv |
http://hdl.handle.net/10362/117017 |
url |
http://hdl.handle.net/10362/117017 |
dc.language.iso.fl_str_mv |
eng |
language |
eng |
dc.relation.none.fl_str_mv |
1944-8244 PURE: 18416957 https://doi.org/10.1021/acsami.9b21636 |
dc.rights.driver.fl_str_mv |
info:eu-repo/semantics/openAccess |
eu_rights_str_mv |
openAccess |
dc.format.none.fl_str_mv |
10 application/pdf |
dc.source.none.fl_str_mv |
reponame:Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) instname:Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informação instacron:RCAAP |
instname_str |
Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informação |
instacron_str |
RCAAP |
institution |
RCAAP |
reponame_str |
Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) |
collection |
Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) |
repository.name.fl_str_mv |
Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) - Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informação |
repository.mail.fl_str_mv |
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1799138043986182144 |