Handling magnetic and structural properties of EuMnO3 thin films by the combined effect of Lu doping and substrate strain

Detalhes bibliográficos
Autor(a) principal: Romaguera-Barcelay, Y.
Data de Publicação: 2018
Outros Autores: Figueiras, F.G., Moreira, J. Agostinho, Pérez-de-la-Cruz, J., Tavares, P.B., Almeida, A.
Tipo de documento: Artigo
Idioma: eng
Título da fonte: Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos)
Texto Completo: http://hdl.handle.net/10773/37252
Resumo: This work aims to understand the alterations induced by film/substrate lattice mismatch in structure, lattice dynamics and magnetic response of orthorhombic Eu1-xLuxMnO3 thin films within the range 0 ≤ x ≤ 0.4, when compared to results reported for ceramics with analogous composition. Thin films, which have been deposited onto Pt/Ti/SiO2/Si(100) oriented substrates via chemical method, exhibit noteworthy modifications in the magnetic ordering properties and, contrary to ceramics, do not show any sharp phase transition to the paramagnetic state. This reveals an induced ferromagnetic response in the films which is stable up to 100 K. X-ray diffraction and Raman spectroscopy measurements have been performed to identify the mechanically compressive state induced by the substrate and Lu doping. This facilitates insight into the magnetoelastic coupling effect in these films which is driven by alterations in electronic orbital overlapping and the associated antiferromagnetic superexchange interactions.
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spelling Handling magnetic and structural properties of EuMnO3 thin films by the combined effect of Lu doping and substrate strainThin filmsRaman spectroscopyMagnetismMagnetoelastic couplingThis work aims to understand the alterations induced by film/substrate lattice mismatch in structure, lattice dynamics and magnetic response of orthorhombic Eu1-xLuxMnO3 thin films within the range 0 ≤ x ≤ 0.4, when compared to results reported for ceramics with analogous composition. Thin films, which have been deposited onto Pt/Ti/SiO2/Si(100) oriented substrates via chemical method, exhibit noteworthy modifications in the magnetic ordering properties and, contrary to ceramics, do not show any sharp phase transition to the paramagnetic state. This reveals an induced ferromagnetic response in the films which is stable up to 100 K. X-ray diffraction and Raman spectroscopy measurements have been performed to identify the mechanically compressive state induced by the substrate and Lu doping. This facilitates insight into the magnetoelastic coupling effect in these films which is driven by alterations in electronic orbital overlapping and the associated antiferromagnetic superexchange interactions.Elsevier2023-04-21T07:50:59Z2018-09-25T00:00:00Z2018-09-25info:eu-repo/semantics/publishedVersioninfo:eu-repo/semantics/articleapplication/pdfhttp://hdl.handle.net/10773/37252eng0925-838810.1016/j.jallcom.2018.05.223Romaguera-Barcelay, Y.Figueiras, F.G.Moreira, J. AgostinhoPérez-de-la-Cruz, J.Tavares, P.B.Almeida, A.info:eu-repo/semantics/openAccessreponame:Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos)instname:Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informaçãoinstacron:RCAAP2024-02-22T12:11:51Zoai:ria.ua.pt:10773/37252Portal AgregadorONGhttps://www.rcaap.pt/oai/openaireopendoar:71602024-03-20T03:07:52.001240Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) - Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informaçãofalse
dc.title.none.fl_str_mv Handling magnetic and structural properties of EuMnO3 thin films by the combined effect of Lu doping and substrate strain
title Handling magnetic and structural properties of EuMnO3 thin films by the combined effect of Lu doping and substrate strain
spellingShingle Handling magnetic and structural properties of EuMnO3 thin films by the combined effect of Lu doping and substrate strain
Romaguera-Barcelay, Y.
Thin films
Raman spectroscopy
Magnetism
Magnetoelastic coupling
title_short Handling magnetic and structural properties of EuMnO3 thin films by the combined effect of Lu doping and substrate strain
title_full Handling magnetic and structural properties of EuMnO3 thin films by the combined effect of Lu doping and substrate strain
title_fullStr Handling magnetic and structural properties of EuMnO3 thin films by the combined effect of Lu doping and substrate strain
title_full_unstemmed Handling magnetic and structural properties of EuMnO3 thin films by the combined effect of Lu doping and substrate strain
title_sort Handling magnetic and structural properties of EuMnO3 thin films by the combined effect of Lu doping and substrate strain
author Romaguera-Barcelay, Y.
author_facet Romaguera-Barcelay, Y.
Figueiras, F.G.
Moreira, J. Agostinho
Pérez-de-la-Cruz, J.
Tavares, P.B.
Almeida, A.
author_role author
author2 Figueiras, F.G.
Moreira, J. Agostinho
Pérez-de-la-Cruz, J.
Tavares, P.B.
Almeida, A.
author2_role author
author
author
author
author
dc.contributor.author.fl_str_mv Romaguera-Barcelay, Y.
Figueiras, F.G.
Moreira, J. Agostinho
Pérez-de-la-Cruz, J.
Tavares, P.B.
Almeida, A.
dc.subject.por.fl_str_mv Thin films
Raman spectroscopy
Magnetism
Magnetoelastic coupling
topic Thin films
Raman spectroscopy
Magnetism
Magnetoelastic coupling
description This work aims to understand the alterations induced by film/substrate lattice mismatch in structure, lattice dynamics and magnetic response of orthorhombic Eu1-xLuxMnO3 thin films within the range 0 ≤ x ≤ 0.4, when compared to results reported for ceramics with analogous composition. Thin films, which have been deposited onto Pt/Ti/SiO2/Si(100) oriented substrates via chemical method, exhibit noteworthy modifications in the magnetic ordering properties and, contrary to ceramics, do not show any sharp phase transition to the paramagnetic state. This reveals an induced ferromagnetic response in the films which is stable up to 100 K. X-ray diffraction and Raman spectroscopy measurements have been performed to identify the mechanically compressive state induced by the substrate and Lu doping. This facilitates insight into the magnetoelastic coupling effect in these films which is driven by alterations in electronic orbital overlapping and the associated antiferromagnetic superexchange interactions.
publishDate 2018
dc.date.none.fl_str_mv 2018-09-25T00:00:00Z
2018-09-25
2023-04-21T07:50:59Z
dc.type.status.fl_str_mv info:eu-repo/semantics/publishedVersion
dc.type.driver.fl_str_mv info:eu-repo/semantics/article
format article
status_str publishedVersion
dc.identifier.uri.fl_str_mv http://hdl.handle.net/10773/37252
url http://hdl.handle.net/10773/37252
dc.language.iso.fl_str_mv eng
language eng
dc.relation.none.fl_str_mv 0925-8388
10.1016/j.jallcom.2018.05.223
dc.rights.driver.fl_str_mv info:eu-repo/semantics/openAccess
eu_rights_str_mv openAccess
dc.format.none.fl_str_mv application/pdf
dc.publisher.none.fl_str_mv Elsevier
publisher.none.fl_str_mv Elsevier
dc.source.none.fl_str_mv reponame:Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos)
instname:Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informação
instacron:RCAAP
instname_str Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informação
instacron_str RCAAP
institution RCAAP
reponame_str Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos)
collection Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos)
repository.name.fl_str_mv Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) - Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informação
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