Superconductivity in magnetically ordered Ru1-xIr xSr2GdCu2O8 compounds
Autor(a) principal: | |
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Data de Publicação: | 2003 |
Outros Autores: | , , , , , |
Tipo de documento: | Artigo |
Idioma: | eng |
Título da fonte: | Brazilian Journal of Physics |
Texto Completo: | http://old.scielo.br/scielo.php?script=sci_arttext&pid=S0103-97332003000400009 |
Resumo: | We have performed a systematic study of the structural, transport, and magnetic properties of polycrystalline samples of the magnetic superconductors Ru1-xIr xSr2GdCu2O8; x = 0, 0.02, 0.05, 0.10, and 0.15. The samples were prepared by solid state reaction and sintered at 1060 ºC for 72 h under O2 flow. X-ray diffraction analysis shows that all samples are nearly single phase and that the lattice parameters are independent of Ir content. Transport properties measurements revealed that the Ru substitution by Ir results in a decrease of Tc,onset from ~50 K (x = 0) to ~30 K (x = 0.10). Further addition of Ir (x > 0.10) causes an evolution from metallic to nonmetallic behavior of r(T). We have also found that magnetic order develops in the undoped Ru-1212 materials near T M ~ 130 K. This temperature decreases linearly with increasing Ir content at the rate of ~ -1.6 K / Ir at.%, suggesting that Ir effectively substitutes Ru in the RuO planes. A subtle drop in r(T) is observed close to T M, probably due to the suppression of the spin-flip scattering. The magnetoresistivity measurements revealed that the temperature Tc,zero, in which r(T) ~ 0, decreases rapidly for low applied magnetic fields (H < 2 T), and that this drop becomes much less pronounced in higher magnetic fields (2 < H < 18 T). The appreciable broadening of r(T) curves at low magnetic fields is reminiscent of the behavior in high-Tc materials showing granular behavior, as for example in Sm1.85Ce0.15CuO4-y. |
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Brazilian Journal of Physics |
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Superconductivity in magnetically ordered Ru1-xIr xSr2GdCu2O8 compoundsWe have performed a systematic study of the structural, transport, and magnetic properties of polycrystalline samples of the magnetic superconductors Ru1-xIr xSr2GdCu2O8; x = 0, 0.02, 0.05, 0.10, and 0.15. The samples were prepared by solid state reaction and sintered at 1060 ºC for 72 h under O2 flow. X-ray diffraction analysis shows that all samples are nearly single phase and that the lattice parameters are independent of Ir content. Transport properties measurements revealed that the Ru substitution by Ir results in a decrease of Tc,onset from ~50 K (x = 0) to ~30 K (x = 0.10). Further addition of Ir (x > 0.10) causes an evolution from metallic to nonmetallic behavior of r(T). We have also found that magnetic order develops in the undoped Ru-1212 materials near T M ~ 130 K. This temperature decreases linearly with increasing Ir content at the rate of ~ -1.6 K / Ir at.%, suggesting that Ir effectively substitutes Ru in the RuO planes. A subtle drop in r(T) is observed close to T M, probably due to the suppression of the spin-flip scattering. The magnetoresistivity measurements revealed that the temperature Tc,zero, in which r(T) ~ 0, decreases rapidly for low applied magnetic fields (H < 2 T), and that this drop becomes much less pronounced in higher magnetic fields (2 < H < 18 T). The appreciable broadening of r(T) curves at low magnetic fields is reminiscent of the behavior in high-Tc materials showing granular behavior, as for example in Sm1.85Ce0.15CuO4-y.Sociedade Brasileira de Física2003-12-01info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersiontext/htmlhttp://old.scielo.br/scielo.php?script=sci_arttext&pid=S0103-97332003000400009Brazilian Journal of Physics v.33 n.4 2003reponame:Brazilian Journal of Physicsinstname:Sociedade Brasileira de Física (SBF)instacron:SBF10.1590/S0103-97332003000400009info:eu-repo/semantics/openAccessAndrade,S.Fonseca,F. C.Jardim,R. F.Bossi,I.Torikachvili,M. S.Lacerda,A. H.Ben-Dor,L.eng2005-11-25T00:00:00Zoai:scielo:S0103-97332003000400009Revistahttp://www.sbfisica.org.br/v1/home/index.php/pt/ONGhttps://old.scielo.br/oai/scielo-oai.phpsbfisica@sbfisica.org.br||sbfisica@sbfisica.org.br1678-44480103-9733opendoar:2005-11-25T00:00Brazilian Journal of Physics - Sociedade Brasileira de Física (SBF)false |
dc.title.none.fl_str_mv |
Superconductivity in magnetically ordered Ru1-xIr xSr2GdCu2O8 compounds |
title |
Superconductivity in magnetically ordered Ru1-xIr xSr2GdCu2O8 compounds |
spellingShingle |
Superconductivity in magnetically ordered Ru1-xIr xSr2GdCu2O8 compounds Andrade,S. |
title_short |
Superconductivity in magnetically ordered Ru1-xIr xSr2GdCu2O8 compounds |
title_full |
Superconductivity in magnetically ordered Ru1-xIr xSr2GdCu2O8 compounds |
title_fullStr |
Superconductivity in magnetically ordered Ru1-xIr xSr2GdCu2O8 compounds |
title_full_unstemmed |
Superconductivity in magnetically ordered Ru1-xIr xSr2GdCu2O8 compounds |
title_sort |
Superconductivity in magnetically ordered Ru1-xIr xSr2GdCu2O8 compounds |
author |
Andrade,S. |
author_facet |
Andrade,S. Fonseca,F. C. Jardim,R. F. Bossi,I. Torikachvili,M. S. Lacerda,A. H. Ben-Dor,L. |
author_role |
author |
author2 |
Fonseca,F. C. Jardim,R. F. Bossi,I. Torikachvili,M. S. Lacerda,A. H. Ben-Dor,L. |
author2_role |
author author author author author author |
dc.contributor.author.fl_str_mv |
Andrade,S. Fonseca,F. C. Jardim,R. F. Bossi,I. Torikachvili,M. S. Lacerda,A. H. Ben-Dor,L. |
description |
We have performed a systematic study of the structural, transport, and magnetic properties of polycrystalline samples of the magnetic superconductors Ru1-xIr xSr2GdCu2O8; x = 0, 0.02, 0.05, 0.10, and 0.15. The samples were prepared by solid state reaction and sintered at 1060 ºC for 72 h under O2 flow. X-ray diffraction analysis shows that all samples are nearly single phase and that the lattice parameters are independent of Ir content. Transport properties measurements revealed that the Ru substitution by Ir results in a decrease of Tc,onset from ~50 K (x = 0) to ~30 K (x = 0.10). Further addition of Ir (x > 0.10) causes an evolution from metallic to nonmetallic behavior of r(T). We have also found that magnetic order develops in the undoped Ru-1212 materials near T M ~ 130 K. This temperature decreases linearly with increasing Ir content at the rate of ~ -1.6 K / Ir at.%, suggesting that Ir effectively substitutes Ru in the RuO planes. A subtle drop in r(T) is observed close to T M, probably due to the suppression of the spin-flip scattering. The magnetoresistivity measurements revealed that the temperature Tc,zero, in which r(T) ~ 0, decreases rapidly for low applied magnetic fields (H < 2 T), and that this drop becomes much less pronounced in higher magnetic fields (2 < H < 18 T). The appreciable broadening of r(T) curves at low magnetic fields is reminiscent of the behavior in high-Tc materials showing granular behavior, as for example in Sm1.85Ce0.15CuO4-y. |
publishDate |
2003 |
dc.date.none.fl_str_mv |
2003-12-01 |
dc.type.driver.fl_str_mv |
info:eu-repo/semantics/article |
dc.type.status.fl_str_mv |
info:eu-repo/semantics/publishedVersion |
format |
article |
status_str |
publishedVersion |
dc.identifier.uri.fl_str_mv |
http://old.scielo.br/scielo.php?script=sci_arttext&pid=S0103-97332003000400009 |
url |
http://old.scielo.br/scielo.php?script=sci_arttext&pid=S0103-97332003000400009 |
dc.language.iso.fl_str_mv |
eng |
language |
eng |
dc.relation.none.fl_str_mv |
10.1590/S0103-97332003000400009 |
dc.rights.driver.fl_str_mv |
info:eu-repo/semantics/openAccess |
eu_rights_str_mv |
openAccess |
dc.format.none.fl_str_mv |
text/html |
dc.publisher.none.fl_str_mv |
Sociedade Brasileira de Física |
publisher.none.fl_str_mv |
Sociedade Brasileira de Física |
dc.source.none.fl_str_mv |
Brazilian Journal of Physics v.33 n.4 2003 reponame:Brazilian Journal of Physics instname:Sociedade Brasileira de Física (SBF) instacron:SBF |
instname_str |
Sociedade Brasileira de Física (SBF) |
instacron_str |
SBF |
institution |
SBF |
reponame_str |
Brazilian Journal of Physics |
collection |
Brazilian Journal of Physics |
repository.name.fl_str_mv |
Brazilian Journal of Physics - Sociedade Brasileira de Física (SBF) |
repository.mail.fl_str_mv |
sbfisica@sbfisica.org.br||sbfisica@sbfisica.org.br |
_version_ |
1754734860448038912 |