Atmospheric aerosols in Amazonia and land use change: from natural biogenic to biomass burning conditions

Detalhes bibliográficos
Autor(a) principal: Artaxo, Paulo
Data de Publicação: 2013
Outros Autores: Rizzo, Luciana Varanda [UNIFESP], Brito, Joel F., Barbosa, Henrique M. J., Arana, Andrea, Sena, Elisa T., Cirino, Glauber G., Bastos, Wanderlei, Martin, Scot T., Andreae, Meinrat O.
Tipo de documento: Artigo
Idioma: eng
Título da fonte: Repositório Institucional da UNIFESP
Texto Completo: http://repositorio.unifesp.br/handle/11600/35658
http://dx.doi.org/10.1039/c3fd00052d
Resumo: In the wet season, a large portion of the Amazon region constitutes one of the most pristine continental areas, with very low concentrations of atmospheric trace gases and aerosol particles. However, land use change modifies the biosphere-atmosphere interactions in such a way that key processes that maintain the functioning of Amazonia are substantially altered. This study presents a comparison between aerosol properties observed at a preserved forest site in Central Amazonia (TT34 North of Manaus) and at a heavily biomass burning impacted site in south-western Amazonia (PVH, close to Porto Velho). Amazonian aerosols were characterized in detail, including aerosol size distributions, aerosol light absorption and scattering, optical depth and aerosol inorganic and organic composition, among other properties. the central Amazonia site (TT34) showed low aerosol concentrations (PM2.5 of 1.3 +/- 0.7 mu g m(-3) and 3.4 +/- 2.0 mu g m(-3) in the wet and dry seasons, respectively), with a median particle number concentration of 220 cm(-3) in the wet season and 2200 cm(-3) in the dry season. At the impacted site (PVH), aerosol loadings were one order of magnitude higher (PM2.5 of 10.2 +/- 9.0 mu g m(-3) and 33.0 +/- 36.0 mu g m(-3) in the wet and dry seasons, respectively). the aerosol number concentration at the impacted site ranged from 680 cm(-3) in the wet season up to 20 000 cm(-3) in the dry season. An aerosol chemical speciation monitor (ACSM) was deployed in 2013 at both sites, and it shows that
id UFSP_41ebbf6f31ebac9eed8ee42a8abc4321
oai_identifier_str oai:repositorio.unifesp.br:11600/35658
network_acronym_str UFSP
network_name_str Repositório Institucional da UNIFESP
repository_id_str 3465
spelling Artaxo, PauloRizzo, Luciana Varanda [UNIFESP]Brito, Joel F.Barbosa, Henrique M. J.Arana, AndreaSena, Elisa T.Cirino, Glauber G.Bastos, WanderleiMartin, Scot T.Andreae, Meinrat O.Universidade de São Paulo (USP)Universidade Federal de São Paulo (UNIFESP)INPAUniv Fed Rondonia UNIRHarvard UnivMax Planck Inst Chem2016-01-24T14:30:50Z2016-01-24T14:30:50Z2013-01-01Faraday Discussions. Cambridge: Royal Soc Chemistry, v. 165, p. 203-235, 2013.1359-6640http://repositorio.unifesp.br/handle/11600/35658http://dx.doi.org/10.1039/c3fd00052dWOS000329068600011.pdf10.1039/c3fd00052dWOS:000329068600011In the wet season, a large portion of the Amazon region constitutes one of the most pristine continental areas, with very low concentrations of atmospheric trace gases and aerosol particles. However, land use change modifies the biosphere-atmosphere interactions in such a way that key processes that maintain the functioning of Amazonia are substantially altered. This study presents a comparison between aerosol properties observed at a preserved forest site in Central Amazonia (TT34 North of Manaus) and at a heavily biomass burning impacted site in south-western Amazonia (PVH, close to Porto Velho). Amazonian aerosols were characterized in detail, including aerosol size distributions, aerosol light absorption and scattering, optical depth and aerosol inorganic and organic composition, among other properties. the central Amazonia site (TT34) showed low aerosol concentrations (PM2.5 of 1.3 +/- 0.7 mu g m(-3) and 3.4 +/- 2.0 mu g m(-3) in the wet and dry seasons, respectively), with a median particle number concentration of 220 cm(-3) in the wet season and 2200 cm(-3) in the dry season. At the impacted site (PVH), aerosol loadings were one order of magnitude higher (PM2.5 of 10.2 +/- 9.0 mu g m(-3) and 33.0 +/- 36.0 mu g m(-3) in the wet and dry seasons, respectively). the aerosol number concentration at the impacted site ranged from 680 cm(-3) in the wet season up to 20 000 cm(-3) in the dry season. An aerosol chemical speciation monitor (ACSM) was deployed in 2013 at both sites, and it shows thatFundação de Amparo à Pesquisa do Estado de São Paulo (FAPESP)Conselho Nacional de Desenvolvimento Científico e Tecnológico (CNPq)INCT AmazoniaFP6 project EUCAARIMax Planck SocietyUniv São Paulo, Inst Phys, BR-05508090 São Paulo, BrazilUniversidade Federal de São Paulo, Inst Environm Chem & Pharmaceut Sci, Dept Earth & Exact Sci, BR-09972270 Diadema São Paulo, BrazilINPA, BR-69067375 Manaus, Amazonas, BrazilUniv Fed Rondonia UNIR, Lab Biogeoquim Ambiental Wolfgang C Pfeiffer, Rondonia, BrazilHarvard Univ, Sch Engn & Appl Sci, Cambridge, MA 02138 USAHarvard Univ, Dept Earth & Planetary Sci, Cambridge, MA 02138 USAMax Planck Inst Chem, Biogeochem Dept, D-55020 Mainz, GermanyUniversidade Federal de São Paulo, Inst Environm Chem & Pharmaceut Sci, Dept Earth & Exact Sci, BR-09972270 Diadema São Paulo, BrazilFAPESP: 2008/58100-2FAPESP: 2010/52658-1FAPESP: 2011/50170-4FAPESP: 2012/14437-9CNPq: 475735-2012-9FP6 project EUCAARI: 34684Web of Science203-235engRoyal Soc ChemistryFaraday DiscussionsAtmospheric aerosols in Amazonia and land use change: from natural biogenic to biomass burning conditionsinfo:eu-repo/semantics/publishedVersioninfo:eu-repo/semantics/articleinfo:eu-repo/semantics/openAccessreponame:Repositório Institucional da UNIFESPinstname:Universidade Federal de São Paulo (UNIFESP)instacron:UNIFESPORIGINALWOS000329068600011.pdfapplication/pdf2261687${dspace.ui.url}/bitstream/11600/35658/1/WOS000329068600011.pdfced01f1806b099362ea8643c05483b54MD51open accessTEXTWOS000329068600011.pdf.txtWOS000329068600011.pdf.txtExtracted texttext/plain104605${dspace.ui.url}/bitstream/11600/35658/9/WOS000329068600011.pdf.txt1ac12fbacde569b5ad6058e55dd510c7MD59open accessTHUMBNAILWOS000329068600011.pdf.jpgWOS000329068600011.pdf.jpgIM Thumbnailimage/jpeg6645${dspace.ui.url}/bitstream/11600/35658/11/WOS000329068600011.pdf.jpg21b49c53926754d6761b76632f604ad2MD511open access11600/356582023-06-05 19:24:04.148open accessoai:repositorio.unifesp.br:11600/35658Repositório InstitucionalPUBhttp://www.repositorio.unifesp.br/oai/requestopendoar:34652023-06-05T22:24:04Repositório Institucional da UNIFESP - Universidade Federal de São Paulo (UNIFESP)false
dc.title.en.fl_str_mv Atmospheric aerosols in Amazonia and land use change: from natural biogenic to biomass burning conditions
title Atmospheric aerosols in Amazonia and land use change: from natural biogenic to biomass burning conditions
spellingShingle Atmospheric aerosols in Amazonia and land use change: from natural biogenic to biomass burning conditions
Artaxo, Paulo
title_short Atmospheric aerosols in Amazonia and land use change: from natural biogenic to biomass burning conditions
title_full Atmospheric aerosols in Amazonia and land use change: from natural biogenic to biomass burning conditions
title_fullStr Atmospheric aerosols in Amazonia and land use change: from natural biogenic to biomass burning conditions
title_full_unstemmed Atmospheric aerosols in Amazonia and land use change: from natural biogenic to biomass burning conditions
title_sort Atmospheric aerosols in Amazonia and land use change: from natural biogenic to biomass burning conditions
author Artaxo, Paulo
author_facet Artaxo, Paulo
Rizzo, Luciana Varanda [UNIFESP]
Brito, Joel F.
Barbosa, Henrique M. J.
Arana, Andrea
Sena, Elisa T.
Cirino, Glauber G.
Bastos, Wanderlei
Martin, Scot T.
Andreae, Meinrat O.
author_role author
author2 Rizzo, Luciana Varanda [UNIFESP]
Brito, Joel F.
Barbosa, Henrique M. J.
Arana, Andrea
Sena, Elisa T.
Cirino, Glauber G.
Bastos, Wanderlei
Martin, Scot T.
Andreae, Meinrat O.
author2_role author
author
author
author
author
author
author
author
author
dc.contributor.institution.none.fl_str_mv Universidade de São Paulo (USP)
Universidade Federal de São Paulo (UNIFESP)
INPA
Univ Fed Rondonia UNIR
Harvard Univ
Max Planck Inst Chem
dc.contributor.author.fl_str_mv Artaxo, Paulo
Rizzo, Luciana Varanda [UNIFESP]
Brito, Joel F.
Barbosa, Henrique M. J.
Arana, Andrea
Sena, Elisa T.
Cirino, Glauber G.
Bastos, Wanderlei
Martin, Scot T.
Andreae, Meinrat O.
description In the wet season, a large portion of the Amazon region constitutes one of the most pristine continental areas, with very low concentrations of atmospheric trace gases and aerosol particles. However, land use change modifies the biosphere-atmosphere interactions in such a way that key processes that maintain the functioning of Amazonia are substantially altered. This study presents a comparison between aerosol properties observed at a preserved forest site in Central Amazonia (TT34 North of Manaus) and at a heavily biomass burning impacted site in south-western Amazonia (PVH, close to Porto Velho). Amazonian aerosols were characterized in detail, including aerosol size distributions, aerosol light absorption and scattering, optical depth and aerosol inorganic and organic composition, among other properties. the central Amazonia site (TT34) showed low aerosol concentrations (PM2.5 of 1.3 +/- 0.7 mu g m(-3) and 3.4 +/- 2.0 mu g m(-3) in the wet and dry seasons, respectively), with a median particle number concentration of 220 cm(-3) in the wet season and 2200 cm(-3) in the dry season. At the impacted site (PVH), aerosol loadings were one order of magnitude higher (PM2.5 of 10.2 +/- 9.0 mu g m(-3) and 33.0 +/- 36.0 mu g m(-3) in the wet and dry seasons, respectively). the aerosol number concentration at the impacted site ranged from 680 cm(-3) in the wet season up to 20 000 cm(-3) in the dry season. An aerosol chemical speciation monitor (ACSM) was deployed in 2013 at both sites, and it shows that
publishDate 2013
dc.date.issued.fl_str_mv 2013-01-01
dc.date.accessioned.fl_str_mv 2016-01-24T14:30:50Z
dc.date.available.fl_str_mv 2016-01-24T14:30:50Z
dc.type.status.fl_str_mv info:eu-repo/semantics/publishedVersion
dc.type.driver.fl_str_mv info:eu-repo/semantics/article
format article
status_str publishedVersion
dc.identifier.citation.fl_str_mv Faraday Discussions. Cambridge: Royal Soc Chemistry, v. 165, p. 203-235, 2013.
dc.identifier.uri.fl_str_mv http://repositorio.unifesp.br/handle/11600/35658
http://dx.doi.org/10.1039/c3fd00052d
dc.identifier.issn.none.fl_str_mv 1359-6640
dc.identifier.file.none.fl_str_mv WOS000329068600011.pdf
dc.identifier.doi.none.fl_str_mv 10.1039/c3fd00052d
dc.identifier.wos.none.fl_str_mv WOS:000329068600011
identifier_str_mv Faraday Discussions. Cambridge: Royal Soc Chemistry, v. 165, p. 203-235, 2013.
1359-6640
WOS000329068600011.pdf
10.1039/c3fd00052d
WOS:000329068600011
url http://repositorio.unifesp.br/handle/11600/35658
http://dx.doi.org/10.1039/c3fd00052d
dc.language.iso.fl_str_mv eng
language eng
dc.relation.ispartof.none.fl_str_mv Faraday Discussions
dc.rights.driver.fl_str_mv info:eu-repo/semantics/openAccess
eu_rights_str_mv openAccess
dc.format.none.fl_str_mv 203-235
dc.publisher.none.fl_str_mv Royal Soc Chemistry
publisher.none.fl_str_mv Royal Soc Chemistry
dc.source.none.fl_str_mv reponame:Repositório Institucional da UNIFESP
instname:Universidade Federal de São Paulo (UNIFESP)
instacron:UNIFESP
instname_str Universidade Federal de São Paulo (UNIFESP)
instacron_str UNIFESP
institution UNIFESP
reponame_str Repositório Institucional da UNIFESP
collection Repositório Institucional da UNIFESP
bitstream.url.fl_str_mv ${dspace.ui.url}/bitstream/11600/35658/1/WOS000329068600011.pdf
${dspace.ui.url}/bitstream/11600/35658/9/WOS000329068600011.pdf.txt
${dspace.ui.url}/bitstream/11600/35658/11/WOS000329068600011.pdf.jpg
bitstream.checksum.fl_str_mv ced01f1806b099362ea8643c05483b54
1ac12fbacde569b5ad6058e55dd510c7
21b49c53926754d6761b76632f604ad2
bitstream.checksumAlgorithm.fl_str_mv MD5
MD5
MD5
repository.name.fl_str_mv Repositório Institucional da UNIFESP - Universidade Federal de São Paulo (UNIFESP)
repository.mail.fl_str_mv
_version_ 1802764183188537344