Atmospheric aerosols in Amazonia and land use change: from natural biogenic to biomass burning conditions
Autor(a) principal: | |
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Data de Publicação: | 2013 |
Outros Autores: | , , , , , , , , |
Tipo de documento: | Artigo |
Idioma: | eng |
Título da fonte: | Repositório Institucional da UNIFESP |
Texto Completo: | http://dx.doi.org/10.1039/c3fd00052d http://repositorio.unifesp.br/handle/11600/35658 |
Resumo: | In the wet season, a large portion of the Amazon region constitutes one of the most pristine continental areas, with very low concentrations of atmospheric trace gases and aerosol particles. However, land use change modifies the biosphere-atmosphere interactions in such a way that key processes that maintain the functioning of Amazonia are substantially altered. This study presents a comparison between aerosol properties observed at a preserved forest site in Central Amazonia (TT34 North of Manaus) and at a heavily biomass burning impacted site in south-western Amazonia (PVH, close to Porto Velho). Amazonian aerosols were characterized in detail, including aerosol size distributions, aerosol light absorption and scattering, optical depth and aerosol inorganic and organic composition, among other properties. the central Amazonia site (TT34) showed low aerosol concentrations (PM2.5 of 1.3 +/- 0.7 mu g m(-3) and 3.4 +/- 2.0 mu g m(-3) in the wet and dry seasons, respectively), with a median particle number concentration of 220 cm(-3) in the wet season and 2200 cm(-3) in the dry season. At the impacted site (PVH), aerosol loadings were one order of magnitude higher (PM2.5 of 10.2 +/- 9.0 mu g m(-3) and 33.0 +/- 36.0 mu g m(-3) in the wet and dry seasons, respectively). the aerosol number concentration at the impacted site ranged from 680 cm(-3) in the wet season up to 20 000 cm(-3) in the dry season. An aerosol chemical speciation monitor (ACSM) was deployed in 2013 at both sites, and it shows that |
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Atmospheric aerosols in Amazonia and land use change: from natural biogenic to biomass burning conditionsIn the wet season, a large portion of the Amazon region constitutes one of the most pristine continental areas, with very low concentrations of atmospheric trace gases and aerosol particles. However, land use change modifies the biosphere-atmosphere interactions in such a way that key processes that maintain the functioning of Amazonia are substantially altered. This study presents a comparison between aerosol properties observed at a preserved forest site in Central Amazonia (TT34 North of Manaus) and at a heavily biomass burning impacted site in south-western Amazonia (PVH, close to Porto Velho). Amazonian aerosols were characterized in detail, including aerosol size distributions, aerosol light absorption and scattering, optical depth and aerosol inorganic and organic composition, among other properties. the central Amazonia site (TT34) showed low aerosol concentrations (PM2.5 of 1.3 +/- 0.7 mu g m(-3) and 3.4 +/- 2.0 mu g m(-3) in the wet and dry seasons, respectively), with a median particle number concentration of 220 cm(-3) in the wet season and 2200 cm(-3) in the dry season. At the impacted site (PVH), aerosol loadings were one order of magnitude higher (PM2.5 of 10.2 +/- 9.0 mu g m(-3) and 33.0 +/- 36.0 mu g m(-3) in the wet and dry seasons, respectively). the aerosol number concentration at the impacted site ranged from 680 cm(-3) in the wet season up to 20 000 cm(-3) in the dry season. An aerosol chemical speciation monitor (ACSM) was deployed in 2013 at both sites, and it shows thatUniv São Paulo, Inst Phys, BR-05508090 São Paulo, BrazilUniversidade Federal de São Paulo, Inst Environm Chem & Pharmaceut Sci, Dept Earth & Exact Sci, BR-09972270 Diadema São Paulo, BrazilINPA, BR-69067375 Manaus, Amazonas, BrazilUniv Fed Rondonia UNIR, Lab Biogeoquim Ambiental Wolfgang C Pfeiffer, Rondonia, BrazilHarvard Univ, Sch Engn & Appl Sci, Cambridge, MA 02138 USAHarvard Univ, Dept Earth & Planetary Sci, Cambridge, MA 02138 USAMax Planck Inst Chem, Biogeochem Dept, D-55020 Mainz, GermanyUniversidade Federal de São Paulo, Inst Environm Chem & Pharmaceut Sci, Dept Earth & Exact Sci, BR-09972270 Diadema São Paulo, BrazilWeb of ScienceFundação de Amparo à Pesquisa do Estado de São Paulo (FAPESP)Conselho Nacional de Desenvolvimento Científico e Tecnológico (CNPq)INCT AmazoniaFP6 project EUCAARIMax Planck SocietyFAPESP: 2008/58100-2FAPESP: 2010/52658-1FAPESP: 2011/50170-4FAPESP: 2012/14437-9CNPq: 475735-2012-9FP6 project EUCAARI: 34684Royal Soc ChemistryUniversidade de São Paulo (USP)Universidade Federal de São Paulo (UNIFESP)INPAUniv Fed Rondonia UNIRHarvard UnivMax Planck Inst ChemArtaxo, PauloRizzo, Luciana Varanda [UNIFESP]Brito, Joel F.Barbosa, Henrique M. J.Arana, AndreaSena, Elisa T.Cirino, Glauber G.Bastos, WanderleiMartin, Scot T.Andreae, Meinrat O.2016-01-24T14:30:50Z2016-01-24T14:30:50Z2013-01-01info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersion203-235application/pdfhttp://dx.doi.org/10.1039/c3fd00052dFaraday Discussions. Cambridge: Royal Soc Chemistry, v. 165, p. 203-235, 2013.10.1039/c3fd00052dWOS000329068600011.pdf1359-6640http://repositorio.unifesp.br/handle/11600/35658WOS:000329068600011engFaraday Discussionsinfo:eu-repo/semantics/openAccessreponame:Repositório Institucional da UNIFESPinstname:Universidade Federal de São Paulo (UNIFESP)instacron:UNIFESP2024-08-08T17:07:07Zoai:repositorio.unifesp.br/:11600/35658Repositório InstitucionalPUBhttp://www.repositorio.unifesp.br/oai/requestbiblioteca.csp@unifesp.bropendoar:34652024-08-08T17:07:07Repositório Institucional da UNIFESP - Universidade Federal de São Paulo (UNIFESP)false |
dc.title.none.fl_str_mv |
Atmospheric aerosols in Amazonia and land use change: from natural biogenic to biomass burning conditions |
title |
Atmospheric aerosols in Amazonia and land use change: from natural biogenic to biomass burning conditions |
spellingShingle |
Atmospheric aerosols in Amazonia and land use change: from natural biogenic to biomass burning conditions Artaxo, Paulo |
title_short |
Atmospheric aerosols in Amazonia and land use change: from natural biogenic to biomass burning conditions |
title_full |
Atmospheric aerosols in Amazonia and land use change: from natural biogenic to biomass burning conditions |
title_fullStr |
Atmospheric aerosols in Amazonia and land use change: from natural biogenic to biomass burning conditions |
title_full_unstemmed |
Atmospheric aerosols in Amazonia and land use change: from natural biogenic to biomass burning conditions |
title_sort |
Atmospheric aerosols in Amazonia and land use change: from natural biogenic to biomass burning conditions |
author |
Artaxo, Paulo |
author_facet |
Artaxo, Paulo Rizzo, Luciana Varanda [UNIFESP] Brito, Joel F. Barbosa, Henrique M. J. Arana, Andrea Sena, Elisa T. Cirino, Glauber G. Bastos, Wanderlei Martin, Scot T. Andreae, Meinrat O. |
author_role |
author |
author2 |
Rizzo, Luciana Varanda [UNIFESP] Brito, Joel F. Barbosa, Henrique M. J. Arana, Andrea Sena, Elisa T. Cirino, Glauber G. Bastos, Wanderlei Martin, Scot T. Andreae, Meinrat O. |
author2_role |
author author author author author author author author author |
dc.contributor.none.fl_str_mv |
Universidade de São Paulo (USP) Universidade Federal de São Paulo (UNIFESP) INPA Univ Fed Rondonia UNIR Harvard Univ Max Planck Inst Chem |
dc.contributor.author.fl_str_mv |
Artaxo, Paulo Rizzo, Luciana Varanda [UNIFESP] Brito, Joel F. Barbosa, Henrique M. J. Arana, Andrea Sena, Elisa T. Cirino, Glauber G. Bastos, Wanderlei Martin, Scot T. Andreae, Meinrat O. |
description |
In the wet season, a large portion of the Amazon region constitutes one of the most pristine continental areas, with very low concentrations of atmospheric trace gases and aerosol particles. However, land use change modifies the biosphere-atmosphere interactions in such a way that key processes that maintain the functioning of Amazonia are substantially altered. This study presents a comparison between aerosol properties observed at a preserved forest site in Central Amazonia (TT34 North of Manaus) and at a heavily biomass burning impacted site in south-western Amazonia (PVH, close to Porto Velho). Amazonian aerosols were characterized in detail, including aerosol size distributions, aerosol light absorption and scattering, optical depth and aerosol inorganic and organic composition, among other properties. the central Amazonia site (TT34) showed low aerosol concentrations (PM2.5 of 1.3 +/- 0.7 mu g m(-3) and 3.4 +/- 2.0 mu g m(-3) in the wet and dry seasons, respectively), with a median particle number concentration of 220 cm(-3) in the wet season and 2200 cm(-3) in the dry season. At the impacted site (PVH), aerosol loadings were one order of magnitude higher (PM2.5 of 10.2 +/- 9.0 mu g m(-3) and 33.0 +/- 36.0 mu g m(-3) in the wet and dry seasons, respectively). the aerosol number concentration at the impacted site ranged from 680 cm(-3) in the wet season up to 20 000 cm(-3) in the dry season. An aerosol chemical speciation monitor (ACSM) was deployed in 2013 at both sites, and it shows that |
publishDate |
2013 |
dc.date.none.fl_str_mv |
2013-01-01 2016-01-24T14:30:50Z 2016-01-24T14:30:50Z |
dc.type.driver.fl_str_mv |
info:eu-repo/semantics/article |
dc.type.status.fl_str_mv |
info:eu-repo/semantics/publishedVersion |
format |
article |
status_str |
publishedVersion |
dc.identifier.uri.fl_str_mv |
http://dx.doi.org/10.1039/c3fd00052d Faraday Discussions. Cambridge: Royal Soc Chemistry, v. 165, p. 203-235, 2013. 10.1039/c3fd00052d WOS000329068600011.pdf 1359-6640 http://repositorio.unifesp.br/handle/11600/35658 WOS:000329068600011 |
url |
http://dx.doi.org/10.1039/c3fd00052d http://repositorio.unifesp.br/handle/11600/35658 |
identifier_str_mv |
Faraday Discussions. Cambridge: Royal Soc Chemistry, v. 165, p. 203-235, 2013. 10.1039/c3fd00052d WOS000329068600011.pdf 1359-6640 WOS:000329068600011 |
dc.language.iso.fl_str_mv |
eng |
language |
eng |
dc.relation.none.fl_str_mv |
Faraday Discussions |
dc.rights.driver.fl_str_mv |
info:eu-repo/semantics/openAccess |
eu_rights_str_mv |
openAccess |
dc.format.none.fl_str_mv |
203-235 application/pdf |
dc.publisher.none.fl_str_mv |
Royal Soc Chemistry |
publisher.none.fl_str_mv |
Royal Soc Chemistry |
dc.source.none.fl_str_mv |
reponame:Repositório Institucional da UNIFESP instname:Universidade Federal de São Paulo (UNIFESP) instacron:UNIFESP |
instname_str |
Universidade Federal de São Paulo (UNIFESP) |
instacron_str |
UNIFESP |
institution |
UNIFESP |
reponame_str |
Repositório Institucional da UNIFESP |
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Repositório Institucional da UNIFESP |
repository.name.fl_str_mv |
Repositório Institucional da UNIFESP - Universidade Federal de São Paulo (UNIFESP) |
repository.mail.fl_str_mv |
biblioteca.csp@unifesp.br |
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