Metallic islands in the Kondo insulator SmB6
Autor(a) principal: | |
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Data de Publicação: | 2020 |
Outros Autores: | , , , , , , , , |
Tipo de documento: | Artigo |
Idioma: | eng |
Título da fonte: | Repositório Institucional da UNESP |
DOI: | 10.1103/PhysRevResearch.2.043181 |
Texto Completo: | http://dx.doi.org/10.1103/PhysRevResearch.2.043181 http://hdl.handle.net/11449/221752 |
Resumo: | The predicted interplay between Kondo physics and nontrivial topology in SmB6 has stimulated many experimental reports, some of which are in apparent contradiction. The origin of the dispute may lie in the fragility of the Kondo insulating phase in the presence of Sm vacancies (Kondo holes) and/or natural impurities, such as Gd3+. In this work, we locally investigate this fragility for Al flux grown Sm1-xGdxB6 single crystals (0≤x≤0.02) by combining electron spin resonance (ESR) and complementary bulk measurements. The Gd3+ ESR spectra in a highly dilute regime (x∼0.0004) display the features of an insulating cubic environment. Remarkably, a metallic ESR line shape is observed for more concentrated samples (x≥0.004), even though these systems are still in a reasonably dilute regime and show insulating dc electrical resistivity. Our data indicate that the Kondo insulating state is destroyed locally around impurities before a global percolation occurs. This result not only explains the discrepancy between dc and ac conductivity but also provides a scenario to explain the presence of quantum oscillations in magnetization in the absence of quantum oscillations in electrical resistivity. |
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Metallic islands in the Kondo insulator SmB6The predicted interplay between Kondo physics and nontrivial topology in SmB6 has stimulated many experimental reports, some of which are in apparent contradiction. The origin of the dispute may lie in the fragility of the Kondo insulating phase in the presence of Sm vacancies (Kondo holes) and/or natural impurities, such as Gd3+. In this work, we locally investigate this fragility for Al flux grown Sm1-xGdxB6 single crystals (0≤x≤0.02) by combining electron spin resonance (ESR) and complementary bulk measurements. The Gd3+ ESR spectra in a highly dilute regime (x∼0.0004) display the features of an insulating cubic environment. Remarkably, a metallic ESR line shape is observed for more concentrated samples (x≥0.004), even though these systems are still in a reasonably dilute regime and show insulating dc electrical resistivity. Our data indicate that the Kondo insulating state is destroyed locally around impurities before a global percolation occurs. This result not only explains the discrepancy between dc and ac conductivity but also provides a scenario to explain the presence of quantum oscillations in magnetization in the absence of quantum oscillations in electrical resistivity.Instituto de Física Gleb Wataghin UNICAMPMax Planck Institute for Chemical Physics of SolidsLos Alamos National LaboratoryPOSMAT Faculdade de Ciências UNESP, C.P. 473Departamento de Física Faculdade de Ciências UNESP, C.P. 473Department of Physics and Astronomy University of CaliforniaPOSMAT Faculdade de Ciências UNESP, C.P. 473Departamento de Física Faculdade de Ciências UNESP, C.P. 473Universidade Estadual de Campinas (UNICAMP)Max Planck Institute for Chemical Physics of SolidsLos Alamos National LaboratoryUniversidade Estadual Paulista (UNESP)University of CaliforniaSouza, J. C.Rosa, P. F.S.Sichelschmidt, J.Carlone, M. [UNESP]Venegas, P. A. [UNESP]Malcolms, M. O.Menegasso, P. M.Urbano, R. R.Fisk, Z.Pagliuso, P. G.2022-04-28T19:40:15Z2022-04-28T19:40:15Z2020-11-03info:eu-repo/semantics/publishedVersioninfo:eu-repo/semantics/articlehttp://dx.doi.org/10.1103/PhysRevResearch.2.043181Physical Review Research, v. 2, n. 4, 2020.2643-1564http://hdl.handle.net/11449/22175210.1103/PhysRevResearch.2.0431812-s2.0-85106381837Scopusreponame:Repositório Institucional da UNESPinstname:Universidade Estadual Paulista (UNESP)instacron:UNESPengPhysical Review Researchinfo:eu-repo/semantics/openAccess2022-04-28T19:40:15Zoai:repositorio.unesp.br:11449/221752Repositório InstitucionalPUBhttp://repositorio.unesp.br/oai/requestopendoar:29462024-08-05T21:57:05.519316Repositório Institucional da UNESP - Universidade Estadual Paulista (UNESP)false |
dc.title.none.fl_str_mv |
Metallic islands in the Kondo insulator SmB6 |
title |
Metallic islands in the Kondo insulator SmB6 |
spellingShingle |
Metallic islands in the Kondo insulator SmB6 Metallic islands in the Kondo insulator SmB6 Souza, J. C. Souza, J. C. |
title_short |
Metallic islands in the Kondo insulator SmB6 |
title_full |
Metallic islands in the Kondo insulator SmB6 |
title_fullStr |
Metallic islands in the Kondo insulator SmB6 Metallic islands in the Kondo insulator SmB6 |
title_full_unstemmed |
Metallic islands in the Kondo insulator SmB6 Metallic islands in the Kondo insulator SmB6 |
title_sort |
Metallic islands in the Kondo insulator SmB6 |
author |
Souza, J. C. |
author_facet |
Souza, J. C. Souza, J. C. Rosa, P. F.S. Sichelschmidt, J. Carlone, M. [UNESP] Venegas, P. A. [UNESP] Malcolms, M. O. Menegasso, P. M. Urbano, R. R. Fisk, Z. Pagliuso, P. G. Rosa, P. F.S. Sichelschmidt, J. Carlone, M. [UNESP] Venegas, P. A. [UNESP] Malcolms, M. O. Menegasso, P. M. Urbano, R. R. Fisk, Z. Pagliuso, P. G. |
author_role |
author |
author2 |
Rosa, P. F.S. Sichelschmidt, J. Carlone, M. [UNESP] Venegas, P. A. [UNESP] Malcolms, M. O. Menegasso, P. M. Urbano, R. R. Fisk, Z. Pagliuso, P. G. |
author2_role |
author author author author author author author author author |
dc.contributor.none.fl_str_mv |
Universidade Estadual de Campinas (UNICAMP) Max Planck Institute for Chemical Physics of Solids Los Alamos National Laboratory Universidade Estadual Paulista (UNESP) University of California |
dc.contributor.author.fl_str_mv |
Souza, J. C. Rosa, P. F.S. Sichelschmidt, J. Carlone, M. [UNESP] Venegas, P. A. [UNESP] Malcolms, M. O. Menegasso, P. M. Urbano, R. R. Fisk, Z. Pagliuso, P. G. |
description |
The predicted interplay between Kondo physics and nontrivial topology in SmB6 has stimulated many experimental reports, some of which are in apparent contradiction. The origin of the dispute may lie in the fragility of the Kondo insulating phase in the presence of Sm vacancies (Kondo holes) and/or natural impurities, such as Gd3+. In this work, we locally investigate this fragility for Al flux grown Sm1-xGdxB6 single crystals (0≤x≤0.02) by combining electron spin resonance (ESR) and complementary bulk measurements. The Gd3+ ESR spectra in a highly dilute regime (x∼0.0004) display the features of an insulating cubic environment. Remarkably, a metallic ESR line shape is observed for more concentrated samples (x≥0.004), even though these systems are still in a reasonably dilute regime and show insulating dc electrical resistivity. Our data indicate that the Kondo insulating state is destroyed locally around impurities before a global percolation occurs. This result not only explains the discrepancy between dc and ac conductivity but also provides a scenario to explain the presence of quantum oscillations in magnetization in the absence of quantum oscillations in electrical resistivity. |
publishDate |
2020 |
dc.date.none.fl_str_mv |
2020-11-03 2022-04-28T19:40:15Z 2022-04-28T19:40:15Z |
dc.type.status.fl_str_mv |
info:eu-repo/semantics/publishedVersion |
dc.type.driver.fl_str_mv |
info:eu-repo/semantics/article |
format |
article |
status_str |
publishedVersion |
dc.identifier.uri.fl_str_mv |
http://dx.doi.org/10.1103/PhysRevResearch.2.043181 Physical Review Research, v. 2, n. 4, 2020. 2643-1564 http://hdl.handle.net/11449/221752 10.1103/PhysRevResearch.2.043181 2-s2.0-85106381837 |
url |
http://dx.doi.org/10.1103/PhysRevResearch.2.043181 http://hdl.handle.net/11449/221752 |
identifier_str_mv |
Physical Review Research, v. 2, n. 4, 2020. 2643-1564 10.1103/PhysRevResearch.2.043181 2-s2.0-85106381837 |
dc.language.iso.fl_str_mv |
eng |
language |
eng |
dc.relation.none.fl_str_mv |
Physical Review Research |
dc.rights.driver.fl_str_mv |
info:eu-repo/semantics/openAccess |
eu_rights_str_mv |
openAccess |
dc.source.none.fl_str_mv |
Scopus reponame:Repositório Institucional da UNESP instname:Universidade Estadual Paulista (UNESP) instacron:UNESP |
instname_str |
Universidade Estadual Paulista (UNESP) |
instacron_str |
UNESP |
institution |
UNESP |
reponame_str |
Repositório Institucional da UNESP |
collection |
Repositório Institucional da UNESP |
repository.name.fl_str_mv |
Repositório Institucional da UNESP - Universidade Estadual Paulista (UNESP) |
repository.mail.fl_str_mv |
|
_version_ |
1822228706068791296 |
dc.identifier.doi.none.fl_str_mv |
10.1103/PhysRevResearch.2.043181 |