Metallic islands in the Kondo insulator SmB6

Detalhes bibliográficos
Autor(a) principal: Souza, J. C.
Data de Publicação: 2020
Outros Autores: Rosa, P. F.S., Sichelschmidt, J., Carlone, M. [UNESP], Venegas, P. A. [UNESP], Malcolms, M. O., Menegasso, P. M., Urbano, R. R., Fisk, Z., Pagliuso, P. G.
Tipo de documento: Artigo
Idioma: eng
Título da fonte: Repositório Institucional da UNESP
DOI: 10.1103/PhysRevResearch.2.043181
Texto Completo: http://dx.doi.org/10.1103/PhysRevResearch.2.043181
http://hdl.handle.net/11449/221752
Resumo: The predicted interplay between Kondo physics and nontrivial topology in SmB6 has stimulated many experimental reports, some of which are in apparent contradiction. The origin of the dispute may lie in the fragility of the Kondo insulating phase in the presence of Sm vacancies (Kondo holes) and/or natural impurities, such as Gd3+. In this work, we locally investigate this fragility for Al flux grown Sm1-xGdxB6 single crystals (0≤x≤0.02) by combining electron spin resonance (ESR) and complementary bulk measurements. The Gd3+ ESR spectra in a highly dilute regime (x∼0.0004) display the features of an insulating cubic environment. Remarkably, a metallic ESR line shape is observed for more concentrated samples (x≥0.004), even though these systems are still in a reasonably dilute regime and show insulating dc electrical resistivity. Our data indicate that the Kondo insulating state is destroyed locally around impurities before a global percolation occurs. This result not only explains the discrepancy between dc and ac conductivity but also provides a scenario to explain the presence of quantum oscillations in magnetization in the absence of quantum oscillations in electrical resistivity.
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spelling Metallic islands in the Kondo insulator SmB6The predicted interplay between Kondo physics and nontrivial topology in SmB6 has stimulated many experimental reports, some of which are in apparent contradiction. The origin of the dispute may lie in the fragility of the Kondo insulating phase in the presence of Sm vacancies (Kondo holes) and/or natural impurities, such as Gd3+. In this work, we locally investigate this fragility for Al flux grown Sm1-xGdxB6 single crystals (0≤x≤0.02) by combining electron spin resonance (ESR) and complementary bulk measurements. The Gd3+ ESR spectra in a highly dilute regime (x∼0.0004) display the features of an insulating cubic environment. Remarkably, a metallic ESR line shape is observed for more concentrated samples (x≥0.004), even though these systems are still in a reasonably dilute regime and show insulating dc electrical resistivity. Our data indicate that the Kondo insulating state is destroyed locally around impurities before a global percolation occurs. This result not only explains the discrepancy between dc and ac conductivity but also provides a scenario to explain the presence of quantum oscillations in magnetization in the absence of quantum oscillations in electrical resistivity.Instituto de Física Gleb Wataghin UNICAMPMax Planck Institute for Chemical Physics of SolidsLos Alamos National LaboratoryPOSMAT Faculdade de Ciências UNESP, C.P. 473Departamento de Física Faculdade de Ciências UNESP, C.P. 473Department of Physics and Astronomy University of CaliforniaPOSMAT Faculdade de Ciências UNESP, C.P. 473Departamento de Física Faculdade de Ciências UNESP, C.P. 473Universidade Estadual de Campinas (UNICAMP)Max Planck Institute for Chemical Physics of SolidsLos Alamos National LaboratoryUniversidade Estadual Paulista (UNESP)University of CaliforniaSouza, J. C.Rosa, P. F.S.Sichelschmidt, J.Carlone, M. [UNESP]Venegas, P. A. [UNESP]Malcolms, M. O.Menegasso, P. M.Urbano, R. R.Fisk, Z.Pagliuso, P. G.2022-04-28T19:40:15Z2022-04-28T19:40:15Z2020-11-03info:eu-repo/semantics/publishedVersioninfo:eu-repo/semantics/articlehttp://dx.doi.org/10.1103/PhysRevResearch.2.043181Physical Review Research, v. 2, n. 4, 2020.2643-1564http://hdl.handle.net/11449/22175210.1103/PhysRevResearch.2.0431812-s2.0-85106381837Scopusreponame:Repositório Institucional da UNESPinstname:Universidade Estadual Paulista (UNESP)instacron:UNESPengPhysical Review Researchinfo:eu-repo/semantics/openAccess2022-04-28T19:40:15Zoai:repositorio.unesp.br:11449/221752Repositório InstitucionalPUBhttp://repositorio.unesp.br/oai/requestopendoar:29462024-08-05T21:57:05.519316Repositório Institucional da UNESP - Universidade Estadual Paulista (UNESP)false
dc.title.none.fl_str_mv Metallic islands in the Kondo insulator SmB6
title Metallic islands in the Kondo insulator SmB6
spellingShingle Metallic islands in the Kondo insulator SmB6
Metallic islands in the Kondo insulator SmB6
Souza, J. C.
Souza, J. C.
title_short Metallic islands in the Kondo insulator SmB6
title_full Metallic islands in the Kondo insulator SmB6
title_fullStr Metallic islands in the Kondo insulator SmB6
Metallic islands in the Kondo insulator SmB6
title_full_unstemmed Metallic islands in the Kondo insulator SmB6
Metallic islands in the Kondo insulator SmB6
title_sort Metallic islands in the Kondo insulator SmB6
author Souza, J. C.
author_facet Souza, J. C.
Souza, J. C.
Rosa, P. F.S.
Sichelschmidt, J.
Carlone, M. [UNESP]
Venegas, P. A. [UNESP]
Malcolms, M. O.
Menegasso, P. M.
Urbano, R. R.
Fisk, Z.
Pagliuso, P. G.
Rosa, P. F.S.
Sichelschmidt, J.
Carlone, M. [UNESP]
Venegas, P. A. [UNESP]
Malcolms, M. O.
Menegasso, P. M.
Urbano, R. R.
Fisk, Z.
Pagliuso, P. G.
author_role author
author2 Rosa, P. F.S.
Sichelschmidt, J.
Carlone, M. [UNESP]
Venegas, P. A. [UNESP]
Malcolms, M. O.
Menegasso, P. M.
Urbano, R. R.
Fisk, Z.
Pagliuso, P. G.
author2_role author
author
author
author
author
author
author
author
author
dc.contributor.none.fl_str_mv Universidade Estadual de Campinas (UNICAMP)
Max Planck Institute for Chemical Physics of Solids
Los Alamos National Laboratory
Universidade Estadual Paulista (UNESP)
University of California
dc.contributor.author.fl_str_mv Souza, J. C.
Rosa, P. F.S.
Sichelschmidt, J.
Carlone, M. [UNESP]
Venegas, P. A. [UNESP]
Malcolms, M. O.
Menegasso, P. M.
Urbano, R. R.
Fisk, Z.
Pagliuso, P. G.
description The predicted interplay between Kondo physics and nontrivial topology in SmB6 has stimulated many experimental reports, some of which are in apparent contradiction. The origin of the dispute may lie in the fragility of the Kondo insulating phase in the presence of Sm vacancies (Kondo holes) and/or natural impurities, such as Gd3+. In this work, we locally investigate this fragility for Al flux grown Sm1-xGdxB6 single crystals (0≤x≤0.02) by combining electron spin resonance (ESR) and complementary bulk measurements. The Gd3+ ESR spectra in a highly dilute regime (x∼0.0004) display the features of an insulating cubic environment. Remarkably, a metallic ESR line shape is observed for more concentrated samples (x≥0.004), even though these systems are still in a reasonably dilute regime and show insulating dc electrical resistivity. Our data indicate that the Kondo insulating state is destroyed locally around impurities before a global percolation occurs. This result not only explains the discrepancy between dc and ac conductivity but also provides a scenario to explain the presence of quantum oscillations in magnetization in the absence of quantum oscillations in electrical resistivity.
publishDate 2020
dc.date.none.fl_str_mv 2020-11-03
2022-04-28T19:40:15Z
2022-04-28T19:40:15Z
dc.type.status.fl_str_mv info:eu-repo/semantics/publishedVersion
dc.type.driver.fl_str_mv info:eu-repo/semantics/article
format article
status_str publishedVersion
dc.identifier.uri.fl_str_mv http://dx.doi.org/10.1103/PhysRevResearch.2.043181
Physical Review Research, v. 2, n. 4, 2020.
2643-1564
http://hdl.handle.net/11449/221752
10.1103/PhysRevResearch.2.043181
2-s2.0-85106381837
url http://dx.doi.org/10.1103/PhysRevResearch.2.043181
http://hdl.handle.net/11449/221752
identifier_str_mv Physical Review Research, v. 2, n. 4, 2020.
2643-1564
10.1103/PhysRevResearch.2.043181
2-s2.0-85106381837
dc.language.iso.fl_str_mv eng
language eng
dc.relation.none.fl_str_mv Physical Review Research
dc.rights.driver.fl_str_mv info:eu-repo/semantics/openAccess
eu_rights_str_mv openAccess
dc.source.none.fl_str_mv Scopus
reponame:Repositório Institucional da UNESP
instname:Universidade Estadual Paulista (UNESP)
instacron:UNESP
instname_str Universidade Estadual Paulista (UNESP)
instacron_str UNESP
institution UNESP
reponame_str Repositório Institucional da UNESP
collection Repositório Institucional da UNESP
repository.name.fl_str_mv Repositório Institucional da UNESP - Universidade Estadual Paulista (UNESP)
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dc.identifier.doi.none.fl_str_mv 10.1103/PhysRevResearch.2.043181