Microwave-Assisted Synthesis of Zn2SnO4 Nanostructures for Photodegradation of Rhodamine B under UV and Sunlight

Detalhes bibliográficos
Autor(a) principal: Rovisco, Ana
Data de Publicação: 2022
Outros Autores: Morais, Maria, Branquinho, Rita, Fortunato, Elvira, Martins, Rodrigo, Barquinha, Pedro
Tipo de documento: Artigo
Idioma: eng
Título da fonte: Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos)
Texto Completo: http://hdl.handle.net/10362/143924
Resumo: Publisher Copyright: © 2022 by the authors. Licensee MDPI, Basel, Switzerland.
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spelling Microwave-Assisted Synthesis of Zn2SnO4 Nanostructures for Photodegradation of Rhodamine B under UV and Sunlightmicrowave-assisted hydrothermal synthesisnanoparticlesnanoplatesphotocatalysispolyhedronsrhodamine BZn2SnO4ZTOChemical Engineering(all)Materials Science(all)SDG 8 - Decent Work and Economic GrowthSDG 12 - Responsible Consumption and ProductionSDG 13 - Climate ActionPublisher Copyright: © 2022 by the authors. Licensee MDPI, Basel, Switzerland.The contamination of water resources by pollutants resulting from human activities represents a major concern nowadays. One promising alternative to solve this problem is the photocatalytic process, which has demonstrated very promising and efficient results. Oxide nanostructures are interesting alternatives for these applications since they present wide band gaps and high surface areas. Among the photocatalytic oxide nanostructures, zinc tin oxide (ZTO) presents itself as an eco-friendly alternative since its composition includes abundant and non-toxic zinc and tin, instead of critical elements. Moreover, ZTO nanostructures have a multiplicity of structures and morphologies possible to be obtained through low-cost solution-based syntheses. In this context, the current work presents an optimization of ZTO nanostructures (polyhedrons, nanoplates, and nanoparticles) obtained by microwave irradiation-assisted hydrothermal synthesis, toward photocatalytic applications. The nanostructures’ photocatalytic activity in the degradation of rhodamine B under both ultraviolet (UV) irradiation and natural sunlight was evaluated. Among the various morphologies, ZTO nanoparticles revealed the best performance, with degradation > 90% being achieved in 60 min under UV irradiation and in 90 min under natural sunlight. The eco-friendly production process and the demonstrated ability of these nanostructures to be used in various water decontamination processes reinforces their sustainability and the role they can play in a circular economy.CENIMAT-i3N - Centro de Investigação de Materiais (Lab. Associado I3N)DCM - Departamento de Ciência dos MateriaisUNINOVA-Instituto de Desenvolvimento de Novas TecnologiasRUNRovisco, AnaMorais, MariaBranquinho, RitaFortunato, ElviraMartins, RodrigoBarquinha, Pedro2022-09-21T22:37:44Z2022-06-202022-06-20T00:00:00Zinfo:eu-repo/semantics/publishedVersioninfo:eu-repo/semantics/article18application/pdfhttp://hdl.handle.net/10362/143924eng2079-4991PURE: 46646785https://doi.org/10.3390/nano12122119info:eu-repo/semantics/openAccessreponame:Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos)instname:Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informaçãoinstacron:RCAAP2024-03-11T05:22:54Zoai:run.unl.pt:10362/143924Portal AgregadorONGhttps://www.rcaap.pt/oai/openaireopendoar:71602024-03-20T03:51:13.204257Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos) - Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informaçãofalse
dc.title.none.fl_str_mv Microwave-Assisted Synthesis of Zn2SnO4 Nanostructures for Photodegradation of Rhodamine B under UV and Sunlight
title Microwave-Assisted Synthesis of Zn2SnO4 Nanostructures for Photodegradation of Rhodamine B under UV and Sunlight
spellingShingle Microwave-Assisted Synthesis of Zn2SnO4 Nanostructures for Photodegradation of Rhodamine B under UV and Sunlight
Rovisco, Ana
microwave-assisted hydrothermal synthesis
nanoparticles
nanoplates
photocatalysis
polyhedrons
rhodamine B
Zn2SnO4
ZTO
Chemical Engineering(all)
Materials Science(all)
SDG 8 - Decent Work and Economic Growth
SDG 12 - Responsible Consumption and Production
SDG 13 - Climate Action
title_short Microwave-Assisted Synthesis of Zn2SnO4 Nanostructures for Photodegradation of Rhodamine B under UV and Sunlight
title_full Microwave-Assisted Synthesis of Zn2SnO4 Nanostructures for Photodegradation of Rhodamine B under UV and Sunlight
title_fullStr Microwave-Assisted Synthesis of Zn2SnO4 Nanostructures for Photodegradation of Rhodamine B under UV and Sunlight
title_full_unstemmed Microwave-Assisted Synthesis of Zn2SnO4 Nanostructures for Photodegradation of Rhodamine B under UV and Sunlight
title_sort Microwave-Assisted Synthesis of Zn2SnO4 Nanostructures for Photodegradation of Rhodamine B under UV and Sunlight
author Rovisco, Ana
author_facet Rovisco, Ana
Morais, Maria
Branquinho, Rita
Fortunato, Elvira
Martins, Rodrigo
Barquinha, Pedro
author_role author
author2 Morais, Maria
Branquinho, Rita
Fortunato, Elvira
Martins, Rodrigo
Barquinha, Pedro
author2_role author
author
author
author
author
dc.contributor.none.fl_str_mv CENIMAT-i3N - Centro de Investigação de Materiais (Lab. Associado I3N)
DCM - Departamento de Ciência dos Materiais
UNINOVA-Instituto de Desenvolvimento de Novas Tecnologias
RUN
dc.contributor.author.fl_str_mv Rovisco, Ana
Morais, Maria
Branquinho, Rita
Fortunato, Elvira
Martins, Rodrigo
Barquinha, Pedro
dc.subject.por.fl_str_mv microwave-assisted hydrothermal synthesis
nanoparticles
nanoplates
photocatalysis
polyhedrons
rhodamine B
Zn2SnO4
ZTO
Chemical Engineering(all)
Materials Science(all)
SDG 8 - Decent Work and Economic Growth
SDG 12 - Responsible Consumption and Production
SDG 13 - Climate Action
topic microwave-assisted hydrothermal synthesis
nanoparticles
nanoplates
photocatalysis
polyhedrons
rhodamine B
Zn2SnO4
ZTO
Chemical Engineering(all)
Materials Science(all)
SDG 8 - Decent Work and Economic Growth
SDG 12 - Responsible Consumption and Production
SDG 13 - Climate Action
description Publisher Copyright: © 2022 by the authors. Licensee MDPI, Basel, Switzerland.
publishDate 2022
dc.date.none.fl_str_mv 2022-09-21T22:37:44Z
2022-06-20
2022-06-20T00:00:00Z
dc.type.status.fl_str_mv info:eu-repo/semantics/publishedVersion
dc.type.driver.fl_str_mv info:eu-repo/semantics/article
format article
status_str publishedVersion
dc.identifier.uri.fl_str_mv http://hdl.handle.net/10362/143924
url http://hdl.handle.net/10362/143924
dc.language.iso.fl_str_mv eng
language eng
dc.relation.none.fl_str_mv 2079-4991
PURE: 46646785
https://doi.org/10.3390/nano12122119
dc.rights.driver.fl_str_mv info:eu-repo/semantics/openAccess
eu_rights_str_mv openAccess
dc.format.none.fl_str_mv 18
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instname:Agência para a Sociedade do Conhecimento (UMIC) - FCT - Sociedade da Informação
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reponame_str Repositório Científico de Acesso Aberto de Portugal (Repositórios Cientìficos)
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